期刊
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
卷 61, 期 51, 页码 -出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/anie.202213328
关键词
Design Strategies; Highly Efficient Hydrogen Production; Small-Molecule Oxidation; Water Electrolysis
资金
- National Natural Science Foundation of China [52025013, 22121005]
- Haihe Laboratory of Sustainable Chemical Transformations
- 111 Project [B12015]
- Fundamental Research Funds for the Central Universities
The electrochemical oxidation of small molecules for hydrogen production and pollutant degradation has great advantages and potential applications.
The electrochemical oxidation of small molecules to generate value-added products has gained enormous interest in recent years because of the advantages of benign operation conditions, high conversion efficiency and selectivity, the absence of external oxidizing agents, and eco-friendliness. Coupling the electrochemical oxidation of small molecules to replace oxygen evolution reaction (OER) at the anode and the hydrogen evolution reaction (HER) at the cathode in an electrolyzer would simultaneously realize the generation of high-value chemicals or pollutant degradation and the highly efficient production of hydrogen. This Minireview presents an introduction on small-molecule choice and design strategies of electrocatalysts as well as recent breakthroughs achieved in the highly efficient production of hydrogen. Finally, challenges and future orientations are highlighted.
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