期刊
INTERNATIONAL JOURNAL OF HYDROGEN ENERGY
卷 47, 期 89, 页码 38055-38074出版社
PERGAMON-ELSEVIER SCIENCE LTD
DOI: 10.1016/j.ijhydene.2022.08.290
关键词
Direct numerical simulation; Ammon-hydrogen-air mixing layers; Auto-ignition; High turbulence; Elevated pressure
资金
- UK Engineering and Physical Sciences Research Council under the project UK Consortium on Mesoscale Engineering Sciences (UKCOMES) [EP/R029598/1]
This study investigated the auto-ignition characteristics of ammonia-air and ammonia-hydrogen-air mixing layers using numerical simulations. The results showed that elevated pressure and hydrogen addition accelerated the auto-ignition process, and the heat release rate had two distinct peaks corresponding to different stages of the process. Turbulence had an impact on both stages for pure ammonia-air mixing layers, while it only affected the thermal runaway stage for ammonia-hydrogen-air mixing layers.
This study investigated auto-ignition characteristics of ammonia-air and ammoniahydrogen-air laminar and turbulent mixing layers by means of direct numerical simulations (DNS) under elevated pressure conditions. The results show that elevated pressure and hydrogen addition accelerate the auto-ignition process, reducing the auto-ignition delay time. Analysis of the heat release rate revealed that the first peak of the heat release rate corresponds to the increment of appearance in temperature (induction stage) and the second peak of the heat release rate corresponds to the steady maximum temperature regime (thermal runaway stage). The results found that both induction and thermal runaway stages are affected by turbulence for pure ammonia-air mixing layers, while only the thermal runaway stage is affected by turbulence for ammonia-hydrogen-air mixing layers. The auto-ignition occurs along the most reactive mixture fraction with lower scalar dissipation rate, being further reduced by elevated pressure and hydrogen addition. Three radicals (NH2, OH, HNO) distinguish the entire auto-ignition process very well for all cases. Crown Copyright (C) 2022 Published by Elsevier Ltd on behalf of Hydrogen Energy Publications LLC.
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