4.8 Article

Substantial contribution of iodine to Arctic ozone destruction

期刊

NATURE GEOSCIENCE
卷 15, 期 10, 页码 770-+

出版社

NATURE PORTFOLIO
DOI: 10.1038/s41561-022-01018-w

关键词

-

资金

  1. European Research Council Executive Agency under the European Union's Horizon 2020 Research and Innovation Program [ERC-2016-COG 726349 CLIMAHAL, ERC-2016-STG 714621 GASPARCON]
  2. European Commission via the EMME-CARE project
  3. Consejo Superior de Investigaciones Cientificas of Spain
  4. European Union's Horizon 2020 Research and Innovation Programme [856612]
  5. Academy of Finland [334514]
  6. Swiss National Science Foundation [200021_188478]
  7. Swiss Polar Institute
  8. U.S. National Science Foundation [1914781, 1807163]
  9. Ministry of Earth Sciences, Government of India
  10. Ferring Pharmaceuticals
  11. Polarstern expedition [AWI-PS122_00]
  12. European ERA-PLANET project iGOSP [689443]
  13. European ERA-PLANET project iCUPE [689443]
  14. FORMAS
  15. Swedish Polar Research Secretariat
  16. Deutsche Forschungsgemeinschaft within the Transregional Collaborative Research Center 'ArctiC Amplification: Climate Relevant Atmospheric and SurfaCe Processes, and Feedback Mechanisms (AC)3' [268020496 - TRR 172]
  17. Academy of Finland (AKA) [334514, 334514] Funding Source: Academy of Finland (AKA)

向作者/读者索取更多资源

The study found that iodine chemistry plays a more important role than bromine chemistry in tropospheric ozone losses in the Arctic. Chemical reactions between iodine and ozone were identified as the second highest contributor to ozone loss over the study period.
Unlike bromine, the effect of iodine chemistry on the Arctic surface ozone budget is poorly constrained. We present ship-based measurements of halogen oxides in the high Arctic boundary layer from the sunlit period of March to October 2020 and show that iodine enhances springtime tropospheric ozone depletion. We find that chemical reactions between iodine and ozone are the second highest contributor to ozone loss over the study period, after ozone photolysis-initiated loss and ahead of bromine. Iodine chemistry plays a more important role than bromine chemistry in tropospheric ozone losses in the Arctic, according to ship-based observations of halogen oxides from March to October 2020.

作者

我是这篇论文的作者
点击您的名字以认领此论文并将其添加到您的个人资料中。

评论

主要评分

4.8
评分不足

次要评分

新颖性
-
重要性
-
科学严谨性
-
评价这篇论文

推荐

暂无数据
暂无数据