期刊
JOURNAL OF THE EUROPEAN CERAMIC SOCIETY
卷 42, 期 13, 页码 5399-5409出版社
ELSEVIER SCI LTD
DOI: 10.1016/j.jeurceramsoc.2022.06.020
关键词
Porous ceramics; Permeability; Precursors; SiC; Carbon fibers
资金
- National Natural Science Foundation of China [51 302 237]
- Science and Technology Program of Fujian Province [2016H6021]
- XMU Undergraduate Innovation and Entrepreneurship Training Programs [S202010384720, S202010384722, 2021X1094]
This study proposes an ingenious method to prepare lightweight porous ceramics with excellent permeability and satisfactory mechanical properties. The introduction of carbon fibers and SiC(rGO)(p) with a honeycomb cellular net-like structure effectively reduces density and improves porosity. The self-supporting porous skeleton, high open porosity, and uniform pore distribution contribute to the brilliant permeability of the ceramics.
Making lightweight porous ceramics with excellent permeability applied for transpiration cooling is still challenging. Herein, an ingenious fabrication method is proposed to successfully prepare C-f/SiC(rGO)(px)/SiC porous ceramics possessing low density, high permeability and satisfactory mechanical properties. The introduction of carbon fibers for constructing channels and SiC(rGO)(p) with three-dimensional (3D) honeycomb cellular net-like structure, could effectively decrease density and improve porosity. Meanwhile, self-supporting porous skeleton, high open porosity and uniform pores distribution contribute to brilliant permeability of the products. Good interfacial compatibility among SiC(rGO)(p), carbon fibers and beta-SiC/SiOxCy/C(free )matrix, as well as toughening effects of carbon fibers are beneficial for enhancing fracture toughness and compressive strength. Particularly, C-f/SiC(rGO)(p0.6)/SiC porous ceramics exhibit low density (1.12 g.cm(-3)), low linear shrinkage (3.22%), especially high permeability (1.36 x10(-7) mm(2)), satisfactory fracture toughness (1.77 MPa.m(1/2)), excellent hardness (3.88 GPa) and compressive strength (6.41 MPa), focusing on potential applications as coolant medium in transpiration cooling.
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