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Recent Developments in Shape Memory Elastomers for Biotechnology Applications

POLYMERS (2022)

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Article Engineering, Environmental

A shape memory and antibacterial cryogel with rapid hemostasis for noncompressible hemorrhage and wound healing

Longtao Yao et al.

Summary: The study prepared a shape memory cryogel composed of QCS and MBG, which showed great potential for clinical application as a novel multifunctional hemostatic due to its efficient hemostatic, antibacterial, and wound healing-promoting properties.

CHEMICAL ENGINEERING JOURNAL (2022)

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Article Chemistry, Physical

Shape-Morphing Thermoactuators: Tetrathiafulvalene-Based Polymer Networks with an Effective Phonon Conduction Pathway

Minwoo Rim et al.

Summary: The development of a high thermal conductivity SMP is crucial for the fabrication of fast-responsive soft thermoactuators, with the TTF-SH monomer providing excellent thermal conductivity without the need for catalysts or initiators. The correlation between heat transfer and shape-morphing speed of the TTF SMP has been established, showing fast shape-morphing response due to its excellent thermal conductivity.

CHEMISTRY OF MATERIALS (2022)

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Article Polymer Science

Novel Composite Planks Made of Shape Memory Polyurethane Foaming Material with Two-Step Foaming Process

Jan-Yi Lin et al.

Summary: This study uses shape memory polyurethane (SMP) foaming material and carbon fiber woven fabrics to prepare sandwich-structured composite planks, which have excellent protection performances and electromagnetic wave shielding effectiveness.

POLYMERS (2022)

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Review Materials Science, Multidisciplinary

Smart materials in architecture for actuator and sensor applications: A review

Martin Sobczyk et al.

Summary: This paper discusses the application of smart materials in addressing challenges in architecture, focusing on civil structures. It examines the types, applications, and innovation potential of smart materials in civil engineering, emphasizing their importance and prospects in the field.

JOURNAL OF INTELLIGENT MATERIAL SYSTEMS AND STRUCTURES (2022)

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Article Polymer Science

Self-Healable and Recyclable Dual-Shape Memory Liquid Metal-Elastomer Composites

Xiaobo Deng et al.

Summary: This study reports a liquid metal-polymer composite that can undergo shape-changing and has self-healing and recyclable properties. The composite has a bilayer structure and achieves excellent shape programming abilities through the phase transitions of the liquid metal and crystalline polyurethane. By designing and building a heat-triggered soft gripper and a light-controlled reconfigurable switch for a circuit, the shape-morphing abilities of the composite are demonstrated.

POLYMERS (2022)

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Article Polymer Science

Synthesis and Characterization of Metallopolymer Networks Featuring Triple Shape-Memory Ability Based on Different Reversible Metal Complexes

Josefine Meurer et al.

Summary: This study synthesizes and characterizes metallopolymer networks with a triple shape-memory ability. The networks exhibit excellent dual and triple shape-memory abilities and have been analyzed using various techniques.

POLYMERS (2022)

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Article Polymer Science

Shape-Memory Composites Based on Ionic Elastomers

Antonio Gonzalez-Jimenez et al.

Summary: This study improves the performance of shape-memory polymers by adding fillers. Adding MWCNTs enhances the shape-memory effect and increases the conductivity of the material, allowing the shape-memory effect to be activated by an electric current. This research contributes to the development of elastic materials with high-performance and controllable shape-memory properties.

POLYMERS (2022)

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Article Polymer Science

Heterogeneous Solid-State Plasticity of a Multi-Functional Metallo-Supramolecular Shape-Memory Polymer towards Arbitrary Shape Programming

Guancong Chen et al.

Summary: This study presents a novel strategy to manipulate the permanent shapes of shape-memory polymers through solid-state plasticity. By utilizing dynamic metallo-supramolecular interactions, a multi-functional shape-memory polymer with tunable permanent shapes is developed. The material exhibits programmable shape-shifting behaviors and has potential practical applications.

POLYMERS (2022)

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Article Polymer Science

Electrospun Smart Oxygen Indicating Tag for Modified Atmosphere Packaging Applications: Fabrication, Characterization and Storage Stability

Shivam Panwar et al.

Summary: Pack integrity is crucial for successful modified atmosphere packaging of food products. This study developed a UV light-activated kappa-carrageenan-based oxygen indicating tag using the electrospinning technique, and its stability during storage was evaluated. The tag showed high sensitivity to oxygen and remained stable for at least 60 days in storage.

POLYMERS (2022)

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Review Polymer Science

Cutting-Edge Progress in Stimuli-Responsive Bioadhesives: From Synthesis to Clinical Applications

Elham Khadem et al.

Summary: With the development of intelligent materials, intelligent bioadhesives that respond to chemical, physical, or biological stimuli have been widely used in biomedical applications. These bioadhesives can undergo a phase shift in response to stimuli such as light, temperature, pH, and electric field, and they have advantages such as ease of use, sustained release, and reduced side effects. Fields such as tissue engineering, drug delivery, and cancer therapy have benefited from smart bioadhesives. However, the development of multifunctional bioadhesives for various biomedical applications is still not fully explored.

POLYMERS (2022)

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Article Chemistry, Multidisciplinary

Hydroxyl-Terminated Polybutadiene-Based Polyurethane with Self-Healing and Reprocessing Capabilities

Jiawei Li et al.

Summary: This study fabricates recyclable HTPB-PUV networks with dynamic boronic ester bonds, which possess superior thermostability and can be reprocessed, self-healed, and welded due to their altered network topologies.

ACS OMEGA (2022)

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Review Biochemistry & Molecular Biology

Non-Covalent Interaction on the Self-Healing of Mechanical Properties in Supramolecular Polymers

Kwanchai Buaksuntear et al.

Summary: This article introduces the intrinsic self-healing strategy based on supramolecular interaction or non-covalent interaction to enhance the mechanical properties of materials. The non-covalent interactions act as transient crosslinking points in materials, preventing and repairing broken polymer chains. Utilizing these strategies can increase the lifetime of products, achieve rapid healing, and reduce accidents and maintenance costs.

INTERNATIONAL JOURNAL OF MOLECULAR SCIENCES (2022)

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Article Polymer Science

Controlling Morphology and Physio-Chemical Properties of Stimulus-Responsive Polyurethane Foams by Altering Chemical Blowing Agent Content

Sayyeda Marziya Hasan et al.

Summary: This study investigates the effects of altering the concentration of a chemical blowing agent on the morphology, thermal and chemical properties, and actuation rates of amorphous shape memory polymer foams. Lower blowing agent concentration results in thicker foam struts and higher tensile modulus, while also reducing the strain at break and glass transition temperature. The findings provide an approach to control the foam properties and morphology in medical applications.

POLYMERS (2022)

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Article Engineering, Chemical

Blends of Poly(vinyl alcohol) and Poly(vinyl pyrrolidone): Interrelation between the Degree of Hydration and Thermal and Mechanical Properties

Petros Oikonomou et al.

Summary: Blends of poly(vinyl alcohol) (PVA) and poly(vinyl pyrrolidone) (PVP) readily absorb water when exposed to external humidity. The physical properties of the blends, including glass transition temperature (Tg) and mechanical properties, are affected by the increase in water content, with a linear relation between the weight fraction of absorbed water and the blend composition observed. Differential scanning calorimetry results showed that the depression of Tg with increasing water content could be accurately described by empirical equations, and the Young modulus of hydrated samples experienced a significant decrease when the blend transitioned from a glassy to rubbery state.

INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH (2021)

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Article Engineering, Chemical

UV Reconfigurable Shape Memory Polyurethane with a High Recovery Ratio under Large Deformation

Jing Hu et al.

Summary: A new type of shape memory thermoplastic polyurethane (TPU) was developed in this research, with photoresponsive anthracene groups incorporated into the hard segment to control stability and recoverability. This material achieved a high shape-fixing/recovery ratio and good performance even under large deformation, as well as free construction of three-dimensional shapes through photodimerization of anthracene groups.

INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH (2021)

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Article Polymer Science

Reconfigurable Surface Micropatterns Based on the Magnetic Field-Induced Shape Memory Effect in Magnetoactive Elastomers

Matija Lovsin et al.

Summary: A surface relief grating with a period of 30 μm is embossed onto the surface of magnetoactive elastomer (MAE) samples in the presence of a moderate magnetic field. The diffraction of the grating can be detected via a laser beam, and the diffraction efficiency depends on the applied magnetic field. The effect is more prominent in MAE samples with a higher content of iron filler.

POLYMERS (2021)

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Article Multidisciplinary Sciences

Current challenges in thermodynamic aspects of rubber foam

Supitta Suethao et al.

Summary: Natural rubber foam produced by the Dunlop method using concentrated natural latex with chemical agents shows increased density and compression strength with higher NR matrix concentration. Mechanical properties were consistent with computational modeling, and thermodynamic aspects demonstrated an increase in internal energy force, entropy, and activation enthalpy with increasing matrix concentration. New scientific concepts for thermodynamic parameters in compressed crosslinked NR foam were proposed and discussed, aiming to improve knowledge and development of rubber foams based on the structure-properties relationship.

SCIENTIFIC REPORTS (2021)

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Article Polymer Science

The Relationship between the Morphology and Elasticity of Natural Rubber Foam Based on the Concentration of the Chemical Blowing Agent

Supitta Suethao et al.

Summary: This study investigated the effect of varying the concentration of chemical blowing agent in rubber foam on its morphological properties and mechanical properties, finding that it affects the former but not the latter, revealing the heterogeneous structure of the foam. The research could be applied in the foam industry for controlling the morphological properties of rubber foam without altering its mechanical properties.

POLYMERS (2021)

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Article Biochemistry & Molecular Biology

Biomass Shape Memory Elastomers with Rapid Self-Healing Properties and High Recyclability

Zixun Chen et al.

Summary: BbPEs were successfully synthesized with shape memory and self-healing abilities by forming abundant hydrogen bonds among amide bonds and physical and chemical cross-linking. The material exhibits good mechanical properties, with a tensile strength of 4.4 +/- 0.1 MPa and shape memory recovery rate of 95% at 60 degrees C. These properties make it suitable for a wide range of practical applications such as intelligent electronic devices and bionic materials.

BIOMACROMOLECULES (2021)

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Article Polymer Science

Shape memory and self-healing behavior of styrene-butadiene-styrene/ethylene-methacrylic acid copolymer (SBS/EMAA) elastomers containing ionic interactions

Wenjing Wu et al.

JOURNAL OF APPLIED POLYMER SCIENCE (2020)

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Article Polymer Science

Star-Shaped Crosslinker for Multifunctional Shape Memory Polyurethane

Xiuhuan Song et al.

POLYMERS (2020)

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Review Materials Science, Multidisciplinary

Smart Polymers for Advanced Applications: A Mechanical Perspective Review

Roberto Brighenti et al.

FRONTIERS IN MATERIALS (2020)

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Review Chemistry, Physical

Recent Progress in Processing Functionally Graded Polymer Foams

Supitta Suethao et al.

MATERIALS (2020)

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Article Polymer Science

Effect of Fillers on the Recovery of Rubber Foam: From Theory to Applications

Thridsawan Prasopdee et al.

POLYMERS (2020)

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Article Engineering, Manufacturing

Magnesium acrylate induced interfacial compatibilization of EPDM/PP thermoplastic vulcanizate and shape memory behavior

Rui Cui et al.

COMPOSITES PART A-APPLIED SCIENCE AND MANUFACTURING (2019)

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Article Polymer Science

Fabrication and Characterization of Thermal-Responsive Biomimetic Small-Scale Shape Memory Wood Composites with High Tensile Strength, High Anisotropy

Luhao Wang et al.

POLYMERS (2019)

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Review Chemistry, Multidisciplinary

Shape Memory Polyurethane and its Composites for Various Applications

Arvind Gupta et al.

APPLIED SCIENCES-BASEL (2019)

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Article Materials Science, Composites

Triple-stimuli responsive shape memory effect of novel polyolefin elastomer/lauric acid/carbon black nanocomposites

Jiang Du et al.

COMPOSITES SCIENCE AND TECHNOLOGY (2019)

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Multi-stable mechanical metamaterials by elastic buckling instability

Hang Yang et al.

JOURNAL OF MATERIALS SCIENCE (2019)

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Article Chemistry, Multidisciplinary

Near-infrared light-induced shape memory, self-healable and anti-bacterial elastomers prepared by incorporation of a diketopyrrolopyrrole-based conjugated polymer

Yaling Zhang et al.

MATERIALS CHEMISTRY FRONTIERS (2019)

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Shape Memory Properties of Polystyrene-block-poly(ethylene-co-butylene)-block-polystyrene (SEBS) ABA Triblock Copolymer Thermoplastic Elastomers

Marcos Pantoja et al.

ACS APPLIED POLYMER MATERIALS (2019)

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Review of Progress in Shape Memory Epoxies and Their Composites

Jozsef Karger-Kocsis et al.

POLYMERS (2018)

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Article Nanoscience & Nanotechnology

3D Printing of Highly Stretchable, Shape-Memory, and Self-Healing Elastomer toward Novel 4D Printing

Xiao Kuang et al.

ACS APPLIED MATERIALS & INTERFACES (2018)

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Unique Shape Memory Elastomer Associated with Reversible Sacrificial Hydrogen Bonds: Tough and Flexible When below Its Tg

Tengfei Lin et al.

ADVANCED ENGINEERING MATERIALS (2018)

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Recent Progress in Shape Memory Polymers for Biomedical Applications

Hong-Mei Chen et al.

CHINESE JOURNAL OF POLYMER SCIENCE (2018)

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4D printed thermally activated self-healing and shape memory polycaprolactone-based polymers

Marta Invernizzi et al.

EUROPEAN POLYMER JOURNAL (2018)

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4D printing of shape memory polyurethane via stereolithography

Tingting Zhao et al.

EUROPEAN POLYMER JOURNAL (2018)

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Enhanced dual-responsive shape memory nanocomposites with rapid and efficient self-healing capability

Shuyun Zhuo et al.

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A UV-curable epoxy with soft segments for 3D-printable shape-memory materials

Jing Wang et al.

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Self-assembly nucleic acid-based biopolymers: learn from the nature

Pitchaya Pakornpadungsit et al.

JOURNAL OF POLYMER RESEARCH (2018)

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Poly(amide-ether) Thermoplastic Elastomers Based on Monodisperse Aromatic Amide Hard Segments as Shape-Memory and Moisture-Responsive Materials

Yuji Shibasaki et al.

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Applications of Shape Memory Polymers in Kinetic Buildings

Jing Li et al.

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Super-tough hydrogels from shape-memory polyurethane with wide-adjustable mechanical properties

Feng Wu et al.

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Douglas Naue Simoes et al.

MATERIALS RESEARCH-IBERO-AMERICAN JOURNAL OF MATERIALS (2017)

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Elastic Shape Memory Hybrids Programmable at Around Body-Temperature for Comfort Fitting

Tao Xi Wang et al.

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A mini review: Shape memory polymers for biomedical applications

Kaojin Wang et al.

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An overview of elastic polymeric shape memory materials for comfort fitting

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Fabrication of shape memory natural rubber using palmitic acid

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Preparation, Characterization, and Mechanism for Biodegradable and Biocompatible Polyurethane Shape Memory Elastomers

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Florence Pilate et al.

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Physical and thermal effects on the shape memory behaviour of auxetic open cell foams

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Recyclable Shape-Memory Polymer: Poly(lactic acid) Crosslinked By a Thermoreversible Diels-Alder Reaction

Kazuhiko Inoue et al.

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Preparation and Characterization of Shape Memory Elastomeric Composites

Xiaofan Luo et al.

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Evaluation of nanoparticulate fillers for development of shape memory polyurethane nanocomposites

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Challenges of Shape Memory Polymers: A Review of the Progress Toward Overcoming SMP's Limitations

Ingrid A. Rousseau

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