期刊
JOURNAL OF ENVIRONMENTAL RADIOACTIVITY
卷 165, 期 -, 页码 197-205出版社
ELSEVIER SCI LTD
DOI: 10.1016/j.jenvrad.2016.09.015
关键词
U-236; Pu isotopes; Coral; Enewetak Atoll; Marshall Islands; Accelerator mass spectrometry
A comprehensive series of nuclear tests were carried out by the United States at Enewetak Atoll in the Marshall Islands, especially between 1952 and 1958. A Porites Lutea coral that was growing in the Enewetak lagoon within a few km of all of the high-yield tests contains a continuous record of isotopes, which are of interest (e.g. C-14, U-236 Pu-239,Pu-240) through the testing period. Prior to the present work, C-14 measurements at similar to 2-month resolution had shown pronounced peaks in the Delta C-14 data that coincided with the times at which tests were conducted. Here we report measurements of U-236 and Pu-239,Pu-240 on the same coral using accelerator mass spectrometry, and again find prominent peaks in the concentrations of these isotopes that closely follow those in C-14. Consistent with the (14) data, the magnitudes of these peaks do not, however, correlate well with the explosive yields of the corresponding tests, indicating that smaller tests probably contributed disproportionately to the debris that fell in the lagoon. Additional information about the different tests can also be obtained from the U-236/Pu-239 and (PU)-P-240/Pu-239 ratios, which are found to vary dramatically over the testing period. In particular, the first thermonuclear test, Ivy-Mike, has characteristic U-236/Pu-239 and Pu-240/Pu-239 signatures which are diagnostic of the first arrival of nuclear test material in various archives. (C) 2016 Elsevier Ltd. All rights reserved.
作者
我是这篇论文的作者
点击您的名字以认领此论文并将其添加到您的个人资料中。
推荐
暂无数据