Spent Li-Ion Battery Electrode Material with Lithium Nickel Manganese Cobalt Oxide as a Reusable Catalyst for Oxidation of Biofurans

Article Chemistry, Multidisciplinary

Direct Reuse of Spent Lithium-Ion Batteries as an Efficient Heterogeneous Catalyst for the Reductive Upgrading of Biomass-Derived Furfural

Emilia Paone et al.

Summary: After appropriate thermal treatments, spent Li-ion batteries can be directly used as catalysts for selective hydrogenation, showing the potential of using and recycling the batteries as precious catalytic materials.

ACS SUSTAINABLE CHEMISTRY & ENGINEERING (2022)

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Article Materials Science, Ceramics

Interactions of Li2O volatilized from ternary lithium-ion battery cathode materials with mullite saggar materials during calcination

Kun Xiang et al.

Summary: In recent years, the increasing demand for refractory kiln saggars has accompanied the rapid development of Li(NixCoyMn1-x-y)O2 (LNCM) materials in ternary lithium-ion batteries. However, saggars used for firing ternary Li-ion battery cathode materials often suffer from severe corrosion and spalling. In this study, non-contact corrosion experiments were conducted to investigate the damage mechanism of mullite saggar materials during interaction with LNCM materials. The phase composition and microstructure of the mullite saggars were analyzed to gain insights into the causes of the deterioration during corrosion.

CERAMICS INTERNATIONAL (2022)

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Article Environmental Sciences

Leaching with mixed organic acids and sulfuric acid to recover cobalt and lithium from lithium ion batteries

Patricia Moises Urias et al.

Summary: This study evaluated the recovery of Co and Li from Li-ion batteries using hydrometallurgy, finding that a leaching solution composed of H(2)SO(4) and fermentation effluent showed high potential for metals recovery. The optimal leaching conditions were determined through Central Composite Designs, leading to a high recovery level of Co (93.35%) and Li (90.50%). Additionally, the presence of a mixture of organic acids and other compounds in the fermentation effluent was found to improve the leaching process.

ENVIRONMENTAL TECHNOLOGY (2021)

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Review Chemistry, Applied

Recent progress on the recycling technology of Li-ion batteries

Yuqing Wang et al.

Summary: This review comprehensively summarizes the recycling technologies for LiNixCoyMnzO2 and LiFePO4-based LIBs, as well as exhausted anode materials, and discusses the challenges and possible strategies for industrial-scale application. The closed-loop strategy for cycling cathode materials is highlighted as an ideal approach for its economic benefit and environmental friendliness.

JOURNAL OF ENERGY CHEMISTRY (2021)

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Article Chemistry, Multidisciplinary

Spent Li-Ion Battery Graphite Turned Into Valuable and Active Catalyst for Electrochemical Oxygen Reduction

Kerli Liivand et al.

Summary: Recycling spent LIBs graphite as a valuable catalyst material for electrochemical reactions shows great potential and importance in reducing waste and reapplying the material for various applications.

CHEMSUSCHEM (2021)

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Article Agricultural Engineering

Catalytic upgrading of biomass derived furans

Fang Deng et al.

Summary: This article covers the catalytic upgrading reactions of biomass-derived renewable furan derivatives furfural and 5-hydroxymethylfurfural, with a focus on developments in the last five years. It also discusses the importance of this renewable feedstock class, preparation methods from monosaccharides, and the diversity of possible transformations. Recent advances in catalytic reductions, oxidations, and carbon number upgrading of biofurans are reviewed, highlighting the progress in developing more stable value-added derivatives.

INDUSTRIAL CROPS AND PRODUCTS (2021)

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Review Chemistry, Physical

Sustainable Li-Ion Batteries: Chemistry and Recycling

Jedrzej Piatek et al.

Summary: The commercial success of Li-ion batteries in the 1990s has led to environmental hazards from disposed batteries, raising questions about the greenness of current recycling technologies. Although industrially applied recycling technologies may have high overall efficiency, they often lack true circularity principles, which calls for a shift towards more sustainable and energy-efficient processes in the recycling of LIBs.

ADVANCED ENERGY MATERIALS (2021)

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Article Chemistry, Multidisciplinary

Upgrading of Light Bio-oil from Solvothermolysis Liquefaction of an Oil Palm Empty Fruit Bunch in Glycerol by Catalytic Hydrodeoxygenation Using NiMo/Al2O3 or CoMo/Al2O3 Catalysts

Chutanan Muangsuwan et al.

Summary: The hydrodeoxygenation process of bio-oil derived from palm empty fruit bunch in glycerol was studied using Ni- and Co-based catalysts on an Al2O3 support in a rotating-bed reactor. The NiMo/Al2O3 catalyst showed the most promising results with improved bio-oil quality in terms of oxygen reduction and increased high heating value. The olefins cyclopentanone and cyclopentene were identified as the main components in the hydrodeoxygenated bio-oil, which can be used for the synthesis of jet-fuel range cycloalkanes.

ACS OMEGA (2021)

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Review Chemistry, Applied

Cellulose and cellulose derivatives: Different colloidal states and food-related applications

Xiangxiang He et al.

Summary: The development of new sources and isolation processes has significantly enhanced cellulose production in various colloidal states. Understanding the correlation between the colloidal states of cellulose and its applications, particularly in the food industry, is essential for improving functional and nutritional properties of food systems. Further research is needed to control and improve the colloidal states of cellulose for enhanced food functionality and nutrition.

CARBOHYDRATE POLYMERS (2021)

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Review Green & Sustainable Science & Technology

Lithium extraction from water lithium resources through green electrochemical-battery approaches: A comprehensive review

Ye Zhang et al.

Summary: The growing market demand for lithium, especially for applications like lithium-ion batteries, highlights the importance of lithium production. Extraction of lithium from water resources, particularly those with high Mg/Li ratios, is becoming more popular due to its low cost and abundant reserves. Among various aqueous lithium-extraction methods, the electrochemical-battery approach is considered the most promising due to its excellent lithium selectivity, high insertion capacity, low energy consumption, high reversibility, and eco-friendliness. Future research should focus on enhancing battery-system stability, process optimization, and reducing operating costs.

JOURNAL OF CLEANER PRODUCTION (2021)

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Article Engineering, Chemical

Ultrasonic-assisted leaching of valuable metals from spent lithium-ion batteries using organic additives

Shuxuan Yan et al.

Summary: The study successfully achieved sustainable recycling of valuable metals from spent lithium-ion batteries using mixed organic acids and bagasse pith as leachants and reductants, with reduced acid consumption and mild leaching conditions for efficient metal dissolution.

SEPARATION AND PURIFICATION TECHNOLOGY (2021)

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Review Energy & Fuels

A review of recycling spent lithium-ion battery cathode materials using hydrometallurgical treatments

Joey Chung-Yen Jung et al.

Summary: With the growing market share of lithium-ion batteries, recycling of spent batteries has become necessary. Various metals can be extracted from these batteries using chemical leaching. This paper provides a comprehensive review of hydrometallurgical technologies for recycling spent lithium-ion cathode materials.

JOURNAL OF ENERGY STORAGE (2021)

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Editorial Material Chemistry, Multidisciplinary

Li-ion battery recycling challenges

Xiaotu Ma et al.

Summary: Given the increasing electrification of vehicles and the mass generation of spent lithium-ion batteries, recycling of LIBs is crucial. However, industrial-level recycling is challenging due to various factors that make large-scale recycling difficult while maintaining economic viability. Addressing these challenges and providing guidance towards solutions and future work is essential.

CHEM (2021)

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Article Engineering, Chemical

Catalytic cascade acetylation-alkylation of biofuran to C17 diesel precursor enabled by a budget acid-switchable catalyst

Chuanhui Li et al.

Summary: Lignocellulosic biomass is a promising feedstock for the synthesis of value-added chemicals and biofuels, but the lack of sufficient carbon-chain length in biomass derivatives poses challenges for producing high-quality diesel fuels. This study successfully synthesized a C-17 diesel precursor TEMF from the cascade acetylation-hydroxyalkylation/alkylation of bio-based 2-methylfuran with acetic anhydride catalyzed by acid-treated montmorillonite, and investigated the catalytic mechanism and the influence of different acid species on the reaction process. A synergistic effect was observed in enabling the synthesis of TEMF, with different acid species mainly catalyzing different steps of the reaction.

CHINESE JOURNAL OF CHEMICAL ENGINEERING (2021)

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Article Engineering, Environmental

Direct recovery of degraded LiCoO2 cathode material from spent lithium-ion batteries: Efficient impurity removal toward practical applications

Huimeng Yang et al.

Summary: This study presents a strategy for directly removing complex impurities and repairing degraded LiCoO2, achieving high recovery rate and excellent performance. The regenerated LiCoO2 exhibits high reversible capacity, cycling stability, and rate capability, comparable to commercial materials.

WASTE MANAGEMENT (2021)

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Review Chemistry, Multidisciplinary

Sustainable Recycling Technology for Li-Ion Batteries and Beyond: Challenges and Future Prospects

Ersha Fan et al.

CHEMICAL REVIEWS (2020)

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Article Metallurgy & Metallurgical Engineering

Selective recovery of valuable metals from industrial waste lithium-ion batteries using citric acid under reductive conditions: Leaching optimization and kinetic analysis

Fei Meng et al.

HYDROMETALLURGY (2020)

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Article Engineering, Environmental

Recycling of cathode material from spent lithium ion batteries using an ultrasound-assisted DL-malic acid leaching system

Peichao Ning et al.

WASTE MANAGEMENT (2020)

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Article Engineering, Environmental

Synergistic leaching of valuable metals from spent Li-ion batteries using sulfuric acid- L-ascorbic acid system

Dongdong Chen et al.

CHEMICAL ENGINEERING JOURNAL (2020)

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Article Chemistry, Multidisciplinary

Selective Recovery of Lithium from Spent Lithium-Ion Batteries by Coupling Advanced Oxidation Processes and Chemical Leaching Processes

Weiguang Lv et al.

ACS SUSTAINABLE CHEMISTRY & ENGINEERING (2020)

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Review Chemistry, Physical

Recent advances in catalytic oxidation of 5-hydroxymethylfurfural

Deyang Zhao et al.

MOLECULAR CATALYSIS (2020)

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Review Chemistry, Multidisciplinary

Polymer Electrolytes for Lithium-Based Batteries: Advances and Prospects

Dong Zhou et al.

CHEM (2019)

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Article Green & Sustainable Science & Technology

Bronsted acidic ionic liquid catalyzed one-pot conversion of cellulose to furanic biocrude and identification of the products using LC-MS

Ananda S. Amarasekara et al.

RENEWABLE ENERGY (2019)

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Article Agricultural Engineering

Acidic ionic liquid catalyzed liquefaction of untreated switchgrass biomass in acetone and Pd-La(OTf)3 catalyzed reduction of the products

Ananda S. Amarasekara et al.

BIOMASS & BIOENERGY (2019)

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Article Nanoscience & Nanotechnology

Understanding the Electrode/Electrolyte Interface Layer on the Li-Rich Nickel Manganese Cobalt Layered Oxide Cathode by XPS

Maral Hekmatfar et al.

ACS APPLIED MATERIALS & INTERFACES (2019)

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Article Green & Sustainable Science & Technology

Recovery of Laminar LiCoO2 Materials from Spent Mobile Phone Batteries by High-Temperature Calcination

Sayed M. Badawy et al.

JOURNAL OF SUSTAINABLE METALLURGY (2019)

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Article Multidisciplinary Sciences

Kinetics and mechanism of the solid-acid catalyzed one-pot conversion of d-fructose to 5, 5′-[oxybis(methylene)]bis[2-furaldehyde] in dimethyl sulfoxide

Ananda S. Amarasekara et al.

SN APPLIED SCIENCES (2019)

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Article Chemistry, Physical

1-(Alkylsulfonic)-3-methylimidazolium chloride Bronsted acidic ionic liquid catalyzed hydrogen peroxide oxidations of biomass derived furan aldehydes

Ananda S. Amarasekara et al.

CATALYSIS COMMUNICATIONS (2018)

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Review Chemistry, Physical

Metal Catalysts for the Efficient Transformation of Biomass-derived HMF and Furfural to Value Added Chemicals

Kavita Gupta et al.

CHEMCATCHEM (2018)

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Article Green & Sustainable Science & Technology

Selective recovery of valuable metals from spent lithium-ion batteries - Process development and kinetics evaluation

Wenfang Gao et al.

JOURNAL OF CLEANER PRODUCTION (2018)

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Review Electrochemistry

Recent Advancements in Polymer-Based Composite Electrolytes for Rechargeable Lithium Batteries

Shuang-Jie Tan et al.

ELECTROCHEMICAL ENERGY REVIEWS (2018)

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Article Chemistry, Multidisciplinary

A two-step efficient preparation of a renewable dicarboxylic acid monomer 5,5′-[oxybis(methylene)]bis[2-furancarboxylic acid] from D-fructose and its application in polyester synthesis

Ananda S. Amarasekara et al.

GREEN CHEMISTRY (2017)

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Article Chemistry, Physical

Furfural: A Promising Platform Compound for Sustainable Production of C4 and C5 Chemicals

Xiaodan Li et al.

ACS CATALYSIS (2016)

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Review Chemistry, Physical

Polymer electrolytes for lithium polymer batteries

Lizhen Long et al.

JOURNAL OF MATERIALS CHEMISTRY A (2016)

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Article Chemistry, Applied

Hydrolysis of cellulose catalyzed by novel acidic ionic liquids

Kelei Zhuo et al.

CARBOHYDRATE POLYMERS (2015)

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Article Agricultural Engineering

NaOH catalyzed condensation reactions between levulinic acid and biomass derived furan-aldehydes in water

Ananda S. Amarasekara et al.

INDUSTRIAL CROPS AND PRODUCTS (2015)

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Article Engineering, Environmental

Potential Environmental and Human Health Impacts of Rechargeable Lithium Batteries in Electronic Waste

Daniel Hsing Po Kang et al.

ENVIRONMENTAL SCIENCE & TECHNOLOGY (2013)

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Article Chemistry, Multidisciplinary

Selective oxidation of HMF to DFF using Ru/γ-alumina catalyst in moderate boiling solvents toward industrial production

Churchil A. Antonyraj et al.

JOURNAL OF INDUSTRIAL AND ENGINEERING CHEMISTRY (2013)

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Article Engineering, Chemical

Degradation of Cellulose in Dilute Aqueous Solutions of Acidic Ionic Liquid 1-(1-Propylsulfonic)-3-methylimidazolium Chloride, and p-Toluenesulfonic Acid at Moderate Temperatures and Pressures

Ananda S. Amarasekara et al.

INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH (2011)

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Article Polymer Science

Synthesis and Characterization of Poly(2,5-furan dicarboxylate)s Based on a Variety of Diols

Monica Gomes et al.

JOURNAL OF POLYMER SCIENCE PART A-POLYMER CHEMISTRY (2011)

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Review Chemistry, Physical

Biomass into chemicals: Conversion of sugars to furan derivatives by catalytic processes

Xinli Tong et al.

APPLIED CATALYSIS A-GENERAL (2010)

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Article Chemistry, Applied

Homogeneous phase synthesis of cellulose carbamate silica hybrid materials using 1-n-butyl-3-methylimidazolium chloride ionic liquid medium

Ananda S. Amarasekara et al.

CARBOHYDRATE POLYMERS (2009)

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Article Engineering, Chemical

Process integration for the conversion of glucose to 2,5-furandicarboxylic acid

A. Boisen et al.

CHEMICAL ENGINEERING RESEARCH & DESIGN (2009)

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Article Polymer Science

Renewable resources based polymers: Synthesis and characterization of 2,5-diformylfuran-urea resin

Ananda S. Amarasekara et al.

EUROPEAN POLYMER JOURNAL (2009)

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Article Engineering, Chemical

Hydrolysis and Decomposition of Cellulose in Bronsted Acidic Ionic Liquids Under Mild Conditions

Ananda S. Amarasekara et al.

INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH (2009)

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Article Chemistry, Physical

Efficient oxidation of 5-hydroxymethylfurfural to 2,5-diformylfuran using Mn(III)-salen catalysts

Ananda S. Amarasekara et al.

CATALYSIS COMMUNICATIONS (2008)

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Article Chemistry, Physical

Hydrothermal syntheses of layered lithium nickel manganese oxides from mixed layered Ni(OH)2 -: Manganese oxides

YH Xu et al.

CHEMISTRY OF MATERIALS (2002)

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Spent Li-Ion Battery Electrode Material with Lithium Nickel Manganese Cobalt Oxide as a Reusable Catalyst for Oxidation of Biofurans

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