☆ 4.7 Review

Perovskite Quantum Dots for Emerging Displays: Recent Progress and Perspectives

NANOMATERIALS (2022)

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Review Chemistry, Multidisciplinary

Surface Chemistry Engineering of Perovskite Quantum Dots: Strategies, Applications, and Perspectives

Yang Bai et al.

Summary: This article discusses the surface chemistry engineering of metal halide perovskite quantum dots (PQDs) and emphasizes the dual impact of surface ligands on the stability and performance of PQDs, highlighting innovative solutions. Significant achievements in the fields of photovoltaics and optoelectronics have been made through a deep understanding of the surface atomistic structure and defect mechanisms in PQDs.

ADVANCED MATERIALS (2022)

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Article Optics

Quantum-dot color conversion film patterned by screen printing and overprinting process for display backlights

Bingle Huang et al.

Summary: This paper presents an effective approach for preparing quantum-dot color conversion films in white-balance display backlights. The theoretical adjustment method and experimental verification successfully achieved the target white balance.

OPTICS AND LASER TECHNOLOGY (2022)

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Article Optics

Quantum-dot array with a random rough interface encapsulated by atomic layer deposition

Yu Chen et al.

Summary: This study proposes the use of atomic layer deposition (ALD) encapsulation as a stability-improving approach for a quantum-dot micro-structural array (QDMA) and discusses the influence of reaction temperature and deposition thickness on the encapsulation effect and output performance. The experimental results demonstrate significant improvement in stability and output performance for the encapsulated QD backlight.

OPTICS LETTERS (2022)

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Article Multidisciplinary Sciences

Thermal assisted up-conversion electroluminescence in quantum dot light emitting diodes

Qiang Su et al.

Summary: This study reveals the mechanism of hole injection into quantum dots under sub-bandgap bias and confirms thermal-assisted hole injection as the universal mechanism for up-conversion electroluminescence, through temperature-dependent electroluminescence and theoretical analysis.

NATURE COMMUNICATIONS (2022)

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Article Nanoscience & Nanotechnology

Full-visible-spectrum perovskite quantum dots by anion exchange resin assisted synthesis

Chenhui Wang et al.

Summary: In this study, full-visible-spectrum all-inorganic perovskite quantum dots (IPQDs) were successfully synthesized using an environmentally friendly ion-exchange approach with a renewable and low-cost anion exchange resin. The introduction of the anion exchange resin improved the optical performance and surface morphology of the IPQDs. The emission wavelength of the IPQDs could be controlled without changing their crystal phase, and IPQDs with poor morphology and unstable structure could be selectively removed. The photoluminescence quantum yield and fluorescence lifetime of the IPQDs were dramatically improved. This research provides new ideas for the environmentally friendly and sustainable synthesis of IPQDs, and shows great potential in the display field.

NANOPHOTONICS (2022)

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Article Engineering, Environmental

Efficient narrowband red electroluminescence from a thermally activated delayed fluorescence polymer and quantum dot hybrid

Liuqing Yang et al.

Summary: A hybrid emitting layer composed of a TADF polymer and red quantum dots has been proposed for narrowband red electroluminescence. By improving photoluminescent quantum yields and enhancing charge transfer, the wideband TADF is successfully converted to narrowband red emission, achieving a high external quantum efficiency.

CHEMICAL ENGINEERING JOURNAL (2022)

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Article Chemistry, Physical

Water-driven photoluminescence reversibility in CsPbBr3/PDMS-PUa composite

Junhu Cai et al.

Summary: This study systematically explores the mechanism of water interaction with perovskite nanocrystals, revealing the effects of water on fluorescence quenching, reversibility, and passivation of defect states. A new wearable intelligent sensing skin is demonstrated based on the reversible fluorescence mechanism.

NANO RESEARCH (2022)

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Article Engineering, Electrical & Electronic

Tripling Light Conversion Efficiency of μLED Displays by Light Recycling Black Matrix

Xiang Zhang et al.

Summary: This paper proposes a novel internal and external reflective black matrix (IERBM) to improve the light conversion efficiency and blue light utilization of quantum-dot color conversion film (QDCCF) in micro-light-emitting diode (μLED) displays. The optimized IERBM structure can significantly enhance the light conversion efficiency and blue light utilization, resulting in accurate white balance and high color uniformity in the μLED display.

IEEE PHOTONICS JOURNAL (2022)

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Article Materials Science, Multidisciplinary

Multi-layer co-extruded quantum-dot diffuser plate for ultra-large TV backlights

Honglei Ji et al.

Summary: This paper reports on an ultra-large laminated quantum dot diffuser plate for TV backlights, which exhibits outstanding long-term stability in harsh conditions. The TV prototype assembled with this diffuser plate achieves high color gamut, brightness, and uniformity, while having a simpler structure and lower cost compared to conventional QD-film based TVs.

OPTICAL MATERIALS EXPRESS (2022)

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Article Materials Science, Multidisciplinary

Ligand-Free CsPbBr3 Perovskite Quantum Dots in Silica-Aerogel Composites with Enhanced Stability for w-LED and Display by Substituting Pb2+ with Pr3+ or Gd3+ Ions

Chong Zhao et al.

Summary: This study proposes a facile and general method for synthesizing high-stable all-inorganic cesium-lead-halide quantum dots by integrating the growth of perovskite quantum dots with the fabrication process of hydrophobic silica-aerogel powders. The resulting composites show tunable photoluminescence and excellent stability under UV illumination, water moisture, and temperature variation.

ADVANCED OPTICAL MATERIALS (2022)

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Article Chemistry, Analytical

Red and Green Quantum Dot Color Filter for Full-Color Micro-LED Arrays

Bingxin Zhao et al.

Summary: This work demonstrated a method for fabricating color-conversion layers of red and green quantum dots color filters for full-color display arrays. By treating quantum dots with a compound containing epoxy functional groups and combining them with a photo-initiator, the protective function of quantum dots was achieved, and the pixel size of green quantum dot color filters was successfully reduced with a high optical density.

MICROMACHINES (2022)

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Article Materials Science, Multidisciplinary

ZnO Induced Self-Crystallization of CsPb(Br/I)3 Nanocrystal Glasses with Improved Stability for Backlight Display Application

Qin Wang et al.

Summary: Saving energy and reducing consumption are effective methods to alleviate energy shortages. In this study, self-crystallized perovskite materials with high photoluminescence quantum yield and adjustable full width at half maximum were prepared using the traditional melt-quenching method. These materials serve as downconverters for achieving high-brightness red backlight that meets wide color standards, providing an effective approach for fabricating wide color gamut backlights.

JOURNAL OF MATERIALS SCIENCE & TECHNOLOGY (2022)

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Review Nanoscience & Nanotechnology

Progress of Backlight Devices: Emergence of Halide Perovskite Quantum Dots/Nanomaterials

Rajan Kumar Singh et al.

Summary: Display technology is widely used in our daily lives, with LCD and OLED being the dominant technologies. Perovskite quantum dots show promise for backlit display devices, but their complex synthesis is a barrier to commercialization.

FRONTIERS IN NANOTECHNOLOGY (2022)

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Review Chemistry, Multidisciplinary

Aggregation and luminescence in carbonized polymer dots

Chunyuan Kang et al.

Summary: The luminescence mechanism of carbonized polymer dots (CPDs) is discussed in this review, with emphasis on their aggregation behavior. CPDs, as a new kind of luminescent nanomaterials, inherit the stability and biocompatibility of carbon materials, and possess the luminescence tunability, water solubility, and high photoluminescence quantum yield of organic luminescent materials. The review summarizes the special luminescence phenomena of CPDs in the aggregate state and discusses relevant mechanisms to consolidate relevant statements.

AGGREGATE (2022)

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Article Nanoscience & Nanotechnology

Enhanced Stabilities and Production Yields of MAPbBr(3) Quantum Dots and Their Applications as Stretchable and Self-Healable Color Filters

Han Sol Yang et al.

Summary: This study demonstrates the use of methyl acetate (MeOAc) as an effective non-solvent for purifying MAPbBr3 PQDs without causing severe damage, facilitating stable PQDs solutions with high production yields. MeOAc-washed PQDs maintain high photoluminescence (PL) quantum yields and crystalline structures for long periods. Time-resolved PL analysis shows that MeOAc-washed PQDs exhibit suppressed non-radiative recombination and longer PL lifetime compared to acetone-washed and methanol-washed PQDs.

ACS APPLIED MATERIALS & INTERFACES (2021)

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Article Chemistry, Multidisciplinary

Linear Electro-Optic Modulation in Highly Polarizable Organic Perovskites

Meng-Jia Sun et al.

Summary: By introducing BF4- as the X-site molecule, researchers were able to synthesize (DCl)(NH4)(BF4)(3), a material with a linear EO coefficient of 20 pm V-1, surpassing both metal halide perovskites and reported organic perovskites. The EO response of the organic perovskite approaches that of LiNbO3, demonstrating the potential of organically designed perovskites for use in efficient EO modulators.

ADVANCED MATERIALS (2021)

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Article Chemistry, Multidisciplinary

Extremely Stable Luminescent Crosslinked Perovskite Nanoparticles under Harsh Environments over 1.5 Years

Junho Jang et al.

Summary: Organic-inorganic hybrid perovskite nanoparticles (NPs) are a strong candidate for high-efficiency emitters, but their instability has been a critical issue. The reported crosslinked perovskite NP (CPN) shows exceptional stability in harsh environments and under high temperatures and humidity, enabling applications in displays and biocompatible cell proliferation.

ADVANCED MATERIALS (2021)

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Article Multidisciplinary Sciences

Liquid-phase sintering of lead halide perovskites and metal-organic framework glasses

Jingwei Hou et al.

Summary: By utilizing metal-organic framework glasses, a family of scalable composites was created to stabilize lead halide perovskite's nonequilibrium phases, resulting in bright photoluminescence and high stability.

SCIENCE (2021)

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Article Optics

Edge/direct-lit hybrid mini-LED backlight with U-grooved light guiding plates for local dimming

Enguo Chen et al.

Summary: A novel hybrid mini-LED backlight design is proposed in this study, which combines specially designed integrated light guiding plate (LGP) and local dimming technology. The design offers high optical performance and satisfactory local dimming effects, making it suitable for wide applications in large-area displays.

OPTICS EXPRESS (2021)

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Article Engineering, Environmental

Highly stable CsPbBr3 quantum dots by silica-coating and ligand modification for white light-emitting diodes and visible light communication

Xianwen Li et al.

Summary: In this study, stable DDAB-capped CsPbBr3 QDs coated with silica were prepared using a simple method, leading to improved PLQY and stability. These QDs were then applied in high-performance WLEDs, demonstrating excellent luminescent performance and potential for visible light communication.

CHEMICAL ENGINEERING JOURNAL (2021)

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Article Optics

Bright and stable light-emitting diodes made with perovskite nanocrystals stabilized in metal-organic frameworks

Hsinhan Tsai et al.

Summary: The use of metal-organic frameworks to stabilize perovskite nanocrystals for LED production results in bright and stable light emission, overcoming the instability issues associated with solid films.

NATURE PHOTONICS (2021)

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Article Nanoscience & Nanotechnology

Asymmetric Quantum-Dot Pixelation for Color-Converted White Balance

Enguo Chen et al.

Summary: This paper presents an effective method for achieving white balance in QDCCF displays by defining an asymmetric aperture ratio among the three primary-color subpixels. The experimental results show that the proposed approach can achieve high color gamut and is close to the standard light source.

ACS PHOTONICS (2021)

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Article Chemistry, Multidisciplinary

Highly luminescent and stable quasi-2D perovskite quantum dots by introducing large organic cations

Jingxi Wang et al.

Summary: Ultra-stable quasi-two-dimensional perovskite quantum dots have been synthesized by introducing the butylamine cation into the methylamine lead bromide perovskite, showing higher luminescence efficiency and environmental stability. Carbon quantum dot doping effectively passivates defects, further improving stability. This nanomaterial also demonstrates potential in environmental monitoring through a novel colorimetric method for H2O2 detection based on halide ion exchange.

NANOSCALE ADVANCES (2021)

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Article Chemistry, Physical

The role of sodium in stabilizing tin-lead (Sn-Pb) alloyed perovskite quantum dots†

Junke Jiang et al.

Summary: The introduction of sodium enhances the photoluminescence quantum yield of CsSn0.6Pb0.4I3 quantum dots, but the enhanced effect diminishes over time, resulting in a relatively short lifetime of high PLQYs. Engineering the surface termination of the quantum dots may be the next step in maintaining the favorable effect of Na doping for a high and stable PLQY of Sn-Pb QDs.

JOURNAL OF MATERIALS CHEMISTRY A (2021)

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Article Materials Science, Multidisciplinary

Heterogeneous post-passivation of inorganic cesium lead halide perovskite quantum dots for efficient electroluminescent devices

Xuefei Li et al.

Summary: A heterogeneous post-passivation process using formamidinium bromide (FABr) has shown more favorable electrical behavior for inorganic cesium lead halide perovskite quantum dots compared to a homogeneous post-passivation process using didodecyldimethylammonium bromide (DDAB). The FABr-treated quantum dots LEDs achieved a promising external quantum efficiency and luminance, significantly higher than the pristine and DDAB-treated samples. This methodology can also be applied to surface defect passivation of other types of perovskite quantum dots, enhancing both photoluminescence and electroluminescence performance simultaneously.

JOURNAL OF MATERIALS CHEMISTRY C (2021)

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Article Chemistry, Multidisciplinary

A polymer-coated template-confinement CsPbBr3 perovskite quantum dot composite

Jianhua Shen et al.

Summary: The study successfully synthesized polymer-coated CsPbBr3 quantum dots grown in situ on a template, using conjugated linoleic acid (CLA) as a ligand to passivate surface defects of QDs. Mesoporous silica microspheres were used as templates to improve the stability and absolute photoluminescence quantum yield of the quantum dots.

NANOSCALE (2021)

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Article Materials Science, Multidisciplinary

Poly(vinylidene fluoride)-passivated CsPbBr3 perovskite quantum dots with near-unity photoluminescence quantum yield and superior stability

Lin Yang et al.

Summary: In this study, CsPbBr3 quantum dots were synthesized using PVDF as the surface capping ligands, showing high photoluminescence quantum yield and excellent stability. The QLED prepared with the as-prepared QDs exhibited outstanding performance with an external quantum efficiency of 1.71%.

JOURNAL OF MATERIALS CHEMISTRY C (2021)

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Article Materials Science, Multidisciplinary

Engineering Sr-doping for enabling long-term stable FAPb1-xSrxI3 quantum dots with 100% photoluminescence quantum yield

Andres F. Gualdron-Reyes et al.

Summary: The substitution of lead by 7 at% strontium allows for the achievement of FAPb(1-x)Sr(x)I(3) PQDs with 100% PLQY and high stability for 8 months under a relative humidity of 40-50%. The suppression of structural defects mediated by Sr-doping decreases the non-radiative recombination mechanism in PQDs. Increasing the Sr content in PQDs leads to the emergence of a mixture of 2D nanoplatelets/3D nanocubes, caused by a high lead deficiency during the FAPb(1-x)Sr(x)I(3) synthesis.

JOURNAL OF MATERIALS CHEMISTRY C (2021)

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Article Chemistry, Multidisciplinary

Lead-free bright blue light-emitting cesium halide nanocrystals by zinc doping

Heng Xu et al.

Summary: A new class of lead-free non-perovskite blue-emitting cesium bromine and cesium iodine halide nanocrystals have been realized by zinc doping, achieving high photoluminescence quantum yield and excellent air stability. This provides a new avenue for fabricating lead-free halide nanocrystals for blue lighting and display applications.

RSC ADVANCES (2021)

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Review Chemistry, Multidisciplinary

Recent advances in luminescent materials for super-resolution imaging via stimulated emission depletion nanoscopy

Yanzi Xu et al.

Summary: Recent progress on STED fluorophores for super-resolution imaging is outlined, including inorganic fluorophores, fluorescent proteins, organic luminescent materials, aggregation-induced emission (AIE) luminogens, and fluorescent nanoparticles. Characteristics of these aforementioned STED fluorophores are also included and compared to provide a deep understanding of the relationship between the properties in luminescent materials and their performance in STED imaging.

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Bright Blue Light Emission of Ni2+ Ion-Doped CsPbClxBr3-x Perovskite Quantum Dots Enabling Efficient Light-Emitting Devices

Gencai Pan et al.

ACS APPLIED MATERIALS & INTERFACES (2020)

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Fei Yang et al.

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Highly Stabilized Gradient Alloy Quantum Dots and Silica Hybrid Nanospheres by Core Double Shells for Photoluminescence Devices

Hongxing Xie et al.

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Stacked Encapsulation Structure for Discretely Distributed Quantum Dot Array

Jing Cai et al.

IEEE PHOTONICS JOURNAL (2020)

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Bipolar-shell resurfacing for blue LEDs based on strongly confined perovskite quantum dots

Yitong Dong et al.

NATURE NANOTECHNOLOGY (2020)

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Perovskite Quantum Dots for Application in High Color Gamut Backlighting Display of Light-Emitting Diodes

Xicheng Wang et al.

ACS ENERGY LETTERS (2020)

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Enhancing the light-emitting performance and stability in CsPbBr3 perovskite quantum dots via simultaneous doping and surface passivation

Hengxiang Yang et al.

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Interfacial optimization of quantum dot and silica hybrid nanocomposite for simultaneous enhancement of fluorescence retention and stability

Hongxing Xie et al.

APPLIED PHYSICS LETTERS (2020)

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Lead-free, stable, high-efficiency (52%) blue luminescent FA3Bi2Br9 perovskite quantum dots

Yalong Shen et al.

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Zhiping Hu et al.

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Thermally Stable Copper(II)-Doped Cesium Lead Halide Perovskite Quantum Dots with Strong Blue Emission

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Improving the Stability of Metal Halide Perovskite Quantum Dots by Encapsulation

Wenzhen Lv et al.

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L-Type Ligand-Assisted Acid-Free Synthesis of CsPbBr3 Nanocrystals with Near-Unity Photoluminescence Quantum Yield and High Stability

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NANO LETTERS (2019)

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Constructing Gradient Energy Levels to Promote Exciton Energy Transfer for Photoluminescence Controllability of All-Inorganic Perovskites and Application in Single-Component WLEDs

Chao Luo et al.

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Vacuum-Drying Processed Micrometer-Thick Stable CsPbBr3 Perovskite Films with Efficient Blue-To-Green Photoconversion

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Bing-Le Huang et al.

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Shuyan Lin et al.

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Highly Efficient Light Emitting Diodes Based on In Situ Fabricated FAPbI3 Nanocrystals: Solvent Effects of On-Chip Crystallization

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Halogen-Hot-Injection Synthesis of Mn-Doped CsPb(Cl/Br)3 Nanocrystals with Blue/Orange Dual-Color Luminescence and High Photoluminescence Quantum Yield

Daqin Chen et al.

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A Facile Synthesis of Water-Resistant CsPbBr3 Perovskite Quantum Dots Loaded Poly(methyl methacrylate) Composite Microspheres Based on In Situ Polymerization

Yuting Cai et al.

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Zhiwen Yang et al.

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Jong Hyun Park et al.

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Mechanochemical synthesis of inorganic halide perovskites: evolution of phase-purity, morphology, and photoluminescence

Francisco Palazon et al.

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Bright and Uniform Green Light Emitting InP/ZnSe/ZnS Quantum Dots for Wide Color Gamut Displays

Yongwook Kim et al.

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Structure optimization of perovskite quantum dot light-emitting diodes

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Enhanced Two-Photon-Pumped Emission from In Situ Synthesized Nonblinking CsPbBr3/SiO2 Nanocrystals with Excellent Stability

Zhiping Hu et al.

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Room-Temperature Red-Green-Blue Whispering-Gallery Mode Lasing and White-Light Emission from Cesium Lead Halide Perovskite (CsPbX3, X = Cl, Br, I) Microstructures

Pengfei Guo et al.

ADVANCED OPTICAL MATERIALS (2018)

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Ioannis Lignos et al.

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Room-Temperature Triple-Ligand Surface Engineering Synergistically Boosts Ink Stability, Recombination Dynamics, and Charge Injection toward EQE-11.6% Perovskite QLEDs

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Postsynthesis Potassium-Modification Method to Improve Stability of CsPbBr3 Perovskite Nanocrystals

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Hong Zhou et al.

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