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Article
Chemistry, Multidisciplinary
Kefeng Ouyang et al.
Summary: A strategy to build an indium metal interphase on the zinc anode surface is proposed, preventing hydrogen evolution reaction and zinc corrosion, guiding smooth zinc deposition. This approach achieves ultrahigh cumulative capacities and stable plating/stripping behavior, with encouraging rate performance and cyclic stability for Zn-V2O5 batteries.
ADVANCED FUNCTIONAL MATERIALS
(2022)
Article
Engineering, Environmental
Chengkai Liu et al.
Summary: The research focuses on fabricating two-dimensional TiO2 nanosheets from Ti3C2Tx MXene via a one-step hydrothermal reaction, with controllable structure and component. The influences of TiO2 nanosheets content in PVA-based gel electrolyte were explored, leading to improved ionic conductivity and mechanical properties, resulting in highly stable Zn plating/stripping and excellent cycling performance.
CHEMICAL ENGINEERING JOURNAL
(2022)
Review
Chemistry, Inorganic & Nuclear
Huihui Yan et al.
Summary: This review discusses the electrolyte strategies for rechargeable aqueous zinc ion batteries (AZIBs), including diverse electrolytes, concentration choices, and flexible hydrogel electrolytes, as well as prospects for biocompatible or biodegradable bio-electrolytes as potential candidates.
COORDINATION CHEMISTRY REVIEWS
(2022)
Article
Nanoscience & Nanotechnology
Qiaotian Xiong et al.
Summary: This study focuses on designing porous and entangled network structures for sulfur-/nitrogen-co-doped kinked carbon nanofibers (S/N-KCNFs) to achieve high flexibility and rate capacities. The synthesized nanofiber films exhibited excellent rate performance and capacity retention, showcasing a new strategy for flexible structure design of high-performance potassium-ion storage materials.
NANO-MICRO LETTERS
(2022)
Article
Chemistry, Multidisciplinary
Yongchang Liang et al.
Summary: This study developed a unique dual-interface engineering strategy to design an efficient ion transport modulator separator for Zn metal batteries. By decorating BaTiO3 (BTO) on glass fiber, the modified separator can capture and accelerate ion transport, and distribute it homogenously, resulting in highly reversible Zn plating/stripping in the anode and improved battery performance.
ADVANCED FUNCTIONAL MATERIALS
(2022)
Article
Chemistry, Multidisciplinary
Yiwen Su et al.
Summary: In this study, a scalable Ti3C2Tx MXene-decorated Janus separator was designed and prepared, demonstrating superior performance in achieving dendrite-free zinc anodes. The separator exhibited abundant surface polar groups, good electrolyte wettability, and high ionic conductivity, which facilitated homogeneous current distribution and promoted zinc nucleation kinetics.
ADVANCED FUNCTIONAL MATERIALS
(2022)
Article
Polymer Science
Xiaobo Liang et al.
Summary: The study utilized conductive polyaniline to improve the water resistance, heat resistance, damping performance, mechanical properties, and antistatic properties of waterborne polyurethane-acrylate coatings.
POLYMERS FOR ADVANCED TECHNOLOGIES
(2022)
Article
Chemistry, Physical
Yongtao Wang et al.
Summary: A series of composite solid electrolytes (CSEs) with wide electrochemical stability window and high ionic conductivity were successfully prepared by integrating SiO2 nanoparticles into poly(vinyl ethylene carbonate) polymer electrolyte. These CSEs exhibit enhanced anti-oxidation performances and can be applied in SSLBs with high-voltage cathodes.
Article
Chemistry, Physical
Guoqiang Ma et al.
Summary: In this study, the stability of metallic zinc anode in aqueous batteries was significantly improved by using a non-concentrated aqueous zinc trifluoromethanesulfonate electrolyte with 1,2-dimethoxyethane additive. The introduction of DME disrupted the original hydrogen-bond network of water and created a unique Zn2+-solvation structure, effectively suppressing water-induced side reactions. The in-situ formation of an organic-inorganic hybrid interphase on the zinc anode further prevented water penetration and dendrite growth. This novel electrolyte enabled the zinc anodes to achieve unprecedented cycling stability and high reversibility.
ENERGY STORAGE MATERIALS
(2022)
Article
Thermodynamics
Menglin Wang et al.
Summary: This study analyzed the thermal performance of Ti-based MXene and found that terminal groups could reduce the phonon scattering and improve the thermal conductivity. Ti3C2O2 significantly improved the thermal conductivity of epoxy under lower filler content.
INTERNATIONAL JOURNAL OF HEAT AND MASS TRANSFER
(2022)
Article
Electrochemistry
Mingming Wang et al.
Summary: This study constructs a Zn/Bi electrode by in-situ growth of a Bi-based energizer upon the Zn metal surface using a replacement reaction. Experimental and theoretical calculations demonstrate that the Bi-based energizer composed of metallic Bi and ZnBi alloy contributes significantly to Zn plating/stripping due to strong adsorption energy and fast ion transport rates. The Zn/Bi electrode not only avoids Zn dendrite growth but also improves Zn anode anti-corrosion performance.
Review
Electrochemistry
Teng Zhang et al.
Summary: This review summarizes the recent advances in MXenes for lithium-sulfur batteries (LSBs), including their structural characterization, synthesis methods, and applications as cathodes, separators, and anodes. The challenges and future directions for research are also discussed.
Article
Chemistry, Multidisciplinary
Gang Ge et al.
Summary: MXene serves as a versatile cross-linker in hydrogels, activating fast gelation and enhancing mechanical properties, adhesion, and self-healing ability. Multiscale molecular interactions between MXene and polymers lead to significant variations in gelation behavior among different hydrogels.
Article
Chemistry, Multidisciplinary
Hwansoo Shin et al.
Summary: MXene nanosheets self-assembled into hydrogels can be spun into highly aligned fibers with increased electrical conductivity and Young's modulus. These oriented MXene fibers are expected to have widespread applications in electrical wiring and signal transmission.
Article
Engineering, Environmental
Zhiming Zhao et al.
Summary: The research team bypassed the obstacles by in-situ polymerization of a specific monomer to create amorphous zinc-ion solid-state polymer electrolytes, successfully addressing the challenges in rechargeable zinc-ion batteries. The new electrolyte exhibits high ambient ionic conductivity and low interfacial resistance, achieving highly reversible and dendrite-free zinc electrochemistry.
CHEMICAL ENGINEERING JOURNAL
(2021)
Article
Electrochemistry
Yachun Mao et al.
Summary: In recent years, research on flexible aqueous Zn-ion batteries has been promoted, but dendrite growth on the anode and poor mechanical properties of the flexible polymer electrolyte remain challenges. A CMC/PAM hydrogel electrolyte with a double-network structure has been constructed to address these issues, showing promising potential in improving the performance of flexible ZIBs.
ELECTROCHIMICA ACTA
(2021)
Article
Nanoscience & Nanotechnology
Chuang Sun et al.
Summary: Well-dispersed MXene nanosheets in the electrolyte facilitate Zn2+ migration and deposition, while the MXene interfacial layer induces uniform nucleation. The MXene-containing electrolyte enables dendrite-free Zn plating/striping with high efficiency and superior reversibility.
NANO-MICRO LETTERS
(2021)
Article
Chemistry, Physical
Yong Wang et al.
Summary: Solid polymer electrolytes (SPEs) with in-built inorganic fillers show great potential for safe solid-state batteries due to their flexibility, interfacial wettability, and cost-effectiveness. This study demonstrates the in situ cross-linking of polymer compounds and montmorillonite (MMT) using ultraviolet (UV) light, resulting in a solid composite electrolyte (CMP/MMT) with high ionic conductivity and lithium-ions transference number. The enhanced ionic conductivity is attributed to the electric field effect of MMT, facilitating rapid lithium-ion transport. Density functional theory (DFT) is used to explain the mechanism behind the improved ionic conductivity, showcasing the high capacity and excellent capacity retention of the solid-state battery with CMP/MMT after cycling.
Article
Polymer Science
Xin Huang et al.
Summary: The density and thermodynamic characteristics of hydrogen bonds control the stiffness and stretchability of polymer networks, while the activation energy of chain motion and the recovery rate after mechanical loading depend on the kinetic aspects of the hydrogen bonds.
Article
Chemistry, Physical
Jiawei Wang et al.
Summary: This study presents a new approach for developing natural polymer-based hydrogel electrolytes with high ionic conductivity and good antifreeze capability, achieved through blending guar gum and sodium alginate. The composite hydrogels demonstrated superior electrochemical performance in zinc-ion batteries, with excellent low-temperature discharge performance below -20 degrees C.
ENERGY STORAGE MATERIALS
(2021)
Article
Chemistry, Physical
Zeyu Li et al.
Summary: A novel Li+ conductor based on carbon quantum dots was successfully fabricated in this study, showing high ionic conductivity and excellent stability in Li-metal batteries, as well as the ability to withstand various deformations.
Article
Chemistry, Physical
Xiangcun Li et al.
Summary: A scalable N-doped hierarchically porous membrane with significant porosity has been reported as a protective interlayer for Li metal batteries, reducing safety hazards caused by lithium dendrites. The membrane features interconnected porous networks with carbon nanotubes as cores and N-doped carbon coating as crosslinked shells, allowing uniform distribution of Li+ ions and rapid diffusion of Li ions, leading to high Coulombic efficiency and dendrite-free morphology even after 500 hours of repeated Li plating/stripping processes. The protected Li anode exhibits excellent cycling stability in full cell batteries, with a low capacity decay rate of 0.03% per cycle.
ENERGY STORAGE MATERIALS
(2021)
Article
Nanoscience & Nanotechnology
Dong Liu et al.
Summary: The zinc-ion battery is a novel energy storage device with promising potentials. A novel solid polymer electrolyte utilizing coordination of zinc ions was designed and introduced into an all-solid ZIB, showing outstanding cycling stability and high coulombic efficiency.
ACS APPLIED MATERIALS & INTERFACES
(2021)
Article
Nanoscience & Nanotechnology
Cheuk Ying Chan et al.
Summary: The single-Zn-ion conducting hydrogel electrolyte (SIHE) exhibits single Zn2+ conductivity and outstanding ionic conductivity thanks to the abundant sulfates fixed on the IC polymer backbone, helping to address the issues of nonuniform deposition and parasitic side reactions in ZIBs.
ACS APPLIED MATERIALS & INTERFACES
(2021)
Review
Chemistry, Multidisciplinary
Xiao Wang et al.
Summary: This review discusses the key challenges of rechargeable aqueous zinc-ion batteries, analyzing the structural features and electrochemical properties of different cathode materials, and proposing various electrode design strategies to guide future research activities. The focus is mainly on achieving high energy density and durable cathode materials.
Article
Chemistry, Multidisciplinary
Cong Huang et al.
Summary: The research shows that saccharin (Sac) as an electrolyte additive can regulate the electrical double layer (EDL) structure on the zinc anode, forming a unique solid electrolyte interphase (SEI) that effectively modulates zinc deposition behavior and prevents side reactions, thus improving battery performance.
ADVANCED MATERIALS
(2021)
Article
Engineering, Environmental
Yongchang Liang et al.
Summary: A unique interface strategy, utilizing N,O co-doped Carbon nanofiber (CNF) interlayers on Zn metal anode surface, has been reported to regulate electrodeposition kinetics and inhibit dendrite formation in Aqueous zinc-ion batteries (AZIBs). The modified cell showed high Zn plating/stripping reversibility and stability at high current density, providing a new route to enable dendrite-free Zn metal anodes and high-performance AZIBs.
CHEMICAL ENGINEERING JOURNAL
(2021)
Article
Nanoscience & Nanotechnology
Ying Lin et al.
Summary: This study introduces a new strategy for fabricating highly thermally conductive phase change composites by constructing a spider web-like structured graphene skeleton in paraffin wax, significantly enhancing the material's thermal conductivity. The results demonstrate that the composite exhibits remarkably high thermal conductivity enhancements at low filler loading, showing promising applications in battery thermal management.
NANO-MICRO LETTERS
(2021)
Article
Chemistry, Physical
Shengli Di et al.
Summary: By pre-cycling Zn electrodes in an organic electrolyte, a stable organic-inorganic hybrid SEI layer can be formed on the Zn electrode, effectively reducing dendrite growth and water-induced side reactions in aqueous batteries, and improving the stability and lifespan of Zn electrodes.
ENERGY STORAGE MATERIALS
(2021)
Article
Electrochemistry
Xiulei Ji
Summary: Molten ZnCl2 hydrates are ionic liquids with intriguing physical and electrochemical properties, suitable for use as electrolytes in Zn metal batteries. Understanding the properties of molten ZnCl2 hydrates is crucial for designing high-performance electrolytes.
Article
Chemistry, Multidisciplinary
Yan-Fei Huang et al.
Summary: In this study, a novel approach using a relaxor ferroelectric (RFE) polymer of P(VDF-TrFE-CTFE) as the matrix of solid-state polymer electrolytes (SPEs) significantly increased the ionic conductivity in solid-state lithium metal batteries. The high dielectric constant of P(VDF-TrFE-CTFE) enabled enhanced solvation ability towards lithium ions and promoted dissociation, resulting in improved charge carrier mobility. The hybrid electrolytes with larger dielectric constant showed higher ionic conductivity, and tight interfaces of P(VDF-TrFE-CTFE) based SPEs ensured stable interfacial resistance during cycling, leading to stable cycling performance in LiFePO4/Li and LiNi0.8Co0.1Mo0.1O2/Li batteries at 25 degrees C. This work suggests a new research direction to construct SPEs with high ionic conductivity by increasing the dielectric constant of polymers.
ENERGY & ENVIRONMENTAL SCIENCE
(2021)
Article
Chemistry, Multidisciplinary
Ze Chen et al.
Summary: In this study, the issues faced by the zinc metal anodes in aqueous zinc ion batteries (ZIBs) were addressed using a solid polymer electrolyte, resulting in the development of all-solid-state ZIBs with superior stability and reliability. By effectively suppressing dendrites and side reactions, excellent cycling performance of up to 10,000 cycles was achieved, with the batteries able to function normally in temperatures ranging from -35 degrees Celsius to 100 degrees Celsius.
ENERGY & ENVIRONMENTAL SCIENCE
(2021)
Article
Chemistry, Physical
Xiaotong Wang et al.
Summary: By incorporating Ti3C2Tx MXene filler, the GPE membrane demonstrated improved electrochemical performance and enhanced conductivity, while preventing the formation of sodium dendrites on the electrode surface.
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ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
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