Janus Carbon Nanotube@poly(butylene adipate-co-terephthalate) Fabric for Stable and Efficient Solar-Driven Interfacial Evaporation

Solar-driven seawater desalination is considered a promising method for alleviating the water crisis worldwide. In recent years, significant efforts have been undertaken to optimize heat management and minimize salt blockage during solar-driven seawater desalination. However, it remains challenging to achieve an efficient and stable seawater evaporator simply and practically. Here, we designed and prepared a novel three-dimensional (3D) water channel evaporator (3D WCE) equipped with a Janus CNT@PBAT fabric (JCPF). The as-prepared Janus CNT@PBAT fabric has broad-band light absorption (similar to 97.8%), excellent superhydrophobicity (similar to 162 degrees), and photothermal properties. After optimizing the structure of the thermal insulator, our designed evaporator could realize the equilibrium between enhanced thermal management and sufficient water supply. As a result, the as-prepared evaporator achieved an excellent evaporation rate of 1.576 kg center dot m-2 center dot h-1 and an energy efficiency of over 92.7% under 1 sun irradiation in 3.5 wt % saline water. Moreover, this evaporator also revealed good salt rejection performance compared to the traditional two-dimensional (2D) water channel evaporator (2D WCE) in high saline water, which could maintain stable evaporation rates under long-term evaporation of 8 h. Our study may develop a simple method for the design and fabrication of a low-cost, effective, and stable solar-driven evaporator for seawater desalination.

Automated summary

Solar-driven seawater desalination is a promising method for addressing the global water crisis. This study presents a novel three-dimensional water channel evaporator equipped with a Janus CNT@PBAT fabric, which achieves excellent evaporation rate and energy efficiency through enhanced thermal management and salt rejection performance.