4.6 Article

Interfacial phase frustration stabilizes unconventional skyrmion crystals

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NPJ QUANTUM MATERIALS
卷 7, 期 1, 页码 -

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NATURE PORTFOLIO
DOI: 10.1038/s41535-022-00483-1

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  1. U.S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division

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This article presents a general method to induce exotic magnetic phases using interfacial phase frustration within artificially grown superlattices. Three unconventional magnetic phases are obtained through Monte Carlo calculations, and these frustration-induced phases can greatly enhance the spin chirality-driven topological Hall conductivity. This method provides a playground to realize unconventional magnetic phases in any family of materials that can be grown in superlattices.
Chiral magnetic phases with an unconventional topological twist in the magnetization are of huge interest due to their potential in spintronics applications. Here, we present a general method to induce such exotic magnetic phases using interfacial phase frustration within artificially grown superlattices. To demonstrate our method, we consider a multilayer with two different chiral magnetic phases as the competing orders at the top and bottom and show, using Monte Carlo calculations, that the interfacial phase frustration is realized at the central layer. In particular, we obtain three unconventional phases: a checkerboard skyrmion crystal, an incommensurate skyrmion stripe, and a ferrimagnetic skyrmion crystal. In these frustration-induced phases, the spin chirality-driven topological Hall conductivity can be largely enhanced. This method provides a playground to realize unconventional magnetic phases in any family of materials that can be grown in superlattices.

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