4.4 Article

Environmental recovery from 137Cs contamination in Japanese coastal waters shown by comparison of temporal distributions with European seas

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ELSEVIER SCI LTD
DOI: 10.1016/j.jenvrad.2022.106961

关键词

Effective half life; Chernobyl Nuclear Power Plant accident; Fukushima Dai-ichi Nuclear Power Plant accident; Riverine137Cs input

资金

  1. Japan Society for the Promotion of Science
  2. [21H03574]

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This study compared the spatial and temporal distributions of 137Cs in the European Baltic Sea and the North and Norwegian Seas after the Chernobyl accident, and in Japanese coastal regions after the Fukushima accident. The results showed that the decrease in 137Cs concentrations largely depended on local geography, and the dilution-diffusion effect of seawater was more significant in Japanese coastal waters.
We compared the spatiotemporal distributions of 137Cs in the European Baltic Sea (semi-enclosed) and the North and Norwegian Seas (open to the ocean) after the Chernobyl Nuclear Power Plant (CHNPP) accident, with those in Japanese coastal regions, including the waters off Miyagi, Fukushima, and Ibaraki prefectures, open to the western North Pacific, after the Fukushima Nuclear Power Plant accident. The effective half-lives 1-9 years after each accident were shortest (1.6-4.7 y) in Japanese coastal waters, 4.9 y in the North Sea, and 14.4 y in the Baltic Sea, suggesting that decreases in 137Cs concentrations are largely dependent on the local geography, and that the dilution-diffusion effect of seawater was greater in the Japanese coastal waters. The effective half-lives of 137Cs in the surface waters of European seas, based on 30 years of data after the CNPP accident, became longer, ranging from 8.4 to 11.9 y. This may be due to the influence of rivers, and a delay in the decrease in 137Cs levels caused by the small difference in radioactivity concentrations between the seas and diluting waters. These results could contribute to the prediction of contamination levels in Japanese coastal waters in the future.

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