期刊
FRONTIERS IN MATERIALS
卷 9, 期 -, 页码 -出版社
FRONTIERS MEDIA SA
DOI: 10.3389/fmats.2022.934759
关键词
ZnO; Fe2O3; composite photocatalysts; sol-gel method; charge carrier; photocatalytic activity
资金
- Core Teacher Cultivating Program of the Yellow River Conservancy Technical Institute [2020HYGG04]
ZnO (ZO), Fe2O3 (FO), and graphene oxide (GO)/ZO/FO/ZnFe2O4 (ZFO) composite photocatalysts with high photocatalytic activity were successfully synthesized using a simple sol-gel method and low-temperature technology. These composite photocatalysts showed efficient degradation of dyes, refractory pollutants, and antibiotics.
ZnO (ZO), Fe2O3 (FO), and graphene oxide (GO)/ZO/FO/ZnFe2O4 (ZFO) composite photocatalysts have been synthesized successfully via a simple sol-gel method and low-temperature technology. The phase structure and microstructural analysis confirmed that the GO/ZO/FO/ZFO magnetic separation photocatalyst is composed of GO, hexagonal ZnO, rhombohedral Fe2O3, and spinel ZnFe2O4 without any other impurities. The GO/ZO/FO/ZFO composite photocatalysts have a high visible light optical absorption coefficient and photocatalytic activity for degrading dyes, refractory pollutants, and antibiotics. The degradation percentages of methyl orange, tetrabromobisphenol A, and oxytetracycline hydrochloride by the GO/ZO/FO/ZFO magnetic separation photocatalyst were 98% for 180 min, 99% for 150 min, and 85% for 180 min, respectively. The special synthesis path leads to the formation of a special heterojunction between GO, ZnO, Fe2O3, and ZnFe2O4, which does not change the optical band gap value of the main lattice Fe2O3, and enhances the surface defects of the GO/ZO/FO/ZFO magnetic separation photocatalyst, resulting in high charge carrier transfer and separation efficiency of the catalyst and then enhanced the photocatalytic activity of the GO/ZO/FO/ZFO magnetic separation photocatalyst.
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