4.7 Article

Analysis on ignition kernel formation in a quiescent mixture: Different characteristic time scales and critical heating powers

期刊

COMBUSTION AND FLAME
卷 245, 期 -, 页码 -

出版社

ELSEVIER SCIENCE INC
DOI: 10.1016/j.combustflame.2022.112336

关键词

Ignition; Thermal runaway; Reaction front; Characteristic time scale; Heating power density

资金

  1. National Natural Science Founda-tion of China [52176096, 520 060 01]

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This study provides a theoretical analysis of flame ignition, focusing on the formation of ignition kernel induced by external heating. The study reveals the three stages and characteristic time scales of ignition kernel formation, and explores the impact of external heating power density on the delay times for reaction front generation and propagation.
Flame ignition is one of the most fundamental and ubiquitous problems in the field of combustion. Flame ignition in a quiescent flammable mixture consists of two phases: ignition kernel formation and subse-quent transition to self-sustained expanding spherical flame. Most of previous studies focused on the second phase while little attention was paid to the first phase. In this work, theoretical analysis is con-ducted for ignition kernel formation induced by external heating within finite domain and finite duration. The ignition kernel formation consists of three stages, i.e., onset of thermal runaway, generation of reac-tion front at the center, and arrival of reaction front at the edge of heating domain. The characteristic time scales for these three stages are evaluated. Good agreement between theoretical analysis and tran-sient simulation has been obtained. The delay times for the generation of reaction front at the center and its propagation to the edge of heating domain decrease rapidly with the external heating power density; and the delay time for thermal runaway is the primary component in the total time for ignition ker-nel formation. Moreover, a minimum power density for external heating below which thermal runaway cannot occur is determined. Since chemical reaction is self-sustained by releasing heat, two additional threshold values of external heating power densities are determined respectively corresponding to spon-taneous generation of reaction front at the center and its subsequent propagation across the edge of heating domain. This study provides useful insights into ignition kernel formation occurring in premixed flame ignition.(c) 2022 The Combustion Institute. Published by Elsevier Inc. All rights reserved.

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