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Article
Multidisciplinary Sciences
Huaihu Sun et al.
Summary: A non-flammable triethyl phosphate (TEP)-based electrolyte with tris(hexafluoroisopropyl)phosphate (THFP) as an additive has been developed. THFP helps to form a stable LiF-rich solid electrolyte interphase (SEI) layer, suppress lithium dendrite growth, and reduce electrolyte decomposition. THFP also participates in the formation of a stable electrolyte interphase (CEI) layer for stable cycling of the cathode.
Article
Chemistry, Physical
Ying Zhang et al.
Summary: This study utilizes a mixture of alizarin red S and p-phenylenediamine redox electrolytes dissolved in KOH solution as the anodic electrolyte for SCs, resulting in a flexible SC device that maintains high performance even under different bending conditions.
Article
Chemistry, Multidisciplinary
Sailin Liu et al.
Summary: This study presents a nonflammable, moderate-concentration electrolyte highly compatible with graphite anodes that exhibits exceptional cycling stability. The stability of the electrolyte is attributed to the nearly 100% solvation of TMP molecules with K+ cations and the formation of a F-rich solid electrolyte interphase. The findings highlight the importance of electrolyte-interface compatibility and offer new opportunities for designing safe and practical PIBs.
ADVANCED MATERIALS
(2021)
Article
Chemistry, Multidisciplinary
Mengfan Zhou et al.
Summary: Potassium ion batteries are considered a promising candidate for future energy storage devices due to their cost-effectiveness, high-voltage, and high-power operation. In addition to electrode materials, electrolytes also play a crucial role in determining cell performance. This Progress Report summarizes the research progress of electrolytes in PIBs and provides comprehensive guidance on the design of electrolyte systems for high performance PIBs.
ADVANCED MATERIALS
(2021)
Article
Chemistry, Multidisciplinary
Hao-Jie Liang et al.
Summary: By rationally designing the solvation configuration, a fully coordinated ether-based electrolyte with strong resistance against oxidation is reported, demonstrating excellent stability and performance with high-voltage cathodes. The assembled full cells show superior rate performance, unprecedented cycling stability, and high energy density, indicating promising prospects for application.
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
(2021)
Article
Chemistry, Multidisciplinary
Li-Li Jiang et al.
Summary: By utilizing a localized high-concentration electrolyte, a uniform and robust solid electrolyte interphase can be achieved on the graphite surface, leading to fast-charging performance and excellent cycling stability of lithium-ion batteries.
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
(2021)
Article
Chemistry, Physical
Sujong Chae et al.
Summary: A localized high-concentration electrolyte was designed for silicon anodes to enhance cycling stability over a wide temperature range, showing potential for improved battery performance. Full cells using this electrolyte retained 80% capacity after 500 cycles, demonstrating enhanced thermal stability. The electrolyte design principles developed in this study can be applied to extend the cycle life of other high-capacity electrode materials.
ACS ENERGY LETTERS
(2021)
Article
Multidisciplinary Sciences
Singyuk Hou et al.
Summary: Rechargeable magnesium and calcium metal batteries show promise as alternatives to lithium-ion batteries due to their high crustal abundance and capacity. By using a specific family of chelants, researchers were able to greatly improve the interfacial charge transfer kinetics and suppress side reactions, resulting in stable and highly reversible cycling performance for the batteries. This work provides a versatile electrolyte design strategy for divalent metal batteries.
Article
Chemistry, Physical
Dandan Yu et al.
Summary: This research introduces a fluorinated co-solvent-modified electrolyte to enhance the performance of graphite cathodes in dual-ion batteries, addressing issues of low Coulombic efficiencies and poor cyclability. By improving the cathode-electrolyte interface, side reactions are effectively inhibited, leading to enhanced stability of the cathodes.
ACS ENERGY LETTERS
(2021)
Article
Chemistry, Multidisciplinary
Chang Liu et al.
Summary: In this study, FeSe2@C NBs were successfully prepared by combining carbon coating, template etching, and hydrothermal selenization strategies. As a cathode material for potassium-ion batteries, FeSe2@C NBs exhibit high specific capacity and long cycle stability.
CHINESE CHEMICAL LETTERS
(2021)
Editorial Material
Chemistry, Multidisciplinary
Xiaotu Ma et al.
Summary: Given the increasing electrification of vehicles and the mass generation of spent lithium-ion batteries, recycling of LIBs is crucial. However, industrial-level recycling is challenging due to various factors that make large-scale recycling difficult while maintaining economic viability. Addressing these challenges and providing guidance towards solutions and future work is essential.
Article
Chemistry, Physical
Siyuan Li et al.
Summary: This study focuses on the design of a dual-layer solid electrolyte interface using lithium difluoro(oxalato)borate as the main salt, which has been successfully applied in phosphate ester/ether mixed electrolytes to improve the safety and reversibility of lithium metal batteries.
ENERGY STORAGE MATERIALS
(2021)
Article
Multidisciplinary Sciences
Leqing Deng et al.
Summary: The potassium-ion battery shows great potential as a post-Li-ion energy storage system, but the lack of high-performance cathode materials has been a barrier to practical applications. In this study, defect-free potassium manganese hexacyanoferrate is investigated as a cathode active material for high-energy and long-lasting potassium-based cells.
NATURE COMMUNICATIONS
(2021)
Article
Chemistry, Multidisciplinary
Zhang Cao et al.
Summary: This study demonstrates the superior cyclability of silicon anodes in lithium-ion batteries using a nonflammable ether-based electrolyte with dual additives. By forming a high-modulus SEI rich in fluoride and boron species, the Si/Li cells achieve a high initial Coulombic efficiency and low capacity-fading rate. Additionally, full cells pairing the unmodified Si anode with commercial cathodes show extended service life, highlighting the potential for developing high-performance Si-based batteries through Si/electrolyte interphase regulation.
ADVANCED MATERIALS
(2021)
Article
Chemistry, Multidisciplinary
Tao Li et al.
Summary: By regulating the electrolyte structure of anions using TPFPB anion acceptors, a stable anion-derived SEI was constructed to improve the stability and cycling performance of lithium metal batteries under practical conditions.
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
(2021)
Article
Materials Science, Multidisciplinary
Meng Zhou et al.
Summary: Biocarbon prepared from corn husks was used as anode material for potassium ion batteries, with the sample prepared at 1300 degrees Celsius showing the best electrochemical performance. The biocarbon exhibited higher graphitic degree and lower surface defects, leading to stable reversible capacity during cycling tests.
Article
Chemistry, Applied
Hao-Jie Liang et al.
Summary: A high-performance graphite@pitch-derived S-doped carbon tempura-like carbon/carbon nanocomposite has been synthesized for potassium-ion batteries, showing impressive rate capabilities and ultralong cyclic stability attributed to complementary advantages and synergy effects.
JOURNAL OF ENERGY CHEMISTRY
(2021)
Article
Chemistry, Physical
Tomooki Hosaka et al.
Summary: The study found that adding DTD as an electrolyte additive for K-metal cells can reduce polarization between electrodes, increase reversible capacity, and suppress irreversible capacity. By inhibiting the formation of oligocarbonates, it passivates and protects the K-metal surface, improving battery performance.
ACS ENERGY LETTERS
(2021)
Review
Chemistry, Multidisciplinary
Xiulin Fan et al.
Summary: The energy density of LIBs has been increased threefold since their introduction, but the capacity of transition metal oxide cathodes is approaching its limit due to stability limitations of electrolytes. To further enhance energy density, new high-capacity and high-voltage cathode materials need to be explored, and graphite anodes may need to be replaced. One of the main challenges for future development is the development of new electrolyte compositions that can accommodate high-voltage cathodes and anodes while ensuring the stability of the batteries.
CHEMICAL SOCIETY REVIEWS
(2021)
Article
Materials Science, Multidisciplinary
Yuyang Yi et al.
Summary: Nitrogen doping in carbon materials has been shown to enhance potassium-ion storage. This study introduces hierarchical N-doped carbon nanopolyhedron@nanosheet composite with tunable doping configurations for advanced potassium-ion hybrid capacitor (PIHC) anode, achieving outstanding rate capability and cyclic performance in half-cell tests. The assembled PIHC full device exhibits high energy/power density and favorable cyclicability, providing innovative insights for high-performance PIHC applications.
Review
Electrochemistry
Xia Cao et al.
Summary: Conventional LiPF6/carbonate-based electrolytes have been widely used in graphite-based lithium ion batteries for their stability, but are less stable in Li metal and silicon anodes. Localized high-concentration electrolytes have unique advantages, forming stable SEI layers to improve stability.
JOURNAL OF THE ELECTROCHEMICAL SOCIETY
(2021)
Article
Materials Science, Multidisciplinary
Sheng S. Zhang
Summary: This article discusses and proposes the design aspects of electrolytes for fast charging of lithium-ion batteries, highlighting how fast charging can exacerbate parasitic reactions and structural degradation of the electrolytes.
Article
Chemistry, Multidisciplinary
Sailin Liu et al.
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
(2020)
Article
Energy & Fuels
Ji Chen et al.
Article
Chemistry, Multidisciplinary
Jing Wu et al.
ADVANCED FUNCTIONAL MATERIALS
(2020)
Article
Chemistry, Physical
Yan Jin et al.
ACS ENERGY LETTERS
(2020)
Article
Chemistry, Multidisciplinary
Ling Fan et al.
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
(2019)
Article
Chemistry, Physical
Haiping Jia et al.
ADVANCED ENERGY MATERIALS
(2019)
Article
Chemistry, Physical
Xia Cao et al.
ACS ENERGY LETTERS
(2019)
Article
Chemistry, Physical
Lei Qin et al.
ADVANCED ENERGY MATERIALS
(2019)
Article
Chemistry, Multidisciplinary
Hao-Jie Liang et al.
ENERGY & ENVIRONMENTAL SCIENCE
(2019)
Article
Chemistry, Multidisciplinary
Xiaodi Ren et al.
Article
Chemistry, Physical
Gabin Yoon et al.
ADVANCED ENERGY MATERIALS
(2017)
Article
Chemistry, Multidisciplinary
Leigang Xue et al.
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
(2017)
Article
Chemistry, Multidisciplinary
Jin Zhao et al.
ADVANCED FUNCTIONAL MATERIALS
(2016)
Article
Chemistry, Multidisciplinary
Zelang Jian et al.
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
(2015)
Review
Chemistry, Physical
John B. Goodenough et al.
CHEMISTRY OF MATERIALS
(2010)
