4.7 Article

Lightweight ceramsite made of recycled waste coal gangue & municipal sludge: Particular heavy metals, physical performance and human health

期刊

JOURNAL OF CLEANER PRODUCTION
卷 376, 期 -, 页码 -

出版社

ELSEVIER SCI LTD
DOI: 10.1016/j.jclepro.2022.134309

关键词

Moreira; Human health; Coal gangue; Municipal sludge; Ceramics; Heavy metals

资金

  1. Science and technology research project of Chongqing Municipal Education Commission [KJQN202100723]
  2. Opening Project of Key Laboratory of Solid Waste Treatment and Resource Recycle, Ministry of Education [20kfgk03]
  3. Opening Project of Key Laboratory of Urban Pollutant Conversion, Chinese Academy of Sciences [KLUPC-KF-2020-2]
  4. Key Laboratory of Advanced Civil Engineering Materials (Tongji University) , Ministry of Education [202103]
  5. Western Scholar of Chinese Academy of Sciences Category A [E2296201]
  6. Chongqing Natural Science Foundation [cstc2019jcyj-msxmX0651]
  7. Chongqing Science and Technology Commission [cstc2017jcyjAX0157]

向作者/读者索取更多资源

This study systematically investigated the physical and chemical properties of coal gangue and municipal sludge, assessed the risks they pose to the environment and human health, and explored the feasibility of using them for ceramsite preparation. The experimental results showed that under certain conditions, the ceramsite made from coal gangue and municipal sludge can meet the relevant standards and is environmentally safe.
Large amounts of coal gangue and municipal sludge are generated from coal mining and municipal sewage. Some scholars have studied their use in ceramics, concrete, land reclamation and so on. However, in current study, heavy metals in coal gangue and municipal sludge in utilization have not been safely controlled, and there are potential risks to the ecological environment and human health. Therefore, this study systematically investigated the basic physical and chemical properties of coal gangue and municipal sludge samples, the ecological envi-ronment safety risk of heavy metals and other harmful substances (soluble phosphorus and fluorine). The results showed that the main compositions of coal gangue and municipal sludge samples were cristobalite, hematite and anorthite, which can be used as raw material for ceramsite preparation. The characteristic heavy metals in coal gangue and municipal sludge were As, Cd, Cu, Ni and Zn, which had certain environmental risks. When the optimum proportion of coal gangue: sludge = 70: 30, adding clay and blowing agent as auxiliary materials to make ceramsite, its properties, including bulk density, cylinder pressure strength and other physical properties, meet the Chinese standard light aggregate and its test method (GB/T 17431). The heavy metal environment and human health assessment model of the product was constructed, in which the risk assessment results are, that the content of characteristic heavy metals in ceramsite was significantly reduced, and this content con-formed to the requirements of heavy metals in the Chinese standard technical specification of cement kiln cooperative disposal of solid waste (GB/T 30760), riskless to the human body and external environment. The compressive strength of the two kinds of ceramsite concrete can reach LC35, and the density grade was 1400-1650 N/m3, which meets the requirements of Chinese standard technical specification for lightweight aggregate concrete (JGJ 51). All the properties of this product meet the corresponding standards and there was no risk to the external environment, to provide theoretical guidance for the harmless and resource utilization of urban sludge and coal gangue.

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