期刊
ACS PHOTONICS
卷 9, 期 9, 页码 3083-3088出版社
AMER CHEMICAL SOC
DOI: 10.1021/acsphotonics.2c00839
关键词
electron optics; coherence; ultrafast electron emission; femtosecond lasers; electron correlations; electron interference
类别
资金
- European Research Council (Consolidator Grant NearFieldAtto and Advanced Grant AccelOnChip)
- Deutsche Forschungsgemein-schaft (DFG, German Research Foundation) [429529648 - TRR 306]
- QuCoLiMa ( Quantum Cooperativity of Light and Matter )
- Sonderforschungsbereich 953 ( Synthetic Carbon Allotropes ) [182849149]
The transverse coherence of electrons is crucial in various applications such as electron microscopy. Pulsed versions of electron microscopy have been developed using femtosecond laser-triggering electron emission. In this study, we observed electron interference fringes and measured how the interference visibility decreases with increasing electron bunch charge. We explained the loss of coherence based on model simulations and linked the visibility reduction to an increase in the effective source size through the van Cittert-Zernike theorem.
The transverse coherence of electrons is of utmost importance in high resolution electron microscopes, point-projection microscopes, low-energy electron microscopy, and various other applications. Pulsed versions of many of these have recently been realized, mostly relying on femtosecond laser-triggering electron emission from a sharp needle source. We here observe electron interference fringes and measure how the interference visibility becomes reduced as we increase the emitted electron bunch charge. Due to the extremely strong spatiotemporal confinement of the electrons generated here, we observe the visibility reduction already at average electron bunch charges of less than 1 electron per pulse, owing to the stochastic nature of the emission process. We can fully and quantitatively explain the loss of coherence based on model simulations. Via the van Cittert-Zernike theorem, we connect the visibility reduction to an increase in the effective source size. We conclude by discussing emittance, brightness, and quantum degeneracy, which have direct ramifications to many setups and devices relying on pulsed coherent electrons.
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