期刊
ORGANIC LETTERS
卷 24, 期 42, 页码 7732-7736出版社
AMER CHEMICAL SOC
DOI: 10.1021/acs.orglett.2c02933
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资金
- National Natural Science Foundation of China [22171277, 22101291, 21821002]
- Shanghai Rising-Star Program [20QA1411400]
- Chinese Academy of Sciences [QYZDJSSWSLH055]
- Shanghai Institute of Organic Chemistry, State Key Laboratory of Organometallic Chemistry
In this study, a class of bifunctional monoprotected amino-imidazoline (MPAI) ligands were developed and applied in Pd-catalyzed C(sp(3))-H arylation of free aliphatic acids. The newly developed MPAI ligand enables the use of 1.0 equiv of aliphatic acids containing an alpha hydrogen for the first time.
Here, we report the development of a class of bifunctional monoprotected amino-imidazoline (MPAI) ligands and their applications in Pd-catalyzed C(sp(3))-H arylation of free aliphatic acids. The newly developed MPAI ligand allows the use of 1.0 equiv of aliphatic acids containing an alpha hydrogen for the first time.
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