☆ 4.8 Review

Regeneration strategies for metal-organic frameworks post acidic gas capture

COORDINATION CHEMISTRY REVIEWS (2022)

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Review Chemistry, Multidisciplinary

Transition metal-based metal-organic frameworks for environmental applications: a review

Yeisy C. Lopez et al.

Summary: Rapid industrialization is deteriorating air and water quality, leading to the need for efficient and affordable remediation strategies. Metal-organic frameworks (MOFs) are emerging materials for environmental remediation applications, with unique properties for the removal and conversion of pollutants. Transition metal frameworks have shown promise in capturing and converting gaseous pollutants, while also being studied for the removal of chemical warfare agents.

ENVIRONMENTAL CHEMISTRY LETTERS (2021)

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Review Chemistry, Physical

Adsorptive removal of different pollutants using metal-organic framework adsorbents

Asiata Omotayo Ibrahim et al.

Summary: This review discusses the applications of metal-organic frameworks (MOFs) as novel carbonaceous nanomaterials for removing pollutants from various environments, highlighting promising MOF adsorbents and emphasizing the importance of their reusability as well as addressing challenges and prospects.

JOURNAL OF MOLECULAR LIQUIDS (2021)

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Article Engineering, Environmental

Fabrication of Cu(BDC)0.5(BDC-NH2)0.5 metal-organic framework for superior H2S removal at room temperature

Nishesh Kumar Gupta et al.

Summary: A mixed ligand Cu-based MOF was synthesized and found to exhibit high adsorption capacity for H2S gas, with significantly improved performance after regeneration. The adsorption mechanism involved breaking Cu-carboxylate bonds and formation of CuS nanoparticles and sulfates, leading to enhanced adsorption capacity of the regenerated sample.

CHEMICAL ENGINEERING JOURNAL (2021)

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Article Energy & Fuels

Adsorption of Carbon Dioxide, Water Vapor, Nitrogen, and Sulfur Dioxide on Activated Carbon for Capture from Flue Gases: Competitive Adsorption and Selectivity Aspects

Jon G. Bell et al.

Summary: This study investigates the importance of adsorbing CO2 emissions and removing acid gases, as well as analyzing the adsorption characteristics and competitive adsorption effects of Filtrasorb 400 activated carbon on its main components. The results show that the enthalpy of adsorption decreases with increasing surface excess, and the adsorption kinetics of CO2 and N2 are too fast to be accurately measured.

ENERGY & FUELS (2021)

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Review Chemistry, Multidisciplinary

Hydrogen sulfide removal technology: A focused review on adsorption and catalytic oxidation

Jae Hwan Yang

Summary: The principal technologies for H2S removal, specifically adsorption and catalytic oxidation, are considered promising for desulfurization. Nanoporous materials are extensively used as sorbents due to their porous characteristics suitable for efficient diffusion and capture of H2S. The modification of these materials with functional groups or various metal oxides can enhance H2S adsorption performance.

KOREAN JOURNAL OF CHEMICAL ENGINEERING (2021)

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Article Chemistry, Inorganic & Nuclear

A Series of new Urea-MOFs Obtained via Post-synthetic Modification of NH2-MIL-101(Cr): SO2, CO2 and H2O Sorption

Niels Tannert et al.

Summary: By post-synthetically converting the amino group in MOF NH2-MIL-101(Cr) into urea groups, four novel urea-MOFs were derived. Among them, the partially p-toluenesulfonyl-urea-modified MOF exhibited exceptional SO2 adsorption capacity due to favorable dipole interactions between SO2 and the sulfonyl group.

ZEITSCHRIFT FUR ANORGANISCHE UND ALLGEMEINE CHEMIE (2021)

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Article Nanoscience & Nanotechnology

Zirconium and Aluminum MOFs for Low-Pressure SO2 Adsorption and Potential Separation: Elucidating the Effect of Small Pores and NH2 Groups

Philipp Brandt et al.

Summary: Research on Zr- and Al-based metal-organic frameworks (MOFs) for SO2 adsorption showed that frameworks with pore sizes in the range of 4-8 angstroms exhibit optimal sorption capabilities at low pressures. MOFs with NH2 functional groups tend to have enhanced affinity for SO2. Stability tests and density functional theory (DFT) simulations provided insights into the adsorption mechanisms and binding energies of different MOFs towards SO2.

ACS APPLIED MATERIALS & INTERFACES (2021)

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Article Nanoscience & Nanotechnology

SO2 Capture by Two Aluminum-Based MOFs: Rigid-like MIL-53(Al)-TDC versus Breathing MIL-53(Al)-BDC

Alfredo Lopez-Olvera et al.

Summary: Metal-organic frameworks MIL-53(Al)-TDC and MIL-53(Al)-BDC were found to exhibit different characteristics in the SO2 adsorption process, both serving as exceptional candidates for SO2 capture with good performance and chemical stability. These two materials also have potential interest in SO2 sensing and storage/transportation applications.

ACS APPLIED MATERIALS & INTERFACES (2021)

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Article Environmental Sciences

Fabrication of Zn-MOF/ZnO nanocomposites for room temperature H2S removal: Adsorption, regeneration, and mechanism

Nishesh Kumar Gupta et al.

Summary: Zn-MOF/ZnO nanocomposites with different organic linkers were successfully prepared and showed excellent H2S adsorption performance. Regeneration using methanol and UV irradiation significantly improved the regeneration rate of the adsorbents. Spectroscopic and XPS analysis confirmed the chemisorption mechanism of H2S on Zn-MOF/ZnO.

CHEMOSPHERE (2021)

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Review Biotechnology & Applied Microbiology

Recent advances in microbial capture of hydrogen sulfide from sour gas via sulfur-oxidizing bacteria

Zheng Chen et al.

Summary: Biological desulfurization offers environmental advantages compared to conventional physicochemical methods, but still faces limitations such as low biomass of sulfur-oxidizing bacteria and process solution acidification, which require enhancement through different research perspectives.

ENGINEERING IN LIFE SCIENCES (2021)

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Article Environmental Sciences

Proof of concept for CUK family metal-organic frameworks as environmentally-friendly adsorbents for benzene vapor

Bhaskar Anand et al.

Summary: The study synthesized three M-CUK analogs under similar conditions to evaluate their adsorption performance on benzene vapor, showing that Co-CUK-1 with cobalt metal centers exhibited the best adsorption performance under 0.05 Pa benzene vapor among the analogs.

ENVIRONMENTAL POLLUTION (2021)

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Article Chemistry, Multidisciplinary

Deep Desulfurization with Record SO2 Adsorption on the Metal-Organic Frameworks

Fuqiang Chen et al.

Summary: This study reported a family of MOFs with abundant hydrogen bond donors that showed high selectivity for capturing sulfur dioxide in flue gas desulfurization and natural gas purification, along with excellent cycling stability. Multiple hydrogen bonding interactions ensured a firm grasp of SO2 molecules within the framework, leading to high uptake and density. The MOFs exhibited ultrahigh adsorption uptake and selectivity, as well as robust cycling stability even after multiple cycles.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2021)

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Article Chemistry, Multidisciplinary

From MOF-199 Microrods to CuO Nanoparticles for Room-Temperature Desulfurization: Regeneration and Repurposing Spent Adsorbents as Sustainable Approaches

Nishesh Kumar Gupta et al.

Summary: The study investigates the thermal transformation of MOF199 microrods to CuO nanoparticles, showing excellent performance in gas adsorption, regeneration efficiency, and photocatalytic degradation. MOF-199 demonstrates promising potential for applications in air and water decontamination, with sustainable approaches reported for future use.

ACS OMEGA (2021)

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Article Chemistry, Multidisciplinary

Cucurbit[6]uril@MIL-101-Cl: loading polar porous cages in mesoporous stable host for enhanced SO2 adsorption at low pressures

Yangyang Sun et al.

Summary: The robust cucurbituril-MOF composite CB6@MIL-101-Cl was synthesized by a wet impregnation method and a concomitant OH-to-Cl ligand exchange, exhibiting excellent adsorption performance for SO2 at low pressure and strong recyclability.

NANOSCALE (2021)

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Article Chemistry, Multidisciplinary

Capture of toxic gases in MOFs: SO2, H2S, NH3 and NOx

Eva Martinez-Ahumada et al.

Summary: MOFs have potential for capturing toxic gases, but their vulnerability to highly corrosive gases is a main drawback, although some examples have shown high chemical stability to certain gases. Understanding the role of different chemical functionalities within the pores of MOFs is crucial for achieving superior captures of toxic gases.

CHEMICAL SCIENCE (2021)

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Article Chemistry, Physical

Identification of the preferential CO and SO2 adsorption sites within NOTT-401

Marcos Rivera-Almazo et al.

Summary: NOTT-401 has been identified as a highly stable adsorbent for SO2 and CO, with excellent cyclability and straightforward regeneration at room temperature. The study sheds light on the role of thiophene and hydroxo functionality in the binding of SO2 or CO within a MOF material.

PHYSICAL CHEMISTRY CHEMICAL PHYSICS (2021)

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Article Nanoscience & Nanotechnology

Defectous UiO-66 MOF Nanocomposites as Reactive Media of Superior Protection against Toxic Vapors

Dimitrios A. Giannakoudakis et al.

ACS APPLIED MATERIALS & INTERFACES (2020)

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Article Nanoscience & Nanotechnology

Metal-Organic Frameworks for the Adsorptive Removal of Gaseous Aliphatic Ketones

Kumar Vikrant et al.

ACS APPLIED MATERIALS & INTERFACES (2020)

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Article Engineering, Chemical

Efficient SO2 Removal Using a Microporous Metal-Organic Framework with Molecular Sieving Effect

Yan Zhang et al.

INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH (2020)

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Article Green & Sustainable Science & Technology

Chemisorption of hydrogen sulfide by metal-organic frameworks and covalent-organic polymers based on experimental/theoretical evaluation

Min-Hee Lee et al.

JOURNAL OF CLEANER PRODUCTION (2020)

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Review Chemistry, Physical

Hydrogen sulfide conversion: How to capture hydrogen and sulfur byphotocatalysis

Meng Dan et al.

JOURNAL OF PHOTOCHEMISTRY AND PHOTOBIOLOGY C-PHOTOCHEMISTRY REVIEWS (2020)

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Review Chemistry, Inorganic & Nuclear

MOF Materials for the Capture of Highly Toxic H2S and SO2

Eva Martinez-Ahumada et al.

ORGANOMETALLICS (2020)

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Article Nanoscience & Nanotechnology

Partially Reversible H2S Adsorption by MFM-300(Sc): Formation of Polysulfides

J. Gabriel Flores et al.

ACS APPLIED MATERIALS & INTERFACES (2020)

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Review Chemistry, Multidisciplinary

Metal-Organic Frameworks against Toxic Chemicals

Timur Islamoglu et al.

CHEMICAL REVIEWS (2020)

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Review Materials Science, Multidisciplinary

Water-based routes for synthesis of metal-organic frameworks: A review

Chongxiong Duan et al.

SCIENCE CHINA-MATERIALS (2020)

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Article Chemistry, Multidisciplinary

Template-Free, Solid-State Synthesis of Hierarchically Macroporous S-Doped TiO2 Nano-Photocatalysts for Efficient Water Remediation

Vishnu V. Pillai et al.

ACS OMEGA (2020)

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Article Chemistry, Multidisciplinary

Transition-Metal-Containing Porphyrin Metal-Organic Frameworks as π-Backbonding Adsorbents for NO2 Removal

Shanshan Shang et al.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2020)

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Article Nanoscience & Nanotechnology

Functionalized NU-1000 with an Iridium Organometallic Fragment: SO2 Capture Enhancement

Saidulu Gorla et al.

ACS APPLIED MATERIALS & INTERFACES (2020)

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Article Chemistry, Multidisciplinary

Adsorption of Nitrogen Dioxide in a Redox-Active Vanadium Metal-Organic Framework Material

Xue Han et al.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2020)

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Review Chemistry, Inorganic & Nuclear

Green synthesis of metal-organic frameworks: A state-of-the-art review of potential environmental and medical applications

Sandeep Kumar et al.

COORDINATION CHEMISTRY REVIEWS (2020)

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Article Chemistry, Multidisciplinary

A Robust and Biocompatible Bismuth Ellagate MOF Synthesized Under Green Ambient Conditions

Erik Svensson Grape et al.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2020)

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Review Chemistry, Physical

Hydrogen Sulfide (H2S) Removal via MOFs

Amvrosios G. Georgiadis et al.

MATERIALS (2020)

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Article Green & Sustainable Science & Technology

The potential utility of HKUST-1 for adsorptive removal of benzene vapor from gaseous streams using a denuder versus a packed-bed adsorption system

Bhaskar Anand et al.

JOURNAL OF CLEANER PRODUCTION (2020)

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Article Nanoscience & Nanotechnology

NO2 Removal under Ambient Conditions by Nanoporous Multivariate Zirconium-Based Metal-Organic Framework

Xinbo Wang et al.

ACS APPLIED NANO MATERIALS (2020)

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Article Materials Science, Multidisciplinary

Water-Based Synthesis of a Stable Iron-Based Metal-Organic Framework for Capturing Toxic Gases

Zhijie Chen et al.

ACS MATERIALS LETTERS (2020)

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Review Chemistry, Multidisciplinary

Critical role of water stability in metal-organic frameworks and advanced modification strategies for the extension of their applicability

Botao Liu et al.

ENVIRONMENTAL SCIENCE-NANO (2020)

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Article Chemistry, Inorganic & Nuclear

Reversible and efficient SO2 capture by a chemically stable MOF CAU-10: experiments and simulations

J. Antonio Zarate et al.

DALTON TRANSACTIONS (2020)

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Article Chemistry, Physical

High and reversible SO2 capture by a chemically stable Cr(III)-based MOF

Eva Martinez-Ahumada et al.

JOURNAL OF MATERIALS CHEMISTRY A (2020)

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Upscale synthesis of a binary pillared layered MOF for hydrocarbon gas storage and separation

Mickaele Bonneau et al.

GREEN CHEMISTRY (2020)

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Review Chemistry, Multidisciplinary

Porous metal-organic frameworks as emerging sorbents for clean air

Xue Han et al.

NATURE REVIEWS CHEMISTRY (2019)

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Metal-Organic Frameworks with Potential Application for SO2 Separation and Flue Gas Desulfurization

Philipp Brandt et al.

ACS APPLIED MATERIALS & INTERFACES (2019)

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Article Environmental Sciences

Regeneration, degradation, and toxicity effect of MOFs: Opportunities and challenges

Pawan Kumar et al.

ENVIRONMENTAL RESEARCH (2019)

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Article Thermodynamics

Shaping metal-organic framework (MOF) powder materials for CO2 capture applications-a thermogravimetric study

Izabela Majchrzak-Kuceba et al.

JOURNAL OF THERMAL ANALYSIS AND CALORIMETRY (2019)

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Synthesis and Photocatalytic Properties of CuO-CuS Core-Shell Nanowires

Yuan-Tse Kao et al.

MATERIALS (2019)

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Review Nanoscience & Nanotechnology

Kinetic stability of metal-organic frameworks for corrosive and coordinating gas capture

Adam J. Rieth et al.

NATURE REVIEWS MATERIALS (2019)

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Capture of nitrogen dioxide and conversion to nitric acid in a porous metal-organic framework

Jiangnan Li et al.

NATURE CHEMISTRY (2019)

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Reversible coordinative binding and separation of sulfur dioxide in a robust metal-organic framework with open copper sites

Gemma L. Smith et al.

NATURE MATERIALS (2019)

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Recycling and regeneration of carbonaceous and porous materials through thermal or solvent treatment

Tanushree Dutta et al.

CHEMICAL ENGINEERING JOURNAL (2019)

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Article Chemistry, Physical

High and energy-efficient reversible SO2 uptake by a robust Sc(III)-based MOF

J. Antonio Zarate et al.

JOURNAL OF MATERIALS CHEMISTRY A (2019)

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Review Chemistry, Multidisciplinary

Carbon capture and conversion using metal-organic frameworks and MOF-based materials

Meili Ding et al.

CHEMICAL SOCIETY REVIEWS (2019)

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Phosphonium zwitterions for lighter and chemically-robust MOFs: highly reversible H2S capture and solvent-triggered release

Joseph E. Reynolds et al.

JOURNAL OF MATERIALS CHEMISTRY A (2019)

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Outstanding reversible H2S capture by an Al(III)-based MOF

J. Antonio Zarate et al.

CHEMICAL COMMUNICATIONS (2019)

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Activation strategies of metal-organic frameworks for the sorption of reduced sulfur compounds

Yaxin Deng et al.

CHEMICAL ENGINEERING JOURNAL (2018)

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Article Chemistry, Physical

Reversible adsorption of nitrogen dioxide within a robust porous metal-organic framework

Xue Han et al.

NATURE MATERIALS (2018)

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A post-synthetic approach triggers selective and reversible sulphur dioxide adsorption on a metal-organic framework

Marta Mon et al.

CHEMICAL COMMUNICATIONS (2018)

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Highly reversible sorption of H2S and CO2 by an environmentally friendly Mg-based MOF

Eli Sanchez-Gonzalez et al.

JOURNAL OF MATERIALS CHEMISTRY A (2018)

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Article Chemistry, Multidisciplinary

Exceptional Adsorption and Binding of Sulfur Dioxide in a Robust Zirconium-Based Metal-Organic Framework

Joseph H. Carter et al.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2018)

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Article Chemistry, Physical

Selective H2S/CO2 Separation by Metal-Organic Frameworks Based on Chemical-Physical Adsorption

Jia Liu et al.

JOURNAL OF PHYSICAL CHEMISTRY C (2017)

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Article Multidisciplinary Sciences

Selective sulfur dioxide adsorption on crystal defect sites on an isoreticular metal organic framework series

L. Marleny Rodriguez-Albelo et al.

NATURE COMMUNICATIONS (2017)

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Article Chemistry, Multidisciplinary

Unique structural micro-adjustments in a new benzothiadiazole-derived Zn(II) metal organic framework via simple photochemical decarboxylation

Xiao Han et al.

CHEMICAL COMMUNICATIONS (2017)

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Article Engineering, Environmental

Isoreticular rare earth fcu-MOFs for the selective removal of H2S from CO2 containing gases

Prashant M. Bhatt et al.

CHEMICAL ENGINEERING JOURNAL (2017)

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Article Chemistry, Physical

Interaction of Acid Gases SO2 and NO2 with Coordinatively Unsaturated Metal Organic Frameworks: M-MOF-74 (M = Zn, Mg, Ni, Co)

Kui Tan et al.

CHEMISTRY OF MATERIALS (2017)

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Highly Efficient Air Desulfurization on Self-Assembled Bundles of Copper Hydroxide Nanorods

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ACS Applied Materials & Interfaces (2016)

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Review Nanoscience & Nanotechnology

Metal-Organic Frameworks as a Potential Platform for Selective Treatment of Gaseous Sulfur Compounds

Kowsalya Vellingiri et al.

ACS APPLIED MATERIALS & INTERFACES (2016)

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Article Chemistry, Multidisciplinary

Extraordinary NO2 Removal by the Metal-Organic Framework UiO-66-NH2

Gregory W. Peterson et al.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2016)

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Article Chemistry, Physical

MaLISA - a cooperative method to release adsorbed gases from metal-organic frameworks

Haiqing Li et al.

JOURNAL OF MATERIALS CHEMISTRY A (2016)

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Article Chemistry, Physical

Engineering the surface of a new class of adsorbents: Metal-organic framework/graphite oxide composites

Camille Petit et al.

JOURNAL OF COLLOID AND INTERFACE SCIENCE (2015)

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Article Chemistry, Applied

H2S interaction with HKUST-1 and ZIF-8 MOFs: A multitechnique study

Jayashree Ethiraj et al.

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Metal-Organic Frameworks for Air Purification of Toxic Chemicals

Jared B. DeCoste et al.

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Toxic gas removal - metal-organic frameworks for the capture and degradation of toxic gases and vapours

Elisa Barea et al.

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Methanol absorption characteristics for the removal of H2S (hydrogen sulfide), COS (carbonyl sulfide) and CO2 (carbon dioxide) in a pilot-scale biomass-to-liquid process

Myung Won Seo et al.

ENERGY (2014)

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Article Chemistry, Multidisciplinary

A robust amino-functionalized titanium(IV) based MOF for improved separation of acid gases

Sebastien Vaesen et al.

CHEMICAL COMMUNICATIONS (2013)

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Article Chemistry, Physical

The effect of SO2 on CO2 capture in zeolitic imidazolate frameworks

Lifeng Ding et al.

PHYSICAL CHEMISTRY CHEMICAL PHYSICS (2013)

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Article Chemistry, Multidisciplinary

Adsorption of hydrogen sulphide on Metal-Organic Frameworks

Juan Jose Gutierrez-Sevillano et al.

RSC ADVANCES (2013)

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Article Engineering, Environmental

Influence of the Concentration of CO2 and SO2 on the Absorption of CO2 by a Lithium Orthosilicate-Based Absorbent

R. Pacciani et al.

ENVIRONMENTAL SCIENCE & TECHNOLOGY (2011)

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Article Nanoscience & Nanotechnology

Reactive Adsorption of NO2 on Copper-Based Metal-Organic Framework and Graphite Oxide/Metal-Organic Framework Composites

Benoit Levasseur et al.

ACS APPLIED MATERIALS & INTERFACES (2010)

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Article Medicine, General & Internal

Hydrogen sulfide exposure in an adult male

Bassam Doujaiji et al.

ANNALS OF SAUDI MEDICINE (2010)

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Article Chemistry, Physical

Hydrogen Sulfide Adsorption on MOFs and MOF/Graphite Oxide Composites

Camille Petit et al.

CHEMPHYSCHEM (2010)

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Review Public, Environmental & Occupational Health

Effects of nitrogen dioxide on human health: Systematic review of experimental and epidemiological studies conducted between 2002 and 2006

Ute Latza et al.

INTERNATIONAL JOURNAL OF HYGIENE AND ENVIRONMENTAL HEALTH (2009)

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Article Medicine, General & Internal

Outdoor air pollution: Nitrogen dioxide, sulfur dioxide, and carbon monoxide health effects

Tze-Ming Chen et al.

AMERICAN JOURNAL OF THE MEDICAL SCIENCES (2007)

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