4.6 Article

Regulation of Synoptic Circulation in Regional PM2.5 Transport for Heavy Air Pollution: Study of 5-year Observation Over Central China

期刊

出版社

AMER GEOPHYSICAL UNION
DOI: 10.1029/2021JD035937

关键词

regional PM2; 5 transport; synoptic circulation; air pollution; central China; FLEXPART-WRF modeling

资金

  1. National Natural Science Foundation of China [42075186, 41830965, 91744209]

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This study reveals the significant regulation of large-scale synoptic circulation on regional PM2.5 transport for heavy air pollution in central China. The observations and simulations identify the transport pathways and circulation patterns governing the transport of PM2.5 from upwind areas to the receptor region.
Regional transport of air pollutants is modulated by large-scale synoptic circulation, which has been poorly understood for heavy air pollution in the downstream receptor region. In the present study of 5-year (2015-2019) observation, we targeted the Twain-Hu Basin (THB), a region of heavy PM2.5 pollution over central China, to investigate the regulation of synoptic circulation governing regional PM2.5 transport for heavy air pollution. It was found that regional transport of PM2.5 predominated 65.2% of the heavy pollution events (HPEs) over the THB based on the statistics of observational environment and meteorology. By employing the FLEXPART-WRF model, the regional transport of PM2.5 from upwind areas in central and eastern China (CEC) to receptor region in the THB was identified with three prominent pathways in the northerly, northeasterly, and easterly directions respectively. We then used T-mode principal component analysis in conjunction with the K-means cluster method to categorize synoptic circulations, and it was recognized that three regional PM2.5 transport pathways for the HPEs over central China were governed respectively by three patterns of synoptic circulation over CEC with (a) weak high air pressure to the north (13.3%), (b) strong high air pressure to the northeast (46.7%), and (c) weak high air pressure to the east (40.0%). This study reveals a significant modulation of large-scale synoptic circulation for regional transport of air pollutants in environmental change.

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