期刊
SCIENTIFIC REPORTS
卷 12, 期 1, 页码 -出版社
NATURE PORTFOLIO
DOI: 10.1038/s41598-022-14845-z
关键词
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资金
- JST-CREST
- JST-Mirai [JPMJCR15F3, JPM-JCR20B4, JPMJMI21G9, JPMJCR16F2]
- JSPS KAKENHI [JP19H01820, JP20H00127, JP20H00354, JP20H01834, JP21H05232, JP21H05233, JP21H05234, JP21K05235, JP21H05236]
This paper presents a dry pick-and-flip assembly technique for angle-resolved photoemission spectroscopy (ARPES) of van der Waals heterostructures. By altering the glass transition temperature of polymers, the flipping assembly of 2D heterostructures is achieved.
We present a dry pick-and-flip assembly technique for angle-resolved photoemission spectroscopy (ARPES) of van der Waals heterostructures. By combining Elvacite2552C acrylic resin and 1-ethyl-3-methylimidazolium ionic liquid, we prepared polymers with glass transition temperatures (T-g) ranging from 37 to 100 degrees C. The adhesion of the polymer to the 2D crystals was enhanced at T-g. By utilizing the difference in T-g, a 2D heterostructure can be transferred from a high-T-g polymer to a lower-T-g polymer, which enables flipping its surface upside down. This process is suitable for assembling heterostructures for ARPES, where the top capping layer should be monolayer graphene. The laser-based micro-focused ARPES measurements of 5-layer WTe2, 3-layer MoTe2, 2-layer WTe2/few-layer -Cr2Ge2Te6, and twisted double bilayer WTe2 demonstrate that this process can be utilized as a versatile sample fabrication method for investigating the energy spectra of 2D heterostructures.
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