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Article
Materials Science, Multidisciplinary
Si Liu et al.
Summary: In this study, researchers proposed a metal passivation technique for aqueous Zn-ion batteries to address the issues of dendrite formation, corrosion, and interfacial parasitic reactions. The technique involved the formation of an interfacial protective layer and the reconstruction of preferred crystal planes on the Zn surface, resulting in improved cycling life and low voltage polarization.
ENERGY & ENVIRONMENTAL MATERIALS
(2023)
Article
Chemistry, Physical
Minghui Qiu et al.
Summary: An ion-oriented interface of few-layer graphene (FLG) was constructed to achieve a long-life zinc (Zn) metal anode, which showed larger capacity and significant stability in cycling behavior, providing a novel approach for high-performance Zn anode fabrication.
JOURNAL OF ALLOYS AND COMPOUNDS
(2022)
Review
Chemistry, Multidisciplinary
Yanyan Wang et al.
Summary: This review provides an overview of advanced electrolyte strategies for optimizing zinc-ion batteries, including improving the compatibility between cathode materials and electrolytes, inhibiting anode corrosion and dendrite growth, extending electrochemical stability windows, enabling wearable applications, and enhancing temperature tolerance. The underlying scientific mechanisms, electrolyte design principles, and recent progress are presented to enhance understanding and inspiration for readers.
Article
Chemistry, Physical
Zhilin Yang et al.
Summary: This study systematically investigates the concept of using reversible lithiophilic sites in the context of Li metal battery performance. By comparing the performance of different types of single-atom doped graphene, it is found that single-atom manganese doped graphene has the most reversible lithiophilic site, which can guide uniform Li deposition and maintain structure stability.
ADVANCED ENERGY MATERIALS
(2022)
Article
Chemistry, Physical
Yongzheng Zhang et al.
Summary: In this study, a charge-enriched strategy through MXene-based polypyrrole (MXene-mPPy) layers was explored to achieve dendrite-free zinc metal anodes. The MXene-mPPy layers exhibited excellent charge enrichment ability and could homogenize the dispersion of electric field and ion flux, resulting in a dendrite-free zinc anode with an ultralong cycling lifespan and superior rate capability.
ADVANCED ENERGY MATERIALS
(2022)
Article
Chemistry, Multidisciplinary
Lin Hong et al.
Summary: This study successfully addresses the issues of dendrite growth and hydrogen evolution reaction on zinc metal anodes in Zn-ion batteries by developing a uniform and robust metallic Sb protective layer. The modified Zn anodes exhibit excellent cycling stability with dendrite-free and hydrogen-free behaviors.
Article
Multidisciplinary Sciences
Jindi Wang et al.
Summary: In this work, conformal growth of zinc hydroxide sulfate (ZHS) was achieved on Zn metal foil through a thermal annealing process, improving Zn2+ conductivity and forming a beneficial SEI layer on the Zn electrode. The achieved Zn electrode exhibited remarkable cycling stability and high efficiency, showcasing potential for practical application in energy storage systems.
Article
Chemistry, Physical
Chaowei Li et al.
Summary: This review elaborates on the fundamental reactions of Zn anodes in alkaline and neutral electrolytes, as well as the issues hindering their performance and the protective strategies to address these issues. It also highlights the challenges and opportunities in the development of high-performance Zn anodes.
ENERGY STORAGE MATERIALS
(2022)
Article
Chemistry, Multidisciplinary
Licheng Miao et al.
Summary: The introduction of a hydrophobic carbonate cosolvent in rechargeable aqueous zinc batteries can address the irreversible issues of Zn metal anodes by breaking the water's H-bond network, replacing solvating H2O, and creating a dendrite-free Zn2+-plating behavior. This efficient strategy with a hydrophobic cosolvent offers a promising direction for designing aqueous battery chemistries.
Article
Engineering, Environmental
Chenhui Ma et al.
Summary: The study improved the performance of aqueous Zn-ion batteries by constructing NiCo-LDH coating on the Zn anode, resulting in stable operation with high efficiency at low current density and impressive capacity at higher current density. This simple and low-cost method shows potential for industrialization of aqueous Zn-ion batteries.
CHEMICAL ENGINEERING JOURNAL
(2022)
Article
Chemistry, Multidisciplinary
Xunzhu Zhou et al.
Summary: This study focuses on constructing a stable anion-derived solid electrolyte interphase (SEI) by adding a co-solvent hydrofluoroether to a high-concentration 1,2-dimethoxyethane (DME) based electrolyte, which effectively restrains the growth of sodium dendrites and enhances the migration rate of sodium ions.
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
(2022)
Article
Engineering, Environmental
Wentao Yuan et al.
Summary: This study builds a robust and conductive ZnSO4.2H2O SEI layer on zinc anode in non-concentrated aqueous electrolyte, which terminates continuous HER and Zn corrosion, leading to high reversibility and long cycling life.
CHEMICAL ENGINEERING JOURNAL
(2022)
Article
Chemistry, Physical
Li-Feng Zhou et al.
Summary: The strategy of using Zn-Al-layered double hydroxides hexagonal nanoplates to modify the zinc metal anode has successfully improved the rechargeability and stability of rechargeable aqueous zinc ion batteries. The integrated electrode shows long-term stability and effectively suppresses zinc deposition and dendrite growth, offering a new pathway for Zn metal anode protection and accelerating the practical application of these batteries.
JOURNAL OF ALLOYS AND COMPOUNDS
(2022)
Article
Chemistry, Physical
Hao Zhang et al.
Summary: High yield carbon dots (CDs) with abundant polar functional groups are used to optimize the electrolyte/Zn interfaces, effectively preventing dendritic growth and parasitic reactions. The CDs also improve the reaction kinetics and lifespan of the Zn anode.
ADVANCED ENERGY MATERIALS
(2022)
Review
Multidisciplinary Sciences
Sailin Liu et al.
Summary: This review examines the failure mechanism of rechargeable zinc metal batteries under temperature influence, presents current electrolyte strategies for improving battery performance in harsh temperatures, and offers perspectives on their industrial application.
Article
Chemistry, Physical
Mintao Wan et al.
Summary: This paper reports a Li/graphene-C/Li3N composite electrode, which addresses the challenges of volume change and side reactions in lithium metal anodes in high energy density batteries through the stability of the graphene framework and the protection layer of Li3N. The electrode exhibits excellent electrochemical performance.
ENERGY STORAGE MATERIALS
(2022)
Article
Chemistry, Physical
Yi Liu et al.
Summary: By adding phosphoric acid to zinc electrolyte, the growth of zinc electrode can be made more uniform and reversible. This approach not only improves the cycling stability and rate capability of zinc-MnO2 batteries, but also makes aqueous zinc metal batteries competitive for practical applications.
ENERGY STORAGE MATERIALS
(2022)
Article
Multidisciplinary Sciences
Ruirui Zhao et al.
Summary: Researchers propose a new electrolyte formulation for aqueous zinc batteries, which involves the addition of lanthanum nitrate to improve the surface morphology of the electrode, enhancing the battery performance and cycle life.
NATURE COMMUNICATIONS
(2022)
Article
Nanoscience & Nanotechnology
Yinger Xiang et al.
Summary: In this study, Sb2S3 modified by carbon dots (Sb2S3@xCDs) was used to improve the initial coulombic efficiency (ICE) of alkali metal-ion batteries. The introduction of oxygen-rich carbon matrix helped inhibit the conversion of sulfur to sulfite, leading to a higher ICE for lithium-ion batteries. Additionally, the presence of Sb-O-C bonds in the interface improved the electronic conductivity and facilitated ion transmission, resulting in a high reversible capacity.
NANO-MICRO LETTERS
(2022)
Article
Nanoscience & Nanotechnology
Xunzhu Zhou et al.
Summary: The study reveals that Zn nuclei grow horizontally in radial direction during initial nucleation and early stages, and they dissolve reversibly in a top-down process. The critical nucleation radius and density are dependent on the electrolyte concentration of ZnCl2, providing guidelines for regulating uniform metal electrodeposition and yielding benefits for the development of anode-free batteries.
ACS APPLIED MATERIALS & INTERFACES
(2021)
Article
Chemistry, Physical
Yan Tan et al.
Summary: This review provides a comprehensive overview of the energy storage mechanisms in rechargeable zinc-ion batteries (ZIBs) and their reaction kinetics, emphasizing ion diffusion coefficients, pseudocapacitive behaviors, theoretically computational zinc-ion migration paths and energy barriers, as well as ion transference in electrolyte and anode. Additionally, advanced electrochemical measurements and theoretical calculation techniques for characterizing kinetic parameters are introduced.
JOURNAL OF POWER SOURCES
(2021)
Article
Chemistry, Physical
Huibing He et al.
Summary: This article discusses the electrochemistry of zinc, the degradation mechanism of zinc anodes, and the surface engineering strategies to address zinc dendrite issues. It summarizes the mechanisms of different coating materials, and proposes a design principle for an ideal interface layer on the zinc metal.
ENERGY STORAGE MATERIALS
(2021)
Review
Chemistry, Multidisciplinary
Xiao Wang et al.
Summary: This review discusses the key challenges of rechargeable aqueous zinc-ion batteries, analyzing the structural features and electrochemical properties of different cathode materials, and proposing various electrode design strategies to guide future research activities. The focus is mainly on achieving high energy density and durable cathode materials.
Article
Chemistry, Multidisciplinary
Jiahui Zhou et al.
Summary: By synthesizing a nitrogen-doped graphene oxide film on zinc foil, this study effectively suppresses hydrogen evolution reactions and passivation, improving the electrochemical performance of aqueous Zn-ion batteries. This research provides a new method for enhancing the application of high-specific-energy AZIBs.
ADVANCED MATERIALS
(2021)
Article
Chemistry, Physical
Ying Zhang et al.
Summary: The unique 2D Zn-Sb3P2O14 protective layer effectively addresses the issues of dendrite growth and side reactions of metallic zinc in aqueous batteries, enabling stable electron deposition and high Coulombic efficiency.
Article
Chemistry, Multidisciplinary
Huijun Yang et al.
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
(2020)
Article
Chemistry, Multidisciplinary
Daliang Han et al.
