☆ 4.8 Review

Emerging Organic Surface Chemistry for Si Anodes in Lithium-Ion Batteries: Advances, Prospects, and Beyond

ADVANCED ENERGY MATERIALS (2022)

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Scalable Synthesis of Pore-Rich Si/C@C Core-Shell-Structured Microspheres for Practical Long-Life Lithium-Ion Battery Anodes

Weili An et al.

Summary: In this study, a large-scale synthesis of a micro/nanostructured pore-rich Si/C microsphere was reported, which showed high porosity and stability, making it a promising anode material for high-energy-density lithium-ion batteries. The material displayed excellent cycle performance and capacity retention due to its structural advantages.

ACS APPLIED MATERIALS & INTERFACES (2022)

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Article Chemistry, Multidisciplinary

Matryoshka-type carbon-stabilized hollow Si spheres as an advanced anode material for lithium-ion batteries

Huimin Wu et al.

Summary: In this study, carbon-stabilized hollow silicon spheres were synthesized using an aluminothermic reduction and calcination process, and their potential as anode materials for lithium-ion batteries was investigated. The results showed that the synthesized Si/C/Si/C anode materials exhibited unique structures with preserved amorphous region and porous structures in the silicon layers. The anode displayed high initial specific capacity and good cycling performance.

CHINESE CHEMICAL LETTERS (2022)

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Article Chemistry, Multidisciplinary

Long-Cycling Sulfide-Based All-Solid-State Batteries Enabled by Electrochemo-Mechanically Stable Electrodes

Daxian Cao et al.

Summary: The anode is crucial for the energy density in all-solid-state lithium batteries. This study investigates the stability, processability, and cost of silicon anodes, highlighting their potential compared to lithium metal. By sandwiching the stabilized cathode and thin solid-state electrolyte with the silicon anode, high cell-level energy density and stability are achieved, inspiring large-scale commercialization of all-solid-state lithium batteries.

ADVANCED MATERIALS (2022)

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Article Chemistry, Multidisciplinary

Ionic electronic conductivity regulation of n-type polyoxadiazole lithium sulfonate conductive polymer binders for high-performance silicon microparticle anodes

Yuanyuan Yu et al.

Summary: A novel n-type conductive polymer binder has been successfully designed and applied to address the issue of cracks and fractures in silicon microparticles during the electrochemical cycle in lithium-ion batteries. By fine-tuning the monomer ratio, the ionic and electronic conductivities of the polymer can be precisely controlled, leading to improved cycling performance.

CHINESE CHEMICAL LETTERS (2021)

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Article Chemistry, Physical

Sticky carbon coating enables high-area-capacity lithium storage of silicon-graphitic carbon hybrid

Zidong Chen et al.

Summary: This study investigates the impact of surface coating layers on the lithium cycling performance of Si-graphitic carbon hybrid particles. It is found that the sticky-carbon coating layer significantly improves the cycle performance by alleviating electrode disintegration and forming a favorable SEI rich in fluorine-polymers. These positive findings highlight the importance of carbon coating layers with reactive surface groups for a wide range of Si-based anodes.

CARBON (2021)

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Article Nanoscience & Nanotechnology

Chemical Coupled PEDOT:PSS/Si Electrode: Suppressed Electrolyte Consumption Enables Long-Term Stability

Xuejiao Liu et al.

Summary: The incorporation of GOPS in Si/PEDOT:PSS electrodes improved the interface compatibility between Si and PEDOT:PSS, leading to the formation of a stable artificial SEI. The optimized electrode showed enhanced cycling performance and rate capability, maintaining 1000 mAh g(-1) for nearly 800 cycles under limited electrolyte. The full battery assembled with NCM 523 cathode achieved a high energy density of 520 Wh kg(-1) and exhibited good stability.

NANO-MICRO LETTERS (2021)

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Article Electrochemistry

Improving Lithium-Ion Diffusion Kinetics in Nano-Si@C Anode Materials with Hierarchical MoS2 Decoration for High-Performance Lithium-Ion Batteries

Xiongbiao Ye et al.

Summary: Introducing MoS2 nanosheets on a silicon anode can enhance structural stability and Li+ diffusion kinetics, resulting in improved performance and reversibility during lithiation/delithiation processes.

CHEMELECTROCHEM (2021)

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Article Multidisciplinary Sciences

1000 Wh L-1 lithium-ion batteries enabled by crosslink-shrunk tough carbon encapsulated silicon microparticle anodes

Fanqi Chen et al.

Summary: This study presents a method to enhance the electrochemical performance of microparticulate silicon by designing a strong and ductile carbon cage using capillary shrinkage of graphene hydrogel. The stable structure, similar to plant cells, shows 'imperfection-tolerance' to irregular volume variation of Si microparticles, maintaining electrode integrity over 1000 cycles with high Coulombic efficiency. The dense and thick microparticulate Si anode achieved an ultra-high volumetric energy density of 1048 Wh L-1 at pouch full-cell level.

NATIONAL SCIENCE REVIEW (2021)

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Article Nanoscience & Nanotechnology

In Situ Developed Si@Polymethyl Methacrylate Capsule as a Li-Ion Battery Anode with High-Rate and Long Cycle-Life

Wei Wang et al.

Summary: A novel Si capsule with in situ developed polymethyl methacrylate (PMMA) shell prepared via microemulsion polymerization shows excellent electrochemical performance and capacity retention at high current densities.

ACS APPLIED MATERIALS & INTERFACES (2021)

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Article Chemistry, Physical

Introducing SiC/C dual-interface on porous silicon anode by a conventional exothermic displacement reaction for improved cycle performance

Wenyang Zhou et al.

Summary: In this study, a porous Si anode protected by SiC/C dual-interface was prepared by a simple method, leading to significantly improved rate capability and cyclability of the battery by enhancing structural integrity.

JOURNAL OF POWER SOURCES (2021)

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Article Chemistry, Physical

Highly elastic and low resistance deformable current collectors for safe and high-performance silicon and metallic lithium anodes

Peng Liang et al.

Summary: By engineering the current collector with a novel strategy, a deformable structure covered with a high electrical conductivity surface is achieved, which stabilizes interfacial stress and improves electrode performance in silicon anode batteries, solid-state batteries, and ionic liquid electrolyte batteries.

JOURNAL OF POWER SOURCES (2021)

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Review Chemistry, Physical

Interface Aspects in All-Solid-State Li-Based Batteries Reviewed

Chunguang Chen et al.

Summary: Efforts to improve Li-ionic conductivity in solid electrolytes for all-solid-state Li-based batteries are crucial, and recent studies highlight the importance of addressing interface issues. Interface problems can significantly hamper electron and Li-ion transport, leading to storage capacity losses and battery failures. Understanding and controlling interfaces is key for optimizing battery performance.

ADVANCED ENERGY MATERIALS (2021)

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Article Chemistry, Multidisciplinary

Stable Silicon Anodes by Molecular Layer Deposited Artificial Zincone Coatings

Tiansheng Mu et al.

Summary: The stable interface between silicon anodes and electrolytes is crucial for reversible electrochemical cycling in lithium-ion batteries. In this study, a zincone polymer coating was controllably deposited on a silicon electrode using molecular layer deposition to serve as an artificial solid electrolyte interface, leading to improved lithium storage performance, high reversible capacity, outstanding cycling stability, and superior rate capability. The in situ conversion of the zincone coating also provides opportunities for constructing functional interfaces on other electrode surfaces, such as lithium/sodium metal.

ADVANCED FUNCTIONAL MATERIALS (2021)

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Article Computer Science, Hardware & Architecture

Battery Day

Jessie Frazelle

Summary: The text provides a detailed examination of the technology behind portable electronics.

COMMUNICATIONS OF THE ACM (2021)

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An additive-free silicon anode in nanotube morphology as a model lithium ion battery material

Ying Zhuo et al.

Summary: Ordered arrays of parallel, cylindrical silicon nanotubes were obtained by aluminothermic reduction of SiO2 nanotubes generated by ALD. These amorphous Si (a-Si) nanotube arrays exhibit electrochemical activity in lithium-ion batteries without additives, showing an increased capacity associated with faradaic reactions. Additionally, the nanotube morphology improves tolerance to fast cycling, as demonstrated by electrochemical impedance spectroscopy and charge-discharge tests.

ELECTROCHIMICA ACTA (2021)

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Article Chemistry, Physical

Robust Solid/Electrolyte Interphase (SEI) Formation on Si Anodes Using Glyme-Based Electrolytes

Guang Yang et al.

Summary: The study demonstrates that glyme-based electrolytes can effectively improve the stability and cycling performance of silicon anodes in lithium-ion batteries, reducing early parasitic current, decreasing interfacial resistance, and promoting capacity retention. Mechanistic investigation shows that GlyEl enriches the SEI on silicon with elastic polyether while diminishing carbonate species, making it a viable option for future high energy density lithium-ion batteries.

ACS ENERGY LETTERS (2021)

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Article Nanoscience & Nanotechnology

Tailoring Stress and Ion-Transport Kinetics via a Molecular Layer Deposition-Induced Artificial Solid Electrolyte Interphase for Durable Silicon Composite Anodes

Jia-Bin Fang et al.

Summary: This study explores the use of titanicone coating prepared by molecular layer deposition as a solid electrolyte interphase layer for silicon anodes, aiming to enhance the performance of lithium-ion batteries. The optimized titanicone-coated anode shows high cycling stability and excellent rate performance, indicating the potential for next-generation lithium-ion batteries.

ACS APPLIED MATERIALS & INTERFACES (2021)

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Design of high-energy-dissipation, deformable binder for high-areal-capacity silicon anode in lithium-ion batteries

Linlin Hu et al.

Summary: By synergizing static and dynamic binders, an efficient energy-dissipation engineering was applied to high-capacity silicon anodes, effectively improving their cycling stability and capacity retention. This strategy successfully avoids degradation of both materials and electrodes, laying the foundation for performance enhancement of silicon-based anodes.

CHEMICAL ENGINEERING JOURNAL (2021)

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Anomalous Si-based composite anode design by densification and coating strategies for practical applications in Li-ion batteries

Moon Kyu Cho et al.

Summary: By optimizing the design of Si/C composite anodes, modifying the surface with chemical vapor deposition, and doping with graphite, the performance of lithium-ion batteries can be significantly improved in terms of cycle life and efficiency.

COMPOSITES PART B-ENGINEERING (2021)

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Article Nanoscience & Nanotechnology

Progressive growth of the solid-electrolyte interphase towards the Si anode interior causes capacity fading

Yang He et al.

Summary: A correlated structural and chemical evolution of silicon and the solid-electrolyte interphase was unveiled in three dimensions by integrating sensitive elemental tomography, an advanced algorithm and cryogenic scanning transmission electron microscopy. The study demonstrated progressive electrolyte permeation and SEI growth along the percolation channel of the nanovoids due to vacancy injection and condensation during the delithiation process, leading to the formation of a 'plum-pudding' structure and the disruption of electron conduction pathways.

NATURE NANOTECHNOLOGY (2021)

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Article Multidisciplinary Sciences

Carbon-free high-loading silicon anodes enabled by sulfide solid electrolytes

Darren H. S. Tan et al.

Summary: The research successfully achieved stable operation of silicon anodes by using the interface passivating properties of sulfide solid electrolytes. Analysis showed that this approach eliminates continuous interfacial growth and irreversible lithium losses. The promising performance of microsilicon full cells can be attributed to the ideal interface properties between microsilicon and sulfide electrolytes and the unique chemomechanical behavior of the lithium-silicon alloy.

SCIENCE (2021)

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Review Multidisciplinary Sciences

Production of high-energy Li-ion batteries comprising silicon-containing anodes and insertion-type cathodes

Gebrekidan Gebresilassie Eshetu et al.

Summary: The authors discuss the use of silicon-containing anodes and insertion-type cathodes in battery systems, which have attracted significant interest for electric vehicles and renewable energy sources. However, these high-energy systems are limited by their complex chemistry and intrinsic drawbacks, requiring corresponding mitigating strategies.

NATURE COMMUNICATIONS (2021)

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Review Chemistry, Physical

Molecular Engineering Approaches to Fabricate Artificial Solid-Electrolyte Interphases on Anodes for Li-Ion Batteries: A Critical Review

Roman G. Fedorov et al.

Summary: A key challenge in lithium-ion batteries is the instability of electrolytes against anode materials, with the solid-electrolyte interphase (SEI) providing stability at the cost of capacity consumption. Artificial SEIs offer more flexibility to tune properties such as chemical composition and impedance, but must ensure sufficient transport properties for Li-ions and stability.

ADVANCED ENERGY MATERIALS (2021)

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Article Chemistry, Physical

Silicon Anodes with Improved Calendar Life Enabled By Multivalent Additives

Yunya Zhang et al.

Summary: By adding small concentrations of multivalent salts into the baseline electrolyte, silicon anodes with superior calendar life can be developed. The Ca additive reacts with F ions in the electrolyte to form a strong and dense layer of nanocrystalline CaF2, effectively protecting the silicon core from side reactions. This approach is universally effective for all available commercial silicon or SiO sources.

ADVANCED ENERGY MATERIALS (2021)

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Millisecond Conversion of Photovoltaic Silicon Waste to Binder-Free High Silicon Content Nanowires Electrodes

Jijun Lu et al.

Summary: An efficient and high-value recycling strategy for photovoltaic silicon waste is proposed in this study, converting it into stable silicon nanowire electrodes for lithium-ion batteries. The resulting electrode exhibits high initial Coulombic efficiency and robust cycle stability, potentially promoting the economic, environmentally friendly, and sustainable development of renewable energy.

ADVANCED ENERGY MATERIALS (2021)

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Correction Chemistry, Physical

Consecutive chemical bonds reconstructing surface structure of silicon anode for high-performance lithium-ion battery (vol 39, pg 354, 2021)

Qiushi Wang et al.

ENERGY STORAGE MATERIALS (2021)

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Consecutive chemical bonds reconstructing surface structure of silicon anode for high-performance lithium-ion battery

Qiushi Wang et al.

Summary: The study proposes a new method to stabilize silicon by successive chemical bond reconstruction, assembling silicon nanoparticles in a carbon-copper framework to provide short-range electron transfer and pulverization suppression, achieving high performance and stability in lithium-ion batteries.

ENERGY STORAGE MATERIALS (2021)

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Modularly aromatic-knit graphitizable phenolic network as a tailored platform for electrochemical applications

Gwan Hyun Choi et al.

Summary: By rearranging the molecular structure of tannic acid, a modularly interconnected TA (m-TA) was created with high residual carbon content and intrinsic graphitic carbonaceous matrix after carbonization. Additionally, electrochemically active metallic species were introduced post-carbonization, enhancing ionic and electrical conductivities of the graphitic sp(2) domains in the carbonized m-TA.

ENERGY & ENVIRONMENTAL SCIENCE (2021)

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High-Energy Nickel-Cobalt-Aluminium Oxide (NCA) Cells on Idle: Anode- versus Cathode-Driven Side Reactions

Alana Zulke et al.

Summary: The study reveals that different states of charge (SoC) have distinct impacts on the capacity fade of commercial lithium-ion cells, with noticeable differences in degradation rates for SoC values below and above 60%. Additionally, the storage state of the cells at different temperatures also affects the degradation rate.

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Mechanically robust and superior conductive n-type polymer binders for high-performance micro-silicon anodes in lithium-ion batteries

Yuanyuan Yu et al.

Summary: This study developed a series of novel n-type conductive polymer binders (CPBs) for SiMP anodes in lithium-ion batteries, demonstrating extraordinary electrochemical performance due to their superior properties. These designed polymers show excellent ionic and electronic conductivity in the n-doping state, filling a current research gap in the field and providing possibilities for preparing high-performance SiMP batteries. Furthermore, the high conductivity of b-POD binder shows better cycling performance and excellent fast-charging ability compared to non-conductive binders, enhancing the practical applications of SiMP batteries.

JOURNAL OF MATERIALS CHEMISTRY A (2021)

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Lithium-activated SnS-graphene alternating nanolayers enable dendrite-free cycling of thin sodium metal anodes in carbonate electrolyte

Wei Liu et al.

Summary: In this study, a lithium-ion activated tin sulfide graphene nanocomposite membrane was used as an artificial solid electrolyte layer for sodium metal batteries, enabling thin sodium metal foils to achieve excellent cyclability in a carbonate electrolyte. Metal cells protected by the membrane showed low-overpotential extended high-rate cycling. The post-mortem analysis revealed that the membrane effectively suppressed metal swelling, dendrite growth, and dead metal formation compared to unprotected samples.

ENERGY & ENVIRONMENTAL SCIENCE (2021)

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Review-Localized High-Concentration Electrolytes for Lithium Batteries

Xia Cao et al.

Summary: Conventional LiPF6/carbonate-based electrolytes have been widely used in graphite-based lithium ion batteries for their stability, but are less stable in Li metal and silicon anodes. Localized high-concentration electrolytes have unique advantages, forming stable SEI layers to improve stability.

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Solid-State Li-Metal Batteries: Challenges and Horizons of Oxide and Sulfide Solid Electrolytes and Their Interfaces

Kun Joong Kim et al.

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An electrolyte additive capable of scavenging HF and PF5 enables fast charging of lithium-ion batteries in LiPF6-based electrolytes

Jung-Gu Han et al.

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In Situ Atomic Force Microscopy Study of Initial Solid Electrolyte Interphase Formation on Silicon Electrodes for Li-Ion Batteries

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Critical Role of Silicon Nanoparticles Surface on Lithium Cell Electrochemical Performance Analyzed by FTIR, Raman, EELS, XPS, NMR, and BDS Spectroscopies

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Scalable production of large quantities of defect-free few-layer graphene by shear exfoliation in liquids

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Silicon-Based Nanomaterials for Lithium-Ion Batteries: A Review

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Stabilizing the Phase Li15Si4 through Lithium-Aluminum Substitution in Li15-xAlxSi4 (0.4 < x < 0.8)-Single Crystal X-ray Structure Determination of Li15Si4 and Li14.37Al0.63Si4

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Understanding Transition-Metal Dissolution Behavior in LiNi0.5Mn1.5O4 High-Voltage Spinel for Lithium Ion Batteries

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Observation of Microstructural Evolution in Li Battery Cathode Oxide Particles by In Situ Electron Microscopy

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Rationally Designed Hierarchical TiO2@Fe2O3 Hollow Nanostructures for Improved Lithium Ion Storage

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Structural and Electrochemical Study of Al2O3 and TiO2 Coated Li1.2Ni0.13Mn0.54Co0.13O2 Cathode Material Using ALD

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Influence of Silicon Nanoscale Building Blocks Size and Carbon Coating on the Performance of Micro-Sized Si-C Composite Li-Ion Anodes

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Silicon nanowire lithium-ion battery anodes with ALD deposited TiN coatings demonstrate a major improvement in cycling performance

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Nanosilicon Electrodes for Lithium-Ion Batteries: Interfacial Mechanisms Studied by Hard and Soft X-ray Photoelectron Spectroscopy

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Chemical Coupling of Carbon Nanotubes and Silicon Nanoparticles for Improved Negative Electrode Performance in Lithium-Ion Batteries

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Alumina-Coated Patterned Amorphous Silicon as the Anode for a Lithium-Ion Battery with High Coulombic Efficiency

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Mechano-chemical radical formation and polymerization initiation during wet grinding of alumina

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A review of the electrochemical performance of alloy anodes for lithium-ion batteries

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The Effects of Native Oxide Surface Layer on the Electrochemical Performance of Si Nanoparticle-Based Electrodes

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Toward Efficient Binders for Li-Ion Battery Si-Based Anodes: Polyacrylic Acid

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Ultralow Dielectric Constant Tetravinyltetramethylcyclotetrasiloxane Films Deposited by Initiated Chemical Vapor Deposition (iCVD)

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Ultrathin Direct Atomic Layer Deposition on Composite Electrodes for Highly Durable and Safe Li-Ion Batteries

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Effect of grinding conditions on mechanochemical grafting of poly(1-vinyl-2-pyrrolidone) onto quartz particles

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Scalable production of graphene sheets by mechanical delamination

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Atomic Layer Deposition: An Overview

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A review of the features and analyses of the solid electrolyte interphase in Li-ion batteries

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Surface chemistry and morphology of the solid electrolyte interphase on silicon nanowire lithium-ion battery anodes

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Real-Time NMR Investigations of Structural Changes in Silicon Electrodes for Lithium-Ion Batteries

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JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2009)

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Initiated and oxidative chemical vapor deposition of polymeric thin films: iCVD and oCVD

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Intrinsically stable dispersions of silicon nanoparticles

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High-performance lithium battery anodes using silicon nanowires

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Mussel-inspired surface chemistry for multifunctional coatings

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In situ conductivity, impedance spectroscopy, and ex situ raman spectra of amorphous silicon during the Insertion/Extraction of lithium

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JOURNAL OF PHYSICAL CHEMISTRY C (2007)

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Lithium insertion into amorphous silicon thin-film electrodes

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Single-molecule mechanics of mussel adhesion

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PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA (2006)

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Thermal decomposition of LiPF6-based electrolytes for lithium-ion batteries

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