期刊
JOURNAL OF HAZARDOUS MATERIALS
卷 301, 期 -, 页码 462-470出版社
ELSEVIER SCIENCE BV
DOI: 10.1016/j.jhazmat.2015.09.027
关键词
Polyoxometalates; Membrane; Adsorption; Catalytic degradation; Dye removal
资金
- Singapore Membrane Technology Centre (SMTC), Nanyang Technological University
- NTU AcRF grant [RG76/12]
- Singapore Economic Development Board
Membrane technique is a promising way for the removal of dyes from wastewater. A unique approach combining both the adsorptive and the catalytic membrane processes was proposed on the basis of a new functionalized membrane. The membrane integrating both the adsorptive and catalytic activities was developed by introducing polyoxometalates (POMs) as an ideal candidate for the membrane functionalization via a novel sal-gel method. A two-step protocol, adsorptive separation and catalytic degradation, was designed for dye removal, realizing an excellent dye rejection with easy and economic membrane regeneration through simply soaking the membrane in a limited volume of dilute oxidant solution. This approach is feasible and versatile owing to the flexible selection of distinct POMs and design of catalytic degradation routes as required. As a result, the current research provides insight into a new methodology of the membrane technique in dye removal applications. (C) 2015 Elsevier B.V. All rights reserved.
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