Structural Fine-Tuning and In-situ Generation of P, O Vacancies in Hollow Co-Ferrocene-MOFs Derived Phosphides for Efficient Water Oxidation

Review Chemistry, Physical

Realizing electrochemical transformation of a metal-organic framework precatalyst into a metal hydroxide-oxy(hydroxide) active catalyst during alkaline water oxidation

Baghendra Singh et al.

Summary: MOF-derived ultrathin metal hydroxide-(oxy)hydroxide nanosheets produced through electrochemical transformation have been explored for electrochemical water oxidation, showing excellent activity and stability.

JOURNAL OF MATERIALS CHEMISTRY A (2022)

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Article Chemistry, Physical

Deeply self-reconstructing CoFe(H3O)(PO4)2 to low-crystalline Fe0.5Co0.5OOH with Fe3+-O-Fe3+ motifs for oxygen evolution reaction

Shenghua Ye et al.

Summary: In this study, phosphate FeCo(H3O)(PO4)(2) nanosheet arrays were synthesized using an electrochemical strategy. It was found that FeCo(H3O)(PO4)(2) nanosheet arrays could undergo significant self-reconstruction under the conditions of oxygen evolution reaction (OER), resulting in the formation of Fe0.5Co0.5OOH nanosheet arrays with low crystallinity. The high Fe content in Fe0.5Co0.5OOH nanosheet arrays promoted the formation of active Fe3+-O-Fe3+ motifs and enhanced the reaction order on the hydroxyl ion, leading to outstanding OER catalytic performances.

APPLIED CATALYSIS B-ENVIRONMENTAL (2022)

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Article Chemistry, Multidisciplinary

Alkaline oxygen evolution: exploring synergy between fcc and hcp cobalt nanoparticles entrapped in N-doped graphene

Ajit Kumar Singh et al.

Summary: The Mott-Schottky catalyst Co@NC demonstrates excellent oxygen evolution activity and long-term stability by entrapping cobalt nanoparticles inside the N-doped graphene shell. The synergy between hcp and fcc cobalt, along with the optimization from the NC shell, plays a major role in improving the catalytic activity.

MATERIALS TODAY CHEMISTRY (2022)

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Article Engineering, Environmental

Electronic modulation of CoP nanoarrays by Cr-doping for efficient overall water splitting

Wanfeng Li et al.

Summary: The 3D self-supported Cr-doped CoP nanoarrays exhibit outstanding catalytic activity for both hydrogen evolution and oxygen evolution reactions, with low overpotentials in acidic, neutral, and alkaline media. The activation process of active sites in transition metal phosphides is confirmed through X-ray photoelectron spectroscopy and theoretical calculations.

CHEMICAL ENGINEERING JOURNAL (2021)

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Review Chemistry, Inorganic & Nuclear

Modulating electronic structure of metal-organic framework derived catalysts for electrochemical water oxidation

Baghendra Singh et al.

Summary: The focus of the research is on the electronic structure engineering of MOF-derived catalysts to improve water oxidation activity. Strategies for tuning electronic properties through interfacial modulation, surface overlayer, Fermi level manipulation, and heterostructure formation have been addressed to enhance the catalytic activity and stability of MOF-derived catalysts.

COORDINATION CHEMISTRY REVIEWS (2021)

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Article Chemistry, Multidisciplinary

Ferrocene-Based Metal-Organic Framework Nanosheets as a Robust Oxygen Evolution Catalyst

Jing Liang et al.

Summary: The study reports the synthesis of two-dimensional metal-organic frameworks on nickel foam, which exhibit superior oxygen evolution reaction performance under alkaline conditions due to the ferrocene units acting as efficient electron transfer intermediates.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2021)

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Review Chemistry, Multidisciplinary

Opportunities and Challenges in Precise Synthesis of Transition Metal Single-Atom Supported by 2D Materials as Catalysts toward Oxygen Reduction Reaction

Wen-Jun Niu et al.

Summary: This review highlights the recent advances in transition metal single-atom catalysts supported by 2D materials for electrocatalytic oxygen reduction reaction (ORR). It discusses the advantages of 2D materials as supporting materials, the identification of active sites, possible catalytic mechanisms, and future perspectives in the field. Additionally, it summarizes the future opportunities and challenges of transition metal single-atom catalysts supported by 2D materials based on the current development trend of ORR catalysts.

ADVANCED FUNCTIONAL MATERIALS (2021)

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Article Chemistry, Physical

Synergistically coupling of Fe-doped CoP nanocubes with CoP nanosheet arrays towards enhanced and robust oxygen evolution electrocatalysis

Deli Jiang et al.

Summary: This study demonstrates an interfacial engineering strategy to prepare a CoFeP/CoP/CC heterostructure catalyst with high-performance and stability for OER electrocatalysis. The catalyst shows superior OER performance with low overpotential and excellent stability, providing an effective approach for designing high-performance OER catalysts through interfacial engineering.

JOURNAL OF COLLOID AND INTERFACE SCIENCE (2021)

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Review Nanoscience & Nanotechnology

Design Engineering, Synthesis Protocols, and Energy Applications of MOF-Derived Electrocatalysts

Amr Radwan et al.

Summary: The significant progress of MOFs-derived electrocatalysts in ORR, OER, and HER applications is mainly attributed to their high-porosity structure, large surface area, and abundant active centers.

NANO-MICRO LETTERS (2021)

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Article Chemistry, Physical

Quasi-Two-Dimensional Earth-Abundant Bimetallic Electrocatalysts for Oxygen Evolution Reactions

Yunhe Zhao et al.

Summary: This study successfully synthesized bimetallic Co-Mo-O ultrathin nanosheets with enriched surface catalytic active site ratio, among which nanosheets with 2:1 Co-to-Mo ratio showed significantly enhanced OER catalytic activity. This 2D morphology of bimetallic materials introduces a promising possibility for creating high-performance electrocatalysts.

ACS ENERGY LETTERS (2021)

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Review Chemistry, Multidisciplinary

Decoupled electrochemical water-splitting systems: a review and perspective

Zachary P. Ifkovits et al.

Summary: Decoupled water splitting technology separates the spatial and temporal coupling of electrolysis reactions through the coupling of intermediate redox mediators, offering flexibility, modularity, and coupling to renewable energy sources as advantages. However, considerations of trade-offs and opportunities for future discovery in practical applications are also worth noting.

ENERGY & ENVIRONMENTAL SCIENCE (2021)

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Article Chemistry, Physical

Ultrafine Ir nanoparticles decorated on FeP/FeOOH with abundant interfaces via a facile corrosive approach for alkaline water-splitting

Zongshi Zhao et al.

Summary: By developing a catalyst structure with abundant interfaces of ultrafine Ir nanoparticles coupled with FeP/FeOOH on iron foam, excellent catalytic activities were demonstrated in 1M KOH, with overall water-splitting achieved at only 1.47 V.

JOURNAL OF MATERIALS CHEMISTRY A (2021)

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Article Chemistry, Multidisciplinary

Self-Supported Transition-Metal-Based Electrocatalysts for Hydrogen and Oxygen Evolution

Hongming Sun et al.

ADVANCED MATERIALS (2020)

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Review Chemistry, Multidisciplinary

State of the Art and Prospects in Metal-Organic Framework (MOF)-Based and MOF-Derived Nanocatalysis

Qi Wang et al.

CHEMICAL REVIEWS (2020)

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Article Chemistry, Multidisciplinary

Interfacial Engineering of W2N/WC Heterostructures Derived from Solid-State Synthesis: A Highly Efficient Trifunctional Electrocatalyst for ORR, OER, and HER

Jinxiang Diao et al.

ADVANCED MATERIALS (2020)

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Review Chemistry, Physical

Recent Advances on Water-Splitting Electrocatalysis Mediated by Noble-Metal-Based Nanostructured Materials

Yingjie Li et al.

ADVANCED ENERGY MATERIALS (2020)

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Article Chemistry, Physical

Potential-Dependent Phase Transition and Mo-Enriched Surface Reconstruction of γ-CoOOH in a Heterostructured Co-Mo2C Precatalyst Enable Water Oxidation

Zongkui Kou et al.

ACS CATALYSIS (2020)

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Article Chemistry, Multidisciplinary

Metal-Organic Framework-Derived Co2P Nanoparticle/Multi-Doped Porous Carbon as a Trifunctional Electrocatalyst

Haitao Liu et al.

ADVANCED MATERIALS (2020)

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Article Chemistry, Multidisciplinary

Mechanism of Oxygen Evolution Catalyzed by Cobalt Oxyhydroxide: Cobalt Superoxide Species as a Key Intermediate and Dioxygen Release as a Rate-Determining Step

Aliki Moysiadou et al.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2020)

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Article Nanoscience & Nanotechnology

Arrayed Cobalt Phosphide Electrocatalyst Achieves Low Energy Consumption and Persistent H2Liberation from Anodic Chemical Conversion

Kai Zhang et al.

NANO-MICRO LETTERS (2020)

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Article Chemistry, Multidisciplinary

Electrochemical transformation of Prussian blue analogues into ultrathin layered double hydroxide nanosheets for water splitting

Baghendra Singh et al.

CHEMICAL COMMUNICATIONS (2020)

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Article Chemistry, Physical

Morphology regulation of metal-organic framework-derived nanostructures for efficient oxygen evolution electrocatalysis

Yuwen Li et al.

JOURNAL OF MATERIALS CHEMISTRY A (2020)

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Article Chemistry, Multidisciplinary

Improved chemical water oxidation with Zn in the tetrahedral site of spinel-type ZnCo2O4 nanostructure

B. Chakraborty et al.

MATERIALS TODAY CHEMISTRY (2020)

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Article Chemistry, Inorganic & Nuclear

3D Ni and Co redox-active metal-organic frameworks based on ferrocenyl diphosphinate and 4,4′-bipyridine ligands as efficient electrocatalysts for the hydrogen evolution reaction

Vera Khrizanforova et al.

DALTON TRANSACTIONS (2020)

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Review Chemistry, Multidisciplinary

A review on fundamentals for designing oxygen evolution electrocatalysts

Jiajia Song et al.

CHEMICAL SOCIETY REVIEWS (2020)

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Article Chemistry, Multidisciplinary

Shifting Oxygen Charge Towards Octahedral Metal: A Way to Promote Water Oxidation on Cobalt Spinel Oxides

Shengnan Sun et al.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2019)

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Editorial Material Energy & Fuels

Considerations for the scaling-up of water splitting catalysts

Jakob Kibsgaard et al.

NATURE ENERGY (2019)

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Article Chemistry, Multidisciplinary

Two Birds with One Stone: Metal-Organic Framework Derived Micro-/Nanostructured Ni2P/Ni Hybrids Embedded in Porous Carbon for Electrocatalysis and Energy Storage

Xiaobin Liu et al.

ADVANCED FUNCTIONAL MATERIALS (2019)

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Article Chemistry, Multidisciplinary

Reducing the Barrier Energy of Self-Reconstruction for Anchored Cobalt Nanoparticles as Highly Active Oxygen Evolution Electrocatalyst

Myeongjin Kim et al.

ADVANCED MATERIALS (2019)

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Article Chemistry, Physical

In Situ Growth of Ni2P-Cu3P Bimetallic Phosphide with Bicontinuous Structure on Self-Supported NiCuC Substrate as an Efficient Hydrogen Evolution Reaction Electrocatalyst

Linping Yu et al.

ACS CATALYSIS (2019)

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Article Nanoscience & Nanotechnology

Cobalt/Molybdenum Phosphide and Oxide Heterostructures Encapsulated in N-Doped Carbon Nanocomposite for Overall Water Splitting in Alkaline Media

Lei Yu et al.

ACS APPLIED MATERIALS & INTERFACES (2019)

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Article Chemistry, Multidisciplinary

H/D Isotope Effects Reveal Factors Controlling Catalytic Activity in Co-Based Oxides for Water Oxidation

Chiara Pasquini et al.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2019)

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Article Chemistry, Multidisciplinary

Construction of FeP Hollow Nanoparticles Densely Encapsulated in Carbon Nanosheet Frameworks for Efficient and Durable Electrocatalytic Hydrogen Production

Fei-Xiang Ma et al.

ADVANCED SCIENCE (2019)

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Review Chemistry, Multidisciplinary

Nanoarchitectonics for Transition-Metal-Sulfide-Based Electrocatalysts for Water Splitting

Yanna Guo et al.

ADVANCED MATERIALS (2019)

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Review Chemistry, Multidisciplinary

Support and Interface Effects in Water-Splitting Electrocatalysts

Jian Zhang et al.

ADVANCED MATERIALS (2019)

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Article Chemistry, Multidisciplinary

Intramolecular electronic coupling in porous iron cobalt (oxy)phosphide nanoboxes enhances the electrocatalytic activity for oxygen evolution

Huabin Zhang et al.

ENERGY & ENVIRONMENTAL SCIENCE (2019)

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Article Chemistry, Physical

Mo2C Nanodots Anchored on N-Doped Porous CNT Microspheres as Electrode for Efficient Li-Ion Storage

Bo Yu et al.

SMALL METHODS (2019)

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Review Chemistry, Multidisciplinary

Robust noble metal-based electrocatalysts for oxygen evolution reaction

Qiurong Shi et al.

CHEMICAL SOCIETY REVIEWS (2019)

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Review Chemistry, Multidisciplinary

Metal Organic Framework Derived Materials: Progress and Prospects for the Energy Conversion and Storage

Arindam Indra et al.

ADVANCED MATERIALS (2018)

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Article Chemistry, Multidisciplinary

Colloidal Cobalt Phosphide Nanocrystals as Trifunctional Electrocatalysts for Overall Water Splitting Powered by a Zinc-Air Battery

Hui Li et al.

ADVANCED MATERIALS (2018)

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Article Chemistry, Multidisciplinary

In Situ Grown Epitaxial Heterojunction Exhibits High-Performance Electrocatalytic Water Splitting

Changrong Zhu et al.

ADVANCED MATERIALS (2018)

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Review Chemistry, Multidisciplinary

Transition Metal Oxides as Electrocatalysts for the Oxygen Evolution Reaction in Alkaline Solutions: An Application-Inspired Renaissance

Fang Song et al.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2018)

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Article Chemistry, Physical

P vacancies-enriched 3D hierarchical reduced cobalt phosphide as a precursor template for defect engineering for efficient water oxidation

Xichen Zhou et al.

JOURNAL OF MATERIALS CHEMISTRY A (2018)

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Article Nanoscience & Nanotechnology

Bimetal Prussian Blue as a Continuously Variable Platform for Investigating the Composition-Activity Relationship of Phosphides-Based Electrocatalysts for Water Oxidation

Zhongtao Li et al.

ACS APPLIED MATERIALS & INTERFACES (2018)

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Article Chemistry, Physical

Exploring Indium-Based Ternary Thiospinel as Conceivable High-Potential Air-Cathode for Rechargeable Zn-Air Batteries

Gengtao Fu et al.

ADVANCED ENERGY MATERIALS (2018)

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Article Chemistry, Physical

Bifunctional sulfur-doped cobalt phosphide electrocatalyst outperforms all-noble-metal electrocatalysts in alkaline electrolyzer for overall water splitting

Mohsin Ali Raza Anjum et al.

NANO ENERGY (2018)

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Article Chemistry, Multidisciplinary

Interfacial Electron Transfer of Ni2P-NiP2 Polymorphs Inducing Enhanced Electrochemical Properties

Tong Liu et al.

ADVANCED MATERIALS (2018)

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Article Chemistry, Physical

Unified structural motifs of the catalytically active state of Co(oxyhydr)oxides during the electrochemical oxygen evolution reaction

Arno Bergmann et al.

NATURE CATALYSIS (2018)

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Article Chemistry, Multidisciplinary

MOF-Derived Bifunctional Cu3P Nanoparticles Coated by a N,P-Codoped Carbon Shell for Hydrogen Evolution and Oxygen Reduction

Rui Wang et al.

ADVANCED MATERIALS (2018)

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Article Chemistry, Physical

Uncovering the Nature of Active Species of Nickel Phosphide Catalysts in High-Performance Electrochemical Overall Water Splitting

Prashanth W. Menezes et al.

ACS CATALYSIS (2017)

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Article Chemistry, Physical

Bimetallic Cobalt-Based Phosphide Zeolitic Imidazolate Framework: CoPx Phase-Dependent Electrical Conductivity and Hydrogen Atom Adsorption Energy for Efficient Overall Water Splitting

Junhua Song et al.

ADVANCED ENERGY MATERIALS (2017)

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Hollow Co2P nanoflowers assembled from nanorods for ultralong cycle-life supercapacitors

Ming Cheng et al.

NANOSCALE (2017)

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Janus Co/CoP Nanoparticles as Efficient Mott-Schottky Electrocatalysts for Overall Water Splitting in Wide pH Range

Zhong-Hua Xue et al.

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Article Chemistry, Physical

Activating and Optimizing Activity of CoS2 for Hydrogen Evolution Reaction through the Synergic Effect of N Dopants and S Vacancies

Jingyan Zhang et al.

ACS ENERGY LETTERS (2017)

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Review Chemistry, Multidisciplinary

Defect Chemistry of Nonprecious-Metal Electrocatalysts for Oxygen Reactions

Dafeng Yan et al.

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Ultrathin Iron-Cobalt Oxide Nanosheets with Abundant Oxygen Vacancies for the Oxygen Evolution Reaction

Linzhou Zhuang et al.

ADVANCED MATERIALS (2017)

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Review Chemistry, Multidisciplinary

Electrocatalysis for the oxygen evolution reaction: recent development and future perspectives

Nian-Tzu Suen et al.

CHEMICAL SOCIETY REVIEWS (2017)

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Iron-Doped Nickel Phosphate as Synergistic Electrocatalyst for Water Oxidation

Yibing Li et al.

CHEMISTRY OF MATERIALS (2016)

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Heterogeneous Spin States in Ultrathin Nanosheets Induce Subtle Lattice Distortion To Trigger Efficient Hydrogen Evolution

Youwen Liu et al.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2016)

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Review Multidisciplinary Sciences

Research opportunities to advance solar energy utilization

Nathan S. Lewis

SCIENCE (2016)

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Article Chemistry, Physical

Uncovering the prominent role of metal ions in octahedral versus tetrahedral sites of cobalt-zinc oxide catalysts for efficient oxidation of water

Prashanth W. Menezes et al.

JOURNAL OF MATERIALS CHEMISTRY A (2016)

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Article Multidisciplinary Sciences

Coordination tuning of cobalt phosphates towards efficient water oxidation catalyst

Hyunah Kim et al.

NATURE COMMUNICATIONS (2015)

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Construction of Efficient 3D Gas Evolution Electrocatalyst for Hydrogen Evolution: Porous FeP Nanowire Arrays on Graphene Sheets

Ya Yan et al.

ADVANCED SCIENCE (2015)

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A Cost-Effective 3D Hydrogen Evolution Cathode with High Catalytic Activity: FeP Nanowire Array as the Active Phase

Ping Jiang et al.

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Vacancy Associates Promoting Solar-Driven Photocatalytic Activity of Ultrathin Bismuth Oxychloride Nanosheets

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Opportunities and challenges for a sustainable energy future

Steven Chu et al.

NATURE (2012)

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Direct-Coupling O2 Bond Forming a Pathway in Cobalt Oxide Water Oxidation Catalysts

Lee-Ping Wang et al.

JOURNAL OF PHYSICAL CHEMISTRY LETTERS (2011)

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Review Chemistry, Multidisciplinary

Ferrocene-Terminated Monolayers Covalently Bound to Hydrogen-Terminated Silicon Surfaces. Toward the Development of Charge Storage and Communication Devices

Bruno Fabre

ACCOUNTS OF CHEMICAL RESEARCH (2010)

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Hollow Ferrocenyl Coordination Polymer Microspheres with Micropores in Shells Prepared by Ostwald Ripening

Jia Huo et al.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2010)

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Review Chemistry, Inorganic & Nuclear

Ferrocene-Containing Coordination Polymers: Ligand Design and Assembled Structures

Ryo Horikoshi et al.

EUROPEAN JOURNAL OF INORGANIC CHEMISTRY (2010)

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Tetragonal Zinc Diphosphide and Its Nanocomposite as an Anode for Lithium Secondary Batteries

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CHEMISTRY OF MATERIALS (2008)

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Review Chemistry, Multidisciplinary

Strained metallocenophanes and related organometallic rings containing pi-hydrocarbon ligands and transition-metal centers

David E. Herbert et al.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2007)

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Structural Fine-Tuning and In-situ Generation of P, O Vacancies in Hollow Co-Ferrocene-MOFs Derived Phosphides for Efficient Water Oxidation

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