期刊
MATERIALS TODAY
卷 59, 期 -, 页码 182-199出版社
ELSEVIER SCI LTD
DOI: 10.1016/j.mattod.2022.08.012
关键词
Electrochemical CO reduction; Multi -carbon products; Catalysts; Mechanism
资金
- National Natural Science Foundation of China [21775067, 22074062, 22176086, 22025208]
- Shandong Provincial Natural Science Foundation [ZR2020ZD37]
- Natural Science Foundation of Jiangsu Province [BK20210189]
- State Key Laboratory of Pollution Control and Resource Reuse [PCRR-ZZ-202106]
- China Postdoctoral Science Foundation [2022M711553]
- Research Fund for Jiangsu Distinguished Professor
This review summarizes the recent research progress in the development of ECOR, including advanced ECOR catalysts and reaction mechanisms. The challenges and prospects in this field are discussed, providing meaningful guidance for grasping ECOR and designing catalysts with enhanced C2+ product selectivity.
The increasing CO2 emissions and accompanying climate challenges have boosted the exploration of candidate pathways for storing and utilizing renewable carbon resources. Electrochemical CO2 reduction (ECO2R) has been proven as a promising technology for artificial carbon fixation. Nevertheless, the unsatisfactory multi-carbon (C2+) product selectivity hinders its widespread use. Recently, the indirect route via electrochemical CO reduction (ECOR) to C2+ products has become a potential alternative through the combination with ECO2R. In this review, we briefly summarize the most recent and instructive research in the ECOR development process from advanced ECOR catalysts and reaction mechanisms. Furthermore, the challenges and outlooks based on current understanding in this field are expounded. These insights and perspectives offer meaningful guidance for grasping ECOR and designing relevant catalysts with enhanced C2+ product selectivity.
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