期刊
CHEMISTRY-A EUROPEAN JOURNAL
卷 28, 期 66, 页码 -出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/chem.202202407
关键词
borate buffer; copper; electrocatalysis; trinuclear; water oxidation
The borate buffer plays both structural and functional roles in a low-cost tri-copper electrocatalyst, facilitating catalytic activity and O-O bond formation.
Borate buffer was found to have both structural and functional roles within a low-cost tri-copper electrocatalyst for homogeneous water oxidation that exhibits a high turnover frequency of 310 s(-1). The borate buffer was shown to facilitate the catalytic activity by both bridging the three Cu ions and participating in O-O bond formation. Phosphate and acetate buffers did not show such roles, making borate a unique player in this catalytic system.
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