期刊
ORGANIC LETTERS
卷 24, 期 39, 页码 7178-7182出版社
AMER CHEMICAL SOC
DOI: 10.1021/acs.orglett.2c02900
关键词
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资金
- National Natural Science Foundation of China [22078268, 21977084]
- Key project of Innovation Research [SWU-XDZD22007]
This paper describes a direct access to benzylic amines from imines and electron-deficient (hetero) arenes via electrochemical radical-radical cross-coupling. The reaction shows a wide range of substrates, excellent functional group tolerance, metal-free conditions, and high atom economy. The insensitivity to air and moisture makes this synthetic strategy more efficient for the construction of various benzylic amine derivatives.
In this paper, a direct access to benzylic amines from imines and electron-deficient (hetero) arenes via electrochemical radical-radical cross-coupling is described. The reaction has the characteristics of the wide range of substrates, excellent functional group tolerance, metal-free and highly atom-economical. The insensitivity to air and moisture makes this synthetic strategy more efficient for the construction of various benzylic amine derivatives.
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