☆ 4.5 Review

A Review on CO2-Based Polyureas and Polyurea Hybrids

ASIAN JOURNAL OF ORGANIC CHEMISTRY (2022)

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Review Chemistry, Multidisciplinary

Homogeneous Catalysis for Sustainable Energy: Hydrogen and Methanol Economies, Fuels from Biomass, and Related Topics

Amit Kumar et al.

Summary: This article reviews recent developments of homogeneous catalysts in emerging applications of sustainable energy, with a focus on hydrogen storage, the methanol economy, and the production of conventional fuels from biomass or lower alkanes. Additionally, the production of ethylene glycol from CO and H-2 is discussed, with particular emphasis on well-defined transition metal complexes, such as pincer complexes, due to their high activity and well-studied mechanisms.

CHEMICAL REVIEWS (2022)

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Review Polymer Science

Hybrid Nonisocyanate Polyurethanes (H-NIPUs): A Pathway towards a Broad Range of Novel Materials

Boris Bizet et al.

Summary: This review summarizes the latest advancements in the development of hybrid nonisocyanate polyurethanes (NIPUs) by combining them with other polymers, such as epoxy, polyacrylic, and silicium-containing polymers. The potential of combining NIPUs with biopolymers is also discussed. The study highlights the importance of synergistic combination of NIPUs with other polymers in the formation of novel materials.

MACROMOLECULAR CHEMISTRY AND PHYSICS (2022)

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Article Materials Science, Multidisciplinary

Organic-Inorganic Polyureas with POSS Cages in the Main Chains via Polycondensation of Diamines with Carbon Dioxide

Bingjie Zhao et al.

Summary: Linear organic-inorganic polyureas (PUreas) with polyhedral oligomeric silsesquioxane (POSS) cages in the main chains were synthesized via polycondensation of diamines with carbon dioxide (CO2). The PUreas exhibited microphase separation with aggregated POSS cages forming spherical microdomains. The introduction of POSS transformed PUrea from a liquid to an elastic solid, behaving as a cross-linked elastomer at room temperature. Additionally, the PUreas displayed self-healing properties through the dynamic exchange of multiple hydrogen bonds.

ACS APPLIED POLYMER MATERIALS (2022)

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Article Materials Science, Multidisciplinary

Biomass-Based Polyureas Derived from Rigid Furfurylamine and Isomannide

Yuan Jiang et al.

Summary: In this study, biomass-based polyureas were prepared using furfurylamine and isomannide-derived dicarbamates. These polyureas exhibited good thermal stability and glass-transition temperatures, making them suitable for various applications.

ACS APPLIED POLYMER MATERIALS (2022)

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Review Chemistry, Multidisciplinary

Exovinylene Cyclic Carbonates: Multifaceted CO2-Based Building Blocks for Modern Chemistry and Polymer Science

Charlene Ngassam Tounzoua et al.

Summary: This Review summarizes the recent advances in the synthesis of exovinylene cyclic carbonates, which can be produced from renewable and inexhaustible carbon dioxide as an alternative to fossil resources. The article focuses on describing the catalysts needed for their preparation and discussing the unique reactivity of these CO2-based heterocycles for the construction of diverse organic building blocks and (functional) polymers. The challenges and the future perspectives in the field are also discussed.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2022)

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Article Polymer Science

Novel carbon dioxide based poly(hydroxyurethane-urea)s: Synthesis and properties

Shan Jiang et al.

Summary: Poly(hydroxyurethane-urea)s (PHUUs) with complementary properties to poly(hydroxyurethane)s (PHUs) and polyureas have great potential for practical applications. Novel PHUUs were synthesized through polyaddition reaction using 5-membered dicyclic carbonates and amino terminal polyurea oligomers. The introduction of urea moieties improved surface hydrophobicity and thermal properties, and the structure of selected diamine influenced glass transition temperature and mechanical properties of PHUUs.

POLYMER (2022)

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Article Chemistry, Physical

Defect-Assisted Electron Tunneling for Photoelectrochemical CO2 Reduction to Ethanol at Low Overpotentials

Miao Kan et al.

Summary: A Si/ZnO/Cu2O p-n-p heterojunction potential well with electron tunnels is fabricated for selective photoelectrochemical CO2 reduction to ethanol. The confined electron energy in tunneling allows for high selectivity in ethanol production, with a Faradaic efficiency of over 60%.

ADVANCED ENERGY MATERIALS (2022)

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Article Chemistry, Multidisciplinary

Highly Branched Polyurea-Based Resins: Clean Synthesis and Wood Bonding Performance

Shuyang Jiang et al.

Summary: The development of green and safe adhesives with high performance is crucial for the sustainability of the wood industry. In this study, highly branched polyureas (HBPUs) were synthesized and used as formaldehyde-free wood adhesives, demonstrating good bonding performance. Additionally, HBPU-formaldehyde (HBPUF) resins were synthesized and showed better bonding performance and lower formaldehyde emission levels compared to conventional urea-formaldehyde (UF) resin.

ACS SUSTAINABLE CHEMISTRY & ENGINEERING (2022)

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Article Chemistry, Physical

Highly stable and selective layered Co-Al-O catalysts for low-temperature CO2 methanation

Zhihao Liu et al.

Summary: A series of layered Co-Al-O catalysts were prepared via a hydrothermal method and reduced at different temperatures. The results showed that the Co-0 content and basic sites on the catalysts increased and then decreased with the reduction temperature, leading to effective hydrogen dissociation and CO2 adsorption. The CoAl-O-600 catalyst exhibited superior performance in CO2 methanation at low temperature and showed excellent resistance to coking and sintering.

APPLIED CATALYSIS B-ENVIRONMENTAL (2022)

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Article Engineering, Environmental

Efficient chemical fixation of CO2 to form switchable ionic liquid to synthesize benzimidazolones under mild conditions

Leizhi Zheng et al.

Summary: The synthesis of benzimidazolone derivatives via the carbonylation of ophenylenediamines with CO2 under mild conditions using DBN as a superbase and the formation of switchable ionic liquids provides a sustainable technique for the production of benzimidazolones.

CHEMICAL ENGINEERING JOURNAL (2022)

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Article Chemistry, Physical

Cyclic oligourea synthesized from CO2: Purification, characterization and properties

Ruhui Shi et al.

Summary: In this study, a cyclic oligourea was synthesized by polycondensation of CO2 with TTD and separated and purified to obtain a high purity product. The cyclic oligourea showed distinct differences in structure and properties compared to its linear analogue, adding a new member to the cyclic polymer family.

GREEN ENERGY & ENVIRONMENT (2022)

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Article Engineering, Environmental

Chemical recycling of poly-(bisphenol A carbonate) by diaminolysis: A new carbon-saving synthetic entry into non-isocyanate polyureas (NIPUreas)

Eugenio Quaranta et al.

Summary: This study presents a novel approach to valorize potentially hazardous PC wastes by regenerating BPA monomers and repurposing waste PC into PUs through a non-isocyanate route. The PUs obtained showed thermally stability and high processing suitability, making them promising materials for various applications.

JOURNAL OF HAZARDOUS MATERIALS (2021)

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Article Chemistry, Multidisciplinary

Direct synthesis of polyureas from the dehydrogenative coupling of diamines and methanol

Amit Kumar et al.

Summary: This study presents a novel method for the direct synthesis of polyureas from diamines and methanol using a ruthenium pincer catalyst. By replacing toxic diisocyanates with renewable and less toxic methanol, the overall process becomes safer and more sustainable. Additionally, the method has been shown to be versatile by synthesizing renewable, chiral, and C-13-labeled polyureas.

CHEMICAL COMMUNICATIONS (2021)

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Article Materials Science, Multidisciplinary

Superstrong Adhesive of Isocyanate-Free Polyurea with a Branched Structure

Hongxing Yang et al.

Summary: This study verified the relationship between branching degree and bonding performance by synthesizing branched polyureas with different branching degrees. The results showed that the bonding strength of branched polyurea increased with an increase of terminal functional groups.

ACS APPLIED POLYMER MATERIALS (2021)

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Article Chemistry, Multidisciplinary

A self-healing and recyclable polyurethane-urea Diels-Alder adduct synthesized from carbon dioxide and furfuryl amine

Peixuan Wu et al.

Summary: The synthesis of a new environmentally friendly, self-healing, and recyclable polymeric material PUUa-DA, using CO2 and bio-based furfuryl amine, demonstrates high thermal stability and mechanical properties. The incorporation of reversible hydrogen bonds and heat-responsive Diels-Alder bonds enables 94% recovery of tensile strength upon heating, making it a potential functional material for various practical applications.

GREEN CHEMISTRY (2021)

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Article Chemistry, Multidisciplinary

Novel Highly Branched Polymer Wood Adhesive Resin

Taohong Li et al.

ACS SUSTAINABLE CHEMISTRY & ENGINEERING (2020)

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Article Polymer Science

Hybrid polyhydroxyurethanes: How to overcome limitations and reach cutting edge properties?

Yvan Ecochard et al.

EUROPEAN POLYMER JOURNAL (2020)

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Article Chemistry, Multidisciplinary

New Kind of Thermoplastic Polyurea Elastomers Synthesized from CO2 and with Self-Healing Properties

Peixuan Wu et al.

ACS SUSTAINABLE CHEMISTRY & ENGINEERING (2020)

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Article Chemistry, Multidisciplinary

Urea and Polyurea Production: An Innovative Solvent- and Catalyst-Free Approach through Catechol Carbonate

Michelina Soccio et al.

ACS SUSTAINABLE CHEMISTRY & ENGINEERING (2020)

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Article Chemistry, Multidisciplinary

Synthesis of Polyurea Thermoplastics through a Nonisocyanate Route Using CO2 and Aliphatic Diamines

Ruhui Shi et al.

ACS SUSTAINABLE CHEMISTRY & ENGINEERING (2020)

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Article Chemistry, Multidisciplinary

Isocyanate- and solvent-free synthesis of melt processible polyurea elastomers derived from urea as a monomer

B. Tyler White et al.

RSC ADVANCES (2020)

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Review Chemistry, Multidisciplinary

New Polymerizations Based on Green Monomer of Carbon Dioxide

Bo Song et al.

ACTA CHIMICA SINICA (2020)

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Article Polymer Science

Amorphous and Crystallizable Thermoplastic Polyureas Synthesized through a One-pot Non-isocyanate Route

Jia-Long Ban et al.

CHINESE JOURNAL OF POLYMER SCIENCE (2019)

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Review Chemistry, Multidisciplinary

CO2 Capture and in situ Catalytic Transformation

Hong-Chen Fu et al.

FRONTIERS IN CHEMISTRY (2019)

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Article Nanoscience & Nanotechnology

Direct Synthesis of Polyurea Thermoplastics from CO2 and Diamines

Shan Jiang et al.

ACS APPLIED MATERIALS & INTERFACES (2019)

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Article Chemistry, Applied

Synthesis of Polyurea via the Addition of Carbon Dioxide to a Diamine Catalyzed by Organic and Inorganic Bases

Pei-Xuan Wu et al.

ADVANCED SYNTHESIS & CATALYSIS (2019)

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Review Chemistry, Multidisciplinary

Advances in the use of CO2 as a renewable feedstock for the synthesis of polymers

Bruno Grignard et al.

CHEMICAL SOCIETY REVIEWS (2019)

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Article Chemistry, Multidisciplinary

Superstretchable, Self-Healing Polymeric Elastomers with Tunable Properties

Peng-Fei Cao et al.

ADVANCED FUNCTIONAL MATERIALS (2018)

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Article Chemistry, Multidisciplinary

Synthesis and characterization of isocyanate-free polyureas

Joseph M. Dennis et al.

GREEN CHEMISTRY (2018)

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Article Polymer Science

Non-isocyanate strategy for anionically stabilized water-borne polyurea dispersions and coatings

Shuang Ma et al.

JOURNAL OF POLYMER SCIENCE PART A-POLYMER CHEMISTRY (2018)

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Article Polymer Science

t-Butyl-Oxycarbonylated Diamines as Building Blocks for Isocyanate-Free Polyurethane/Urea Dispersions and Coatings

Shuang Ma et al.

MACROMOLECULAR RAPID COMMUNICATIONS (2018)

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Article Polymer Science

Unexpected Synthesis of Segmented Poly(hydroxyurea-urethane)s from Dicyclic Carbonates and Diamines by Organocatalysis

Amaury Bossion et al.

MACROMOLECULES (2018)

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Article Chemistry, Multidisciplinary

Transformation of CO2 into polyureas with 3-amino-1,2,4-triazole potassium as a solid base catalyst

Peixue Wang et al.

NEW JOURNAL OF CHEMISTRY (2018)

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Article Polymer Science

Urea as a monomer for isocyanate-free synthesis of segmented poly (dimethyl siloxane) polyureas

Justin M. Sirrine et al.

POLYMER (2018)

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Article Chemistry, Multidisciplinary

Catalytic polymerization of CO2 to polyureas over K3PO4 catalyst

Peixue Wang et al.

JOURNAL OF CO2 UTILIZATION (2018)

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Article Chemistry, Multidisciplinary

Isocyanate-Free Approach to Water-Borne Polyurea Dispersions and Coatings

Shuang Ma et al.

CHEMSUSCHEM (2018)

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Article Materials Science, Multidisciplinary

Isocyanate- and Solvent-Free Route to Thermoplastic Poly(amide-urea) Derived from Renewable Resources

Benjamin S. Ritter et al.

MACROMOLECULAR MATERIALS AND ENGINEERING (2017)

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Article Polymer Science

Non-isocyanate thermoplastic polyureas (NIPUreas) through a methyl carbamate metathesis polymerization

Nasreddine Kebir et al.

EUROPEAN POLYMER JOURNAL (2017)

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Article Chemistry, Multidisciplinary

Polyureas derived from CO2 and diamines: highly efficient catalysts for C-H arylation of benzene

Zhenghui Liu et al.

NEW JOURNAL OF CHEMISTRY (2017)

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Article Chemistry, Multidisciplinary

Synthesis of polyureas with CO2 as carbonyl building block and their high performances

Zhong Ying et al.

JOURNAL OF CO2 UTILIZATION (2017)

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Article Chemistry, Physical

Synthesis of polyurea from 1,6-hexanediamine with CO2 through a two-step polymerization

Shan Jiang et al.

GREEN ENERGY & ENVIRONMENT (2017)

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Article Polymer Science

Synthesis and properties of allyl terminated renewable non-isocyanate polyurethanes (NIPUs) and polyureas (NIPUreas) and study of their photo-crosslinking

Amelie Martin et al.

EUROPEAN POLYMER JOURNAL (2016)

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Article Chemistry, Multidisciplinary

Carbon dioxide as a sustainable resource for macrocyclic oligourea

Z. Ying et al.

GREEN CHEMISTRY (2016)

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Article Chemistry, Multidisciplinary

Synthesis of polyurethane-urea from double CO2-route oligomers

Zhong Ying et al.

GREEN CHEMISTRY (2016)

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Article Engineering, Chemical

Crystallizable and Tough Aliphatic Thermoplastic Polyureas Synthesized through a Nonisocyanate Route

Suqing Li et al.

INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH (2016)

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Article Polymer Science

Poly(urea ester): A family of biodegradable polymers with high melting temperatures

Donglin Tang et al.

JOURNAL OF POLYMER SCIENCE PART A-POLYMER CHEMISTRY (2016)

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Article Chemistry, Physical

Catalysts for Isocyanate-Free Polyurea Synthesis: Mechanism and Application

Shuang Ma et al.

ACS CATALYSIS (2016)

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Article Chemistry, Multidisciplinary

Green synthesis of polyureas from CO2 and diamines with a functional ionic liquid as the catalyst

Peixue Wang et al.

RSC ADVANCES (2016)

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Article Chemistry, Multidisciplinary

Synthesis of a novel hydrophobic polyurea gel from CO2 and amino-modified polysiloxane

Zhong Ying et al.

JOURNAL OF CO2 UTILIZATION (2016)

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Review Chemistry, Multidisciplinary

Isocyanate-Free Routes to Polyurethanes and Poly(hydroxy Urethane)s

Lise Maisonneuve et al.

CHEMICAL REVIEWS (2015)

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Article Chemistry, Multidisciplinary

[n]-Oligourea-Based Green Sorbents with Enhanced CO2 Sorption Capacity

Abdussalam K. Qaroush et al.

CHEMSUSCHEM (2015)

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Article Polymer Science

Poly(hydroxy urethane)s based on renewable diglycerol dicarbonate

Julien L. J. van Velthoven et al.

EUROPEAN POLYMER JOURNAL (2015)

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Article Chemistry, Multidisciplinary

Quantitative synthesis of bis(cyclic carbonate) s by iron catalyst for non-isocyanate polyurethane synthesis

Xingfeng Sheng et al.

GREEN CHEMISTRY (2015)

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Article Chemistry, Multidisciplinary

Enhancing Mechanical Performance of a Covalent Self-Healing Material by Sacrificial Noncovalent Bonds

James A. Neal et al.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2015)

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Article Chemistry, Multidisciplinary

Utilization of carbon dioxide to build a basic block for polymeric materials: an isocyanate-free route to synthesize a soluble oligourea

Zhong Ying et al.

RSC ADVANCES (2015)

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Article Chemistry, Multidisciplinary

Aliphatic thermoplastic polyurethane-ureas and polyureas synthesized through a non-isocyanate route

Suqing Li et al.

RSC ADVANCES (2015)

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Article Chemistry, Physical

Polyurea-supported metal nanocatalysts: Synthesis, characterization and application in selective hydrogenation of o-chloronitrobenzene

Leiduan Hao et al.

JOURNAL OF COLLOID AND INTERFACE SCIENCE (2014)

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Article Polymer Science

High-Performance Segmented Polyurea by Transesterification of Diphenyl Carbonates with Aliphatic Diamines

Wen Chen Pan et al.

JOURNAL OF POLYMER SCIENCE PART A-POLYMER CHEMISTRY (2014)

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Review Chemistry, Multidisciplinary

On the Versatility of Urethane/Urea Bonds: Reversibility, Blocked Isocyanate, and Non-isocyanate Polyurethane

Etienne Delebecq et al.

CHEMICAL REVIEWS (2013)

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Article Chemistry, Physical

Highly efficient isocyanate-free microwave-assisted synthesis of [6]-oligourea

Abdussalam K. Qaroush et al.

CATALYSIS SCIENCE & TECHNOLOGY (2013)

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Article Chemistry, Multidisciplinary

A new route of CO2 catalytic activation: syntheses of N-substituted carbamates from dialkyl carbonates and polyureas

Jianpeng Shang et al.

GREEN CHEMISTRY (2012)

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Article Polymer Science

Chitosan-graft-poly(acrylic acid)/rice husk ash based superabsorbent hydrogel composite: preparation and characterization

Francisco H. A. Rodrigues et al.

JOURNAL OF POLYMER RESEARCH (2012)

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Article Chemistry, Physical

Polyureas from diamines and carbon dioxide: synthesis, structures and properties

Chaoyong Wu et al.

PHYSICAL CHEMISTRY CHEMICAL PHYSICS (2012)

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Article Polymer Science

Well-defined Biobased Segmented Polyureas Synthesis via a TBD-catalyzed Isocyanate-free Route

Donglin Tang et al.

MACROMOLECULAR RAPID COMMUNICATIONS (2011)

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Review Chemistry, Multidisciplinary

Generation, Capture, and Utilization of Industrial Carbon Dioxide

Andrew J. Hunt et al.

CHEMSUSCHEM (2010)

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