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Bioinspired Freeze-Tolerant Soft Materials: Design, Properties, and Applications

SMALL (2022)

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Chan Wang et al.

Summary: Self-healing materials offer significant advantages in biomimetic intelligent robots by reducing safety hazards and economic losses caused by accidental damage. Researchers have developed a versatile ionic hydrogel with fast self-healing ability, ultra-stretchability, and stable conductivity, even in cryogenic environments. This hydrogel has been applied to create an artificial nerve fiber, demonstrating high fidelity and high throughput information interaction in extreme conditions.

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Antifreezing Hydrogel Electrolyte with Ternary Hydrogen Bonding for High-Performance Zinc-Ion Batteries

Siwen Huang et al.

Summary: This study demonstrates a new approach for designing high-performance antifreezing flexible batteries by utilizing the Hofmeister effect and low-concentration salts to regulate the chemical properties of hydrogel electrolytes. The optimized hydrogel electrolyte exhibits excellent flexibility and high ionic conductivity, enabling the zinc-ion battery to achieve good cycling performances even at low temperatures.

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Mechanochromic, Shape-Programmable and Self-Healable Cholesteric Liquid Crystal Elastomers Enabled by Dynamic Covalent Boronic Ester Bonds

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Summary: This study successfully designs and synthesizes a cholesteric liquid crystal elastomer (CLCE) with mechanochromic, shape-programmable, and self-healing capabilities. By introducing dynamic covalent Boronic ester bonds, reversible and dynamic tuning of circularly polarized reflection and robust self-healing abilities were achieved. This research provides insights for the development of 4D programmable photonic actuators.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2022)

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Article Biochemistry & Molecular Biology

Gelatin-Reinforced Zwitterionic Organohydrogel with Tough, Self-Adhesive, Long-Term Moisturizing and Antifreezing Properties for Wearable Electronics

Lilong Cao et al.

Summary: In this study, a novel organohydrogel with excellent mechanical performance, adhesion capacity, and biocompatibility was prepared. The organohydrogel exhibited long-term moisturizing and antifreeze properties, as well as good stability under -40 degrees C. Moreover, it could tightly attach to the human skin and real-time-monitor the motions of joints and the change in mood. This organohydrogel has great potential for wearable sensors under room temperature or extreme environments.

BIOMACROMOLECULES (2022)

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Article Biochemistry & Molecular Biology

Design of an Ice Recrystallization-Inhibiting Polyampholyte-Containing Graft Polymer for Inhibition of Protein Aggregation

Robin Rajan et al.

Summary: This study developed graft copolymers composed of a cryoprotective polymer and poly(vinyl alcohol) to protect proteins from freezing-induced damage. The graft polymers showed higher efficiency than PVA or PLLSA alone and exhibited a synergy between PVA and PLLSA, making them a promising material for long-term storage of proteins under freezing conditions.

BIOMACROMOLECULES (2022)

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Article Chemistry, Physical

Ultradurable, freeze-resistant, and healable MXene-based ionic gels for multi-functional electronic skin

Yao Lu et al.

Summary: This study successfully fabricated an E-skin with excellent performance, high sensitivity, and durability, capable of monitoring various human motions and physiological activities.

NANO RESEARCH (2022)

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Article Chemistry, Physical

A highly sensitive and ultra-stretchable zwitterionic liquid hydrogel-based sensor as anti-freezing ionic skin

Yabin Zhang et al.

Summary: The article presents a novel zwitterionic liquid polymer hydrogel with extraordinary mechanical versatility, high transparency, and conductivity, as well as anti-freezing ability, for multifunctional sensor applications. The hydrogel demonstrates excellent conductivity and low-temperature tolerance due to the conductive zwitterionic nanochannels formed by the zwitterionic liquid and methacrylate lysine. Additionally, the hydrogel exhibits high transparency, remarkable stretchability, self-healing properties, adhesiveness to diverse substrates, and high conductivity even at low temperatures, making it a promising candidate for strain sensors and ionic skin in wearable electronic devices.

JOURNAL OF MATERIALS CHEMISTRY A (2022)

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Review Materials Science, Biomaterials

Macromolecular cryoprotectants for the preservation of mammalian cell culture: lessons from crowding, overview and perspectives

Manish Gore et al.

Summary: Cryopreservation utilizes safe and effective macromolecular cryoprotectants to store mammalian cells at low temperatures, reducing toxicity and risks associated with conventional CPAs. These agents provide cryoprotection through various mechanisms involving macromolecular crowding, influencing the dynamics of freezing medium and cells. Understanding the structures and properties of macromolecular CPAs is crucial for enhancing cell preservation processes and encouraging their use in research.

JOURNAL OF MATERIALS CHEMISTRY B (2022)

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Tough, Antifreezing, and Conductive Hydrogel Based on Gelatin and Oxidized Dextran

Lilong Cao et al.

Summary: This study fabricates a gelatin/oxidized dextran hydrogel with enhanced mechanical strength, antifreeze property, and conductivity due to the synergistic interaction of ammonium sulfate and betaine. The hydrogel shows great potential for monitoring human body joint motion.

ADVANCED MATERIALS TECHNOLOGIES (2022)

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Article Nanoscience & Nanotechnology

Near-Infrared Light-Driven Shape-Programmable Hydrogel Actuators Loaded with Metal-Organic Frameworks

Xinmu Zhang et al.

Summary: This study presents the design and synthesis of near-infrared light-driven hydrogel actuators loaded with metal-organic frameworks. The metal-organic frameworks serve as efficient photothermal nanotransducers and accelerate the adsorption/desorption of water, leading to fast response rates of the actuators. By tailoring the patterning of the hydrogel actuators, different shape-morphing modes can be achieved under near-infrared light irradiation.

ACS APPLIED MATERIALS & INTERFACES (2022)

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Article Chemistry, Multidisciplinary

Anti-Freezing Self-Adhesive Self-Healing Degradable Touch Panel with Ultra-Stretchable Performance Based on Transparent Triboelectric Nanogenerators

Xingkui Guo et al.

Summary: A multi-functional surface-capacitive touch panel based on conductive hydrogels was developed, demonstrating high transparency, ultra-stretchability, and degradability. The touch panel exhibited fast response, high resolution, and low parasitic capacitance, while maintaining its functionalities even in high stretch and subzero conditions.

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Bioinspired Phototropic MXene-Reinforced Soft Tubular Actuators for Omnidirectional Light-Tracking and Adaptive Photovoltaics

Mengyuan Yang et al.

Summary: This article reports on a bioinspired phototropic MXene-reinforced soft tubular actuator that has omnidirectional self-orienting ability and can interact with incident light in all zenithal and azimuthal angles. The innovation of this actuator lies in its optimized materials and structure, which enable fast photoresponse and high light-tracking accuracy. A proof-of-concept demonstration of its application potential in solar energy harvesting is provided.

ADVANCED FUNCTIONAL MATERIALS (2022)

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Anti-freezing and self-healing nanocomposite hydrogels based on poly (vinyl alcohol) for highly sensitive and durable flexible sensors

Yu Nie et al.

Summary: This study successfully designed flexible sensors with anti-freezing properties and achieved high anti-freezing capabilities, mechanical strength, and self-healing efficiency through the synthesis of nanocomposite hydrogels. The flexible sensors exhibit fast response time, wide strain detection range, excellent stability, and fatigue resistance, making them suitable for accurate detection of human motion signals even in extreme low temperatures.

CHEMICAL ENGINEERING JOURNAL (2022)

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Anti-Freezing Strategies of Electrolyte and their Application in Electrochemical Energy Devices

Yao Liu et al.

Summary: This focus review summarizes the modified approaches and applications of electrolytes for anti-freezing performance in electrochemical energy devices. Various strategies and their effects are discussed, and the low-temperature performance indexes of different energy devices are summarized. Challenges and future prospects are also proposed.

CHEMICAL RECORD (2022)

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An anti-freezing and strong wood-derived hydrogel for high-performance electronic skin and wearable sensing

Zhenxing Wang et al.

Summary: Inspired by the structure of biological soft tissues, researchers have developed an anisotropic smart electronic skin system. The system combines a cellulose scaffold derived from natural wood with a polyvinyl alcohol/MXene nanosheets network, exhibiting high toughness and excellent conductivity. The e-skin can realize real-time monitoring of human motions and has anti-freezing and moisturizing capabilities.

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Ultra-antifreeze, ultra-stretchable, transparent, and conductive hydrogel for multi-functional flexible electronics as strain sensor and triboelectric nanogenerator

Xinhuan Dai et al.

Summary: Conductive hydrogels, due to their excellent mechanical flexibility, durability of deformation, and good electrical conductivity, have shown great potential in the field of flexible electronics. However, in order to ensure the stable operation of electronic devices in extreme environments, the development of environmentally robust hydrogels that can withstand extremely low temperatures and overcome dehydration is crucial. In this study, a graphene oxide incorporated hydrogel was developed, which exhibited excellent anti-freeze ability and maintained high sensitivity and stable output performances even at extremely low temperatures. This hydrogel provides a reliable and promising candidate for the new generation of wearable electronics.

NANO RESEARCH (2022)

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Bioinspired light-fueled water-walking soft robots based on liquid crystal network actuators with polymerizable miniaturized gold nanorods

Xiao Yang et al.

Summary: This research demonstrates water strider-inspired water-walking soft robots that can be remotely controlled by light, incorporating superhydrophobic floating surface with hierarchical nanostructures. The soft actuators exhibit photoinduced shape-bending deformation upon cyclic exposure to near-infrared light, enabling the soft robot to walk unidirectionally on water surface.

NANO TODAY (2022)

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Near-Infrared Light-Driven Three-Dimensional Soft Photonic Crystals Loaded with Upconversion Nanoparticles

Yaqi Qiu et al.

Summary: This study demonstrates the near-infrared light-driven reversible and dynamic photonic bandgap modulation of soft photonic crystal through the integration of core-shell upconversion nanoparticles and a novel molecular photoswitch. The intensity ratio of UV/vis luminescence emitted by the UCNPs can be controlled by changing the excitation power, leading to red-shift and blue-shift of the photonic reflection. This work provides new insights into the fabrication of 3D photonic nanostructures with tailorable functionalities for soft-matter photonics and integrated communication technologies.

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Anti-freezing and stretchable triboelectric nanogenerator based on liquid electrode for biomechanical sensing in extreme environment

Xinyang Zhao et al.

Summary: The development of an anti-freezing, stretchable, and liquid electrode-based TENG for biomechanical sensing in extremely cold environments is presented. The technology demonstrates high stretchability and electrical performance output, making it suitable for wearable sensors and powering electronic devices under harsh conditions.

NANO ENERGY (2022)

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Smart Hydrogel Sensors with Antifreezing, Antifouling Properties for Wound Healing

Saihua Tian et al.

Summary: This article presents the preparation of a multifunctional hydrogel for stress sensing and wound healing. The addition of zwitterionic polymers promotes wound healing by affecting macrophage polarization, collagen deposition, and blood vessel formation. Glycerin improves the resilience and frost resistance of the hydrogel, ensuring its functionality in cold environments. Additionally, zwitterionic polymers exhibit high biocompatibility and good electrical conductivity, enhancing sensing sensitivity and stability. This multifunctional hydrogel enables the detection of human vital activities while promoting wound healing, offering new possibilities for diagnosis and wound dressing.

ACS BIOMATERIALS SCIENCE & ENGINEERING (2022)

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Ultrahigh Conductive and Stretchable Eutectogel Electrolyte for High-Voltage Flexible Antifreeze Quasi-solid-state Zinc-Ion Hybrid Supercapacitor

Yihan Wu et al.

Summary: This paper presents a novel aqueous zinc-ion hybrid supercapacitor (ZHSC) with a robust and stretchable eutectogel electrolyte. The gel electrolyte is prepared through a one-step gelation process without additional initiators and crosslinkers. The ZHSC exhibits high ionic conductivity, extended voltage window, high energy density, admirable cycling stability, temperature stability, and bendability, making it a promising candidate for flexible wearable electronic devices.

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Ultrastretchable, Adhesive, Anti-freezing, Conductive, and Self-Healing Hydrogel for Wearable Devices

Xiaoli Zhao et al.

Summary: In this study, an ionic conductive cellulose hydrogel with ultrastretchable, adhesive, anti-freezing, and self-healing properties was fabricated. The hydrogel exhibited excellent mechanical properties and conductivity, making it suitable for human motion detection devices.

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Magnetic Structural Color Hydrogels for Patterned Photonic Crystals and Dynamic Camouflage

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Advances in 4D printing of liquid crystalline elastomers: materials, techniques, and applications

Zhecun Guan et al.

Summary: Liquid crystalline elastomers (LCEs) are polymer networks with liquid crystallinity and elastomeric properties, which can exhibit reversible high-speed and large-scale actuations in response to external stimuli. 4D printing of LCEs allows for microscopic changes in molecular orientation and macroscopic changes in properties, showing promising potentials in fields such as soft robotics, optics, and biomedical devices.

MATERIALS HORIZONS (2022)

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Nanocellulose/LiCl systems enable conductive and stretchable electrolyte hydrogels with tolerance to dehydration and extreme cold conditions

Wenjiao Ge et al.

Summary: The study proposes a double network hydrogel synthesized by one-step polymerization reaction, utilizing LiCl to enhance interactions between the colloidal phase and water molecules, ensuring water retention capability and freezing tolerance over a wide temperature range. The synergy between LiCl and CNF maintains mechanical strength and enables high stretchability and ionic conductivity in the system at low temperatures.

CHEMICAL ENGINEERING JOURNAL (2021)

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A wide temperature-tolerant hydrogel electrolyte mediated by phosphoric acid towards flexible supercapacitors

Jiajun Xu et al.

Summary: A novel hydrogel electrolyte with wide operating temperature range was successfully prepared in this study, which enabled the construction of supercapacitors with excellent flexibility and electrochemical stability from -60°C to 100°C.

CHEMICAL ENGINEERING JOURNAL (2021)

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Bats as natural samplers: First record of the invasive pest rice water weevil Lissorhoptrus oryzophilus in the Iberian Peninsula

Cecilia Montauban et al.

Summary: The global food security challenge is increasing due to the growing human population, leading to expansion of detrimental pest species in agricultural production. The first record of rice water weevil in the Iberian Peninsula was reported, confirming the invasive pest's range expansion using traditional sampling and DNA metabarcoding analysis. The study suggests the potential of insectivorous bats as natural samplers to detect and possibly control pest species in crops.

CROP PROTECTION (2021)

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Capacitive Pressure Sensors Containing Reliefs on Solution-Processable Hydrogel Electrodes

Hongwei Zhou et al.

Summary: By fabricating reliefs on PVA/PANI hydrogel electrodes, the GF of the pressure sensor is enhanced, and controlled by adjusting the composition and relief dimension. The optimized pressure sensor containing reliefs achieves the highest GF and has a sensing range of 0-7.4 kPa.

ACS APPLIED MATERIALS & INTERFACES (2021)

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Adhesive, Stretchable, and Transparent Organohydrogels for Antifreezing, Antidrying, and Sensitive Ionic Skins

Zhirui He et al.

Summary: The study introduces an organohydrogel-based sensor with antifreezing and antidrying properties, featuring high transparency, stretchability, and adhesiveness. It shows stable performance at extreme temperatures or long-term storage, and is capable of detecting various motions.

ACS APPLIED MATERIALS & INTERFACES (2021)

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Article Nanoscience & Nanotechnology

Conductive Hydrogel- and Organohydrogel-Based Stretchable Sensors

Zixuan Wu et al.

Summary: Conductive hydrogels have shown great potential for stretchable electronics, with improved stability, unique properties, and outstanding performance in sensors. However, there is still a lack of systematic summary on their working principles, properties, and applications.

ACS APPLIED MATERIALS & INTERFACES (2021)

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Article Chemistry, Multidisciplinary

Antifreezing Zwitterionic Hydrogel Electrolyte with High Conductivity of 12.6 mS cm-1 at-40 °C through Hydrated Lithium Ion Hopping Migration

Jianbo Yang et al.

Summary: The new zwitterionic polymer hydrogel electrolytes address the challenge of achieving high conductivity and flexibility at subzero temperatures, making them suitable for use in energy storage devices. The antifreezing electrolyte exhibits outstanding conductivity and mechanical properties, leading to high specific capacitance in supercapacitors.

ADVANCED FUNCTIONAL MATERIALS (2021)

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Review Chemistry, Multidisciplinary

Materials, Actuators, and Sensors for Soft Bioinspired Robots

Mahdi Ilami et al.

Summary: Biological systems inspire advancements in soft robotics, leading to the development of bioinspired soft actuators and sensors; this review surveys the progress in these fields between 2017 and 2020, focusing on the materials used in their design.

ADVANCED MATERIALS (2021)

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Review Chemistry, Multidisciplinary

3D Printed Flexible Strain Sensors: From Printing to Devices and Signals

Haodong Liu et al.

Summary: The revolutionary advancements in flexible electronics offer great potential for wearable devices and electronic skin, with flexible strain sensors serving as essential components in integrated electronic systems. 3D printing technology is preferred for manufacturing flexible strain sensors due to its cost-effectiveness, accuracy, and efficiency. Various printing methods, such as DLP, FDM, and DIW, are discussed in this study, along with the sensing mechanisms of the printed sensors and suggestions for future research directions.

ADVANCED MATERIALS (2021)

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Article Chemistry, Multidisciplinary

Near-Infrared Light-Driven Shape-Morphing of Programmable Anisotropic Hydrogels Enabled by MXene Nanosheets

Pan Xue et al.

Summary: This study presents a near-infrared light-driven shape-morphing MXene-containing anisotropic hydrogel actuator, which can perform various functions by controlling electrode pattern, electric field direction, and photopolymerization.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2021)

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Article Chemistry, Physical

Antifreezing and stretchable all-gel-state supercapacitor with enhanced capacitances established by graphene/PEDOT-polyvinyl alcohol hydrogel fibers with dual networks

Ting Xu et al.

Summary: A dual-network hydrogel fiber supercapacitor with excellent capacitance retention in cold environment and good stretchability was successfully constructed in this study. The supercapacitor exhibited high cycling stability and outstanding electrochemical performances, providing a new possibility for power supply of future wearable electronic devices.

CARBON (2021)

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Article Engineering, Environmental

Low-temperature tolerant strain sensors based on triple crosslinked organohydrogels with ultrastretchability

Qingyu Yu et al.

Summary: The XG-Fe3+/PAAm-Gl organohydrogel prepared in this study exhibits extremely high stretchability and strength, and maintains good stretchability, conductivity, and transparency even at -40 degrees Celsius. The bio-sensor fabricated using this organohydrogel shows remarkable sensitivity and a wide strain range under a broad range of temperatures, making it suitable for monitoring human physiological motions in various environments.

CHEMICAL ENGINEERING JOURNAL (2021)

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Article Engineering, Environmental

Anti-freezing, resilient and tough hydrogels for sensitive and large-range strain and pressure sensors

Yanyu Yang et al.

Summary: The study developed a wearable multi-model hydrogel sensor with high sensitivity and large-range detection capacity, featuring anti-freezing, durable properties and good performance within a wide temperature range.

CHEMICAL ENGINEERING JOURNAL (2021)

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Article Chemistry, Physical

Multifunctional Organohydrogel-Based Ionic Skin for Capacitance and Temperature Sensing toward Intelligent Skin-like Devices

Yuan Wei et al.

Summary: The organohydrogel-based ionic skin is fabricated through a unique design strategy, showing excellent stretchability, high Young's modulus, and superior ionic conductivity. This skin possesses durable adhesion and UV-blocking capabilities, as well as environmental stability. With superior mechanical response and thermal perception capacities, it can be used for real-time motion monitoring and dynamic temperature detection.

CHEMISTRY OF MATERIALS (2021)

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Review Materials Science, Multidisciplinary

Poly(N-isopropylacrylamide)-based smart hydrogels: Design, properties and applications

Lin Tang et al.

Summary: PNIPAM-based smart hydrogels are important smart materials with unique thermo-responsive properties and promising applications. This review summarizes the development, fundamental design, synthetic strategies, and potential applications of these materials in various fields.

PROGRESS IN MATERIALS SCIENCE (2021)

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Article Chemistry, Multidisciplinary

Food Waste Durian Rind-Derived Cellulose Organohydrogels: Toward Anti-Freezing and Antimicrobial Wound Dressing

Xi Cui et al.

Summary: Hydrogels synthesized from food waste and byproducts have shown anti-freezing and non-drying properties, along with antimicrobial activity when natural yeast phenolics are added. With no cytotoxicity, these organohydrogels can be applied as wound dressings in medical supplies, even in extreme temperature environments.

ACS SUSTAINABLE CHEMISTRY & ENGINEERING (2021)

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Review Chemistry, Multidisciplinary

Aqueous Rechargeable Metal-Ion Batteries Working at Subzero Temperatures

Yuwei Zhao et al.

Summary: This study discusses the freezing behavior of water and its effects on the subzero performances of ARMBs, summarizes strategies to enhance the subzero temperature performances of ARMBs, and compares the subzero temperature performances of ARMBs and organic electrolyte batteries.

ADVANCED SCIENCE (2021)

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Article Multidisciplinary Sciences

Perfusion, cryopreservation, and nanowarming of whole hearts using colloidally stable magnetic cryopreservation agent solutions

Andreina Chiu-Lam et al.

Summary: The study reports on an mCPA containing superparamagnetic iron oxide nanoparticles that can increase the preservation time of cryopreserved organs through nanowarming, reduce damage caused by slow rewarming, and have low cytotoxicity. The results demonstrate that this formulated mCPA is suitable for perfusion, vitrification, and nanowarming of whole organs.

SCIENCE ADVANCES (2021)

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Article Multidisciplinary Sciences

A thin, deformable, high-performance supercapacitor implant that can be biodegraded and bioabsorbed within an animal body

Hongwei Sheng et al.

Summary: This study introduces a novel fully biodegradable and bioabsorbable high-performance supercapacitor implant that is lightweight, thin, mechanically flexible, tunable in degradation duration, and biocompatible. The supercapacitor utilizes two-dimensional, amorphous molybdenum oxide flakes as electrodes and demonstrates high areal capacitance and energy density. Demonstrations in rat bodies show the potential uses of the supercapacitor implant for powering electronic devices and complete degradation post-implantation.

SCIENCE ADVANCES (2021)

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Article Chemistry, Multidisciplinary

A Spider-Silk-Inspired Wet Adhesive with Supercold Tolerance

Xi Liu et al.

Summary: A robust spider-silk-inspired wet adhesive composed of core-sheath nanostructured fibers has been reported, showing reliable adhesion even in wet and cold conditions, and even in liquid nitrogen. The unique dissolving-wetting-adhering process of core-sheath nanostructured fibers enables the wet adhesion of this adhesive, demonstrating promising applicability in cryogenic environments.

ADVANCED MATERIALS (2021)

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Article Chemistry, Multidisciplinary

Realizing an All-Round Hydrogel Electrolyte toward Environmentally Adaptive Dendrite-Free Aqueous Zn-MnO2 Batteries

Minfeng Chen et al.

Summary: A all-round hydrogel electrolyte was developed using cotton, tetraethyl orthosilicate, and glycerol, exhibiting high ionic conductivity and excellent mechanical properties.

ADVANCED MATERIALS (2021)

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Article Chemistry, Multidisciplinary

Electric-Field-Induced Gradient Ionogels for Highly Sensitive, Broad-Range-Response, and Freeze/Heat-Resistant Ionic Fingers

Yongyuan Ren et al.

Summary: This study demonstrates a gradient ionogel-based flexible iontronic sensor with high sensitivity and broader-range detection. The ionogels exhibit significant differences and show excellent performance under various conditions.

ADVANCED MATERIALS (2021)

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Article Biochemistry & Molecular Biology

Zwitterionic Hydrogel with High Transparency, Ultrastretchability, and Remarkable Freezing Resistance for Wearable Strain Sensors

Qin Jiao et al.

Summary: This study presents the development of an ultrastretchable, highly transparent, and antifreezing zwitterionic-based electronic sensor that can maintain its toughness and transparency down to -40 degrees C. The zwitterionic hydrogel exhibits good biocompatibility and protein adsorption resistance. Such zwitterionic hydrogel-based strain sensors could be highly valuable for wearable electronic devices, especially in extreme environment applications.

BIOMACROMOLECULES (2021)

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Article Materials Science, Composites

Self-healing, anti-freezing, adhesive and remoldable hydrogel sensor with ion-liquid metal dual conductivity for biomimetic skin

Zixuan Zhou et al.

Summary: The flexible wearable epidermal sensors assembled by ultra-sensitive PVA-TA-EGaIn hydrogels show potential in applications such as human motion monitoring, voice recognition, and medical diagnosis, thanks to their adhesiveness, rapid self-healing, high electrical conductivity, mechanical properties, and temperature sensitivity.

COMPOSITES SCIENCE AND TECHNOLOGY (2021)

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Review Chemistry, Applied

Recent advances of organogels: from fabrications and functions to applications

Liangpeng Zeng et al.

Summary: This review focuses on the current advances of organogels, summarizing fundamental understandings and emerging applications, as well as addressing the remaining challenges and future prospects.

PROGRESS IN ORGANIC COATINGS (2021)

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Article Polymer Science

An anti-freezing/drying, adhesive and self-healing motion sensor with humidity-enhanced conductivity

Kaixiang Yang et al.

Summary: A new class of conductive organohydrogel sensors with multipurpose adhesion, anti-freezing/drying, excellent humidity-enhanced conductivity, and self-healing properties have been fabricated. These sensors can be used under both low and high temperatures, featuring the ability to catch water from the environment to enhance conductivity. This work shows promise for the fabrication of high-performance sensing material with multi-functional sensing and synergistic properties.

POLYMER (2021)

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Article Multidisciplinary Sciences

The atomistic details of the ice recrystallisation inhibition activity of PVA

Fabienne Bachtiger et al.

Summary: Understanding ice recrystallisation is crucial for improving current cryopreservation technologies. The authors combine experiments and simulations to reveal the atomistic details of the ice recrystallization inhibition (IRI) activity of poly(vinyl)alcohol-the most potent biomimetic IRI agent.

NATURE COMMUNICATIONS (2021)

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Review Chemistry, Multidisciplinary

Ice Inhibition for Cryopreservation: Materials, Strategies, and Challenges

Tie Chang et al.

Summary: Cryopreservation technology is crucial in biomedical applications, but the formation, growth, and recrystallization of ice crystals pose major challenges. Anti-icing materials and strategies can effectively reduce ice damage and enhance efficiency, including chemical ice-inhibition molecules, advanced engineering strategies, and external physical field technologies. Addressing current challenges and future perspectives in ice inhibition is essential for high-efficiency cryopreservation.

ADVANCED SCIENCE (2021)

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Flexible Antifreeze Zn-Ion Hybrid Supercapacitor Based on Gel Electrolyte with Graphene Electrodes

Jianghe Liu et al.

Summary: The gel electrolyte based on the PVA/Zn/ethylene glycol system shows high ionic conductivity and excellent antifreezing performance. The antifreezing Zn-ion hybrid supercapacitor fabricated with this gel electrolyte exhibits outstanding electrochemical properties and cyclic stability, even under low temperatures, demonstrating its potential for flexible energy storage devices in subzero-temperature environments.

ACS APPLIED MATERIALS & INTERFACES (2021)

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Article Nanoscience & Nanotechnology

Wearable Antifreezing Fiber-Shaped Zn/PANI Batteries with Suppressed Zn Dendrites and Operation in Sweat Electrolytes

Zifeng Cong et al.

Summary: A study introduced an antifreeze, long-life, and dendrite-free fiber-shaped Zn battery that utilizes nanoporous Zn and polyaniline deposited on carbon nanofibers, achieving stable capacity and cycling performance, and maintaining excellent performance even at low temperatures with the addition of an antifreeze agent.

ACS APPLIED MATERIALS & INTERFACES (2021)

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Article Chemistry, Multidisciplinary

Multifunctional Ionic Skin with Sensing, UV-Filtering, Water-Retaining, and Anti-Freezing Capabilities

Jie Wen et al.

Summary: The conductive polymer hydrogel achieved transparent and highly ionically conductive properties through the organic combination of tannic acid-coated hydroxyapatite nanowires (TA@HAP NWs), polyvinyl alcohol (PVA) chains, ethylene glycol (EG), and metal ions. It integrates sensing, UV-filtering, water-retaining, and anti-freezing performances, and provides new ideas for the design of novel ionic skin devices. The inclusion of nanowires improves mechanical properties and UV-shielding ability, while the water-locking effect between EG and water molecules allows the hydrogel to exhibit freezing resistance and moisture retention.

ADVANCED FUNCTIONAL MATERIALS (2021)

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Article Chemistry, Multidisciplinary

Environment Tolerant Conductive Nanocomposite Organohydrogels as Flexible Strain Sensors and Power Sources for Sustainable Electronics

Hongling Sun et al.

Summary: This study demonstrates an environment-tolerant and ultrastretchable organohydrogel through a simple solvent-replacement strategy, achieving excellent temperature tolerance while maintaining stability and conductivity. Experimental results show that, without sacrificing stretchability and conductivity, the organohydrogel is capable of effectively detecting and discriminating human activities in extreme conditions.

ADVANCED FUNCTIONAL MATERIALS (2021)

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Article Chemistry, Multidisciplinary

Ionic Conductive Organohydrogels with Dynamic Pattern Behavior and Multi-Environmental Stability

Jing Liu et al.

Summary: The study prepared an organic hydrogel that shows obvious transparent changes in different solvents and can be used as a dynamic information storage device. It exhibits outstanding freezing resistance and moisturizing properties, and displays stable mechanical sensing performance in various environments.

ADVANCED FUNCTIONAL MATERIALS (2021)

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Article Chemistry, Multidisciplinary

Full-Temperature All-Solid-State Ti3C2Tx/Aramid Fiber Supercapacitor with Optimal Balance of Capacitive Performance and Flexibility

Qi Liu et al.

Summary: This study presents a full-temperature all-solid-state symmetrical flexible fiber supercapacitor with high performance in terms of capacitance and flexibility. The assembled device shows excellent capacitance retention and energy density, as well as good flexibility and electrochemical performance over a wide temperature range.

ADVANCED FUNCTIONAL MATERIALS (2021)

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Review Chemistry, Multidisciplinary

Recent Progress in Flexible Tactile Sensors for Human-Interactive Systems: From Sensors to Advanced Applications

Soonjae Pyo et al.

Summary: This article summarizes important advances in flexible tactile sensors in recent years, including sensor designs and material configurations to improve key performance parameters such as sensitivity, detection range/linearity, response time/hysteresis, spatial resolution/crosstalk, multidirectional force detection, and insensitivity to other stimuli.

ADVANCED MATERIALS (2021)

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Review Biology

Winter is coming: the future of cryopreservation

Sanja Bojic et al.

Summary: The article reviews the widespread use of cryopreservation in biomedicine, discusses the main challenges in organ transplantation, analyzes the advantages and disadvantages of current methods, and outlines the prospects for future development in the field.

BMC BIOLOGY (2021)

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Article Chemistry, Physical

Anti-freezing organohydrogel triboelectric nanogenerator toward highly efficient and flexible human-machine interaction at-30 °C

Zhenyu Xu et al.

Summary: This study developed anti-freezing organohydrogels with excellent properties at -30 degrees C, which were used to create a flexible keyboard for human-machine interaction.

NANO ENERGY (2021)

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Article Entomology

First instar nymphs of two peltoperlid stoneflies (Insecta, Plecoptera, Peltoperlidae)

Shodo Mtow et al.

Summary: The first instar nymphs of two peltoperlid stoneflies were examined and described, revealing differences in body shape and distribution of chloride cells, which may have arisen from different evolutionary pathways and heterochrony.

DEUTSCHE ENTOMOLOGISCHE ZEITSCHRIFT (2021)

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Article Engineering, Chemical

Highly Elastic Anti-fatigue and Anti-freezing Conductive Double Network Hydrogel for Human Body Sensors

Shaoxian Chen et al.

Summary: A novel hydrogel with excellent mechanical properties and high electrical conductivity was successfully synthesized in this study, showing good elasticity, fatigue resistance, and low-temperature resistance. This hydrogel can be used to prepare wearable sensors with high sensitivity and repeatability for accurate monitoring of various human body movements.

INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH (2021)

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Article Biochemistry & Molecular Biology

Discovery of Hyperactive Antifreeze Protein from Phylogenetically Distant Beetles Questions Its Evolutionary Origin

Tatsuya Arai et al.

Summary: The study found that the popular stag beetle synthesizes multiple isoforms of hyperactive antifreeze protein, which helps the beetle survive extreme freezing conditions. The DNA sequences of the beetle are highly similar to those of other hyperactive antifreeze proteins, suggesting a potential unrevealed gene transfer mechanism.

INTERNATIONAL JOURNAL OF MOLECULAR SCIENCES (2021)

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Article Multidisciplinary Sciences

Sea urchin-like microstructure pressure sensors with an ultra-broad range and high sensitivity

Xiu-man Wang et al.

Summary: Researchers have proposed a new design for pressure sensors based on a ternary nanocomposite material, showing high sensitivity, fast response, and wide pressure range. The sensor has broad application prospects in wearable electronics and health monitoring.

NATURE COMMUNICATIONS (2021)

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Article Multidisciplinary Sciences

Imperceptible energy harvesting device and biomedical sensor based on ultraflexible ferroelectric transducers and organic diodes

Andreas Petritz et al.

Summary: This study introduces ultraflexible ferroelectric polymer transducers and organic diodes for imperceptible sensing and energy harvesting, showing enhanced sensitivity and excellent flexibility when integrated on ultrathin substrates. These technologies enable the development of imperceptible wireless e-health patches with improved sensitivity, fast response, and mechanical stability for precise monitoring of vital parameters. Additionally, combining transducers with rectifiers based on ultraflexible organic diodes results in a thin and efficient energy harvesting device with great potential for self-powering e-health systems.

NATURE COMMUNICATIONS (2021)

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Article Chemistry, Physical

Environment-resisted flexible high performance triboelectric nanogenerators based on ultrafast self-healing non-drying conductive organohydrogel

Long-Biao Huang et al.

Summary: A hydrophobic, icephobic, and ultrafast self-healing TENG has been developed for energy harvesting and self-powered sensor applications in harsh environments, showing better electrical output stability and rapid recovery capabilities.

NANO ENERGY (2021)

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Article Energy & Fuels

Ampere-hour-scale zinc-air pouch cells

Sambhaji S. Shinde et al.

Summary: Researchers report a cell-level design for all-solid-state zinc-air pouch cells with exceptionally high energy density and cycle lifespan.

NATURE ENERGY (2021)

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Article Multidisciplinary Sciences

Bioinspired tough gel sheath for robust and versatile surface functionalization

Zhenwei Ma et al.

Summary: This study presents a versatile strategy for functionalizing fiber-based devices such as sutures, enhancing their interfacial adhesion strength, reducing surface stiffness, friction, and drag when interfacing with tissues, while maintaining tensile strength. The technology enables versatile functionalization for infection prevention, wound monitoring, drug delivery, and near-infrared imaging. This platform technology has the potential to impact a wide range of technological areas, from wound management to smart textiles.

SCIENCE ADVANCES (2021)

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Article Nanoscience & Nanotechnology

Bioinspired Color-Changing Photonic Polymer Coatings Based on Three-Dimensional Blue Phase Liquid Crystal Networks

Yanzhao Yang et al.

Summary: This study presents the fabrication of humidity-driven color-changing photonic polymer coatings based on hydrogen-bonded three-dimensional blue phase liquid crystal networks, demonstrating their versatility in applications such as optical sensors, information encryption, adaptive camouflage, and humidity sensors. The research provides new insights into the development of stimuli-responsive advanced functional materials with customizable 3D photonic nanostructures for a wide range of technological applications.

ACS APPLIED MATERIALS & INTERFACES (2021)

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Review Chemistry, Multidisciplinary

Nanocellulose-Based Functional Materials: From Chiral Photonics to Soft Actuator and Energy Storage

Pengfei Lv et al.

Summary: Nanocellulose has attracted extensive research attention due to its renewable, carbon-neutral nature, superior biocompatibility, tailorable surface chemistry, and optical and mechanical properties. Recent advancements in nanocellulose-derived functional materials and their applications in areas such as chiral photonics, soft actuators, energy storage, and biomedical science have been highlighted in this review. Discussion on the design and synthesis strategies, unique properties, underlying mechanisms, and potential applications of nanocellulose-based functional materials provides insights for the rapid development of interdisciplinary fields.

ADVANCED FUNCTIONAL MATERIALS (2021)

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Article Chemistry, Multidisciplinary

An Anti-freezing, Ambient-Stable and Highly Stretchable Ionic Skin with Strong Surface Adhesion for Wearable Sensing and Soft Robotics

Binbin Ying et al.

Summary: The novel iSkin hydrogel-based ionic skin demonstrates high toughness, high stretchability, excellent anti-freezing capability, and strong surface adhesion, making it suitable for wearable sensing and soft robotics with good conductivity and environmental adaptability.

ADVANCED FUNCTIONAL MATERIALS (2021)

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Article Chemistry, Multidisciplinary

A Flexible Multifunctional Triboelectric Nanogenerator Based on MXene/PVA Hydrogel

Xiongxin Luo et al.

Summary: The MXene/polyvinyl alcohol (PVA) hydrogel TENG (MH-TENG) showcases simple fabrication, high output performance, and versatile applications. MXene nanosheets doping enhances the crosslinking of the PVA hydrogel, improving its stretchability.

ADVANCED FUNCTIONAL MATERIALS (2021)

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Article Chemistry, Multidisciplinary

A General Crosslinker Strategy to Realize Intrinsic Frozen Resistance of Hydrogels

Dong Zhang et al.

Summary: The study introduces a novel crosslinking strategy to fabricate a series of antifreezing hydrogels with strong antifreezing and mechanical properties in various environments. The hydrogels are proposed to have a general antifreezing property regardless of their network compositions.

ADVANCED MATERIALS (2021)

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Article Engineering, Multidisciplinary

Lignin sulfonate induced ultrafast polymerization of double network hydrogels with anti-freezing, high strength and conductivity and their sensing applications at extremely cold conditions

Yang Zhang et al.

Summary: The study successfully synthesized a double network hydrogel, which showed improved mechanical properties and conductivity with the addition of lithium chloride, maintaining outstanding performance at extremely low temperatures.

COMPOSITES PART B-ENGINEERING (2021)

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Article Chemistry, Physical

Anti-freezing, moisturizing, resilient and conductive organohydrogel for sensitive pressure sensors

Wenhui Zheng et al.

Summary: Conductive hydrogels with anti-freezing and moisturizing capabilities were developed, showing excellent performance and potential applications in extreme environments.

JOURNAL OF COLLOID AND INTERFACE SCIENCE (2021)

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Article Multidisciplinary Sciences

Self-rechargeable cardiac pacemaker system with triboelectric nanogenerators

Hanjun Ryu et al.

Summary: Self-powered implantable devices have the potential to extend device operation time, but current energy harvesters are insufficient and inconvenient. The authors report on a commercial coin battery-sized high-performance inertia-driven triboelectric nanogenerator based on body motion and gravity, which can be used to charge a lithium-ion battery and integrated into a cardiac pacemaker.

NATURE COMMUNICATIONS (2021)

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Article Multidisciplinary Sciences

Skin-like mechanoresponsive self-healing ionic elastomer from supramolecular zwitterionic network

Wei Zhang et al.

Summary: The stretchable ionic elastomer demonstrated in the study exhibits high stretchability, immense strain-stiffening, good self-healing ability, excellent elasticity, high transparency, anti-freezing properties, water reprocessibility, and easy-to-peel adhesion, making it very promising for use in wearable electronic sensors for human-machine interfacing.

NATURE COMMUNICATIONS (2021)

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Article Multidisciplinary Sciences

Living fabrication of functional semi-interpenetrating polymeric materials

Zhuojun Dai et al.

Summary: Cell-mediated living fabrication has the potential to create materials with versatile, programmable functions. In this study, living materials consisting of semi-interpenetrating polymer networks were engineered using bacteria encapsulated in polymeric microcapsules. These materials enhance mechanical properties and anchor effector proteins for diverse applications.

NATURE COMMUNICATIONS (2021)

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Article Multidisciplinary Sciences

Biomimetic chameleon soft robot with artificial crypsis and disruptive coloration skin

Hyeonseok Kim et al.

Summary: The research successfully develops a next-generation artificial camouflage device with high resolution and real-time adaptation to the surrounding environment by integrating thermochromic liquid crystal layer and silver nanowire heaters in a multilayer structure with an active control system.

NATURE COMMUNICATIONS (2021)

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Review Chemistry, Physical

Multi-Functional Hydrogels for Flexible Zinc-Based Batteries Working under Extreme Conditions

Siyuan Zhao et al.

Summary: Zinc-based batteries with hydrogel electrolytes are promising for flexible energy storage due to their high capacity, low cost, and safety features. However, research on these batteries under extreme conditions is still in the early stages, with many technical issues remaining to be addressed. Design strategies for hydrogel electrolytes suitable for use in all extreme conditions are proposed, along with a discussion on the challenges and future directions of hydrogel electrolytes for zinc-based batteries.

ADVANCED ENERGY MATERIALS (2021)

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Article Chemistry, Multidisciplinary

Highly Stretchable, Self-Healable, Freezing-Tolerant, and Transparent Polyacrylic Acid/Nanochitin Composite Hydrogel for Self-Powered Multifunctional Sensors

Xin Jing et al.

Summary: A polyacrylic acid/nanochitin composite hydrogel with dual cross-linking networks was synthesized to fabricate highly stretchable, transparent, self-healing, and anti-freezing sensors. The sensors showed high sensitivity and could detect multiple external stimuli, operating within a broad temperature range.

ACS SUSTAINABLE CHEMISTRY & ENGINEERING (2021)

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Article Materials Science, Multidisciplinary

3D printed super-anti-freezing self-adhesive human-machine interface

Lei Chen et al.

Summary: The 3D printed hydrogel has excellent stretchability, adhesive behavior, and anti-freezing ability, making it suitable for sensors, self-adhesive electrodes, and other applications, especially performing well in extreme low temperatures.

MATERIALS TODAY PHYSICS (2021)

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Article Multidisciplinary Sciences

Tendon-inspired anti-freezing tough gels

Sidi Duan et al.

Summary: Researchers have developed a method to strengthen polyvinyl alcohol hydrogels inspired by tendons and coniferous trees, enhancing their mechanical properties and freeze resistance. This versatile material has broad applications, such as in manufacturing hydraulic actuators and ionic conductors.

ISCIENCE (2021)

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Article Chemistry, Physical

Rapid and scalable fabrication of ultra-stretchable, anti-freezing conductive gels by cononsolvency effect

Shuwang Wu et al.

Summary: A rapid fabrication strategy was proposed to produce anti-freezing conductive gels in minutes using a water/DMSO binary liquid system. The gel showed excellent mechanical properties and high ionic conductivity at temperatures lower than -50 degrees C, outperforming previous reports. An all-in-one supercapacitor was fabricated to demonstrate the potential of the anti-freezing gel in soft device applications at subzero temperatures, with full recyclability of the material demonstrated.

ECOMAT (2021)

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Review Chemistry, Multidisciplinary

Gels as emerging anti-icing materials: a mini review

Yizhi Zhuo et al.

Summary: Although current anti-icing gels are still in their infancy, their outstanding icephobicity has sparked the emergence of a new group of anti-icing materials, highlighting the need for timely review to drive development towards dedicated applications.

MATERIALS HORIZONS (2021)

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Article Chemistry, Physical

Bioinspired, nucleobase-driven, highly resilient, and fast-responsive antifreeze ionic conductive hydrogels for durable pressure and strain sensors

Xiang Di et al.

Summary: This study fabricated a novel ionic conductive hydrogel with a unique structure, showing excellent stretchability, resilience, sensitivity, and fast strain responsiveness, which can be applied in detecting various daily activities.

JOURNAL OF MATERIALS CHEMISTRY A (2021)

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Article Materials Science, Multidisciplinary

Freezing-tolerant, widely detectable and ultra-sensitive composite organohydrogel for multiple sensing applications

Zhihui Xie et al.

Summary: The research team developed a polydopamine-reduced graphene oxide/sodium alginate/polyacrylamide composite organohydrogel sensor with dual crosslinking networks, which exhibits excellent conductivity and high sensitivity for efficient sensing within a broad strain and temperature range.

JOURNAL OF MATERIALS CHEMISTRY C (2021)

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Article Chemistry, Multidisciplinary

Stimulus-driven liquid metal and liquid crystal network actuators for programmable soft robotics

Pengfei Lv et al.

Summary: A general strategy to integrate electrically conductive liquid metals and shape-morphing liquid crystal networks towards multifunctional and programmable soft robotics is proposed in this study.

MATERIALS HORIZONS (2021)

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Article Chemistry, Physical

Ultrafast fabrication of organohydrogels with UV-blocking, anti-freezing, anti-drying, and skin epidermal sensing properties using lignin-Cu2+ plant catechol chemistry

Dan Sun et al.

Summary: A self-catalytic system using sodium lignosulfonate and copper(ii) ions was developed for rapid fabrication of organohydrogels with multifunctional properties. These materials exhibit UV-blocking and electrically conductive properties, and show anti-freezing and anti-drying abilities due to the presence of glycerol, making them suitable for use as epidermal sensors.

JOURNAL OF MATERIALS CHEMISTRY A (2021)

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Article Chemistry, Multidisciplinary

Stretchable supercapacitor at-30 °C

Xuting Jin et al.

Summary: A highly stretchable and anti-freezing supercapacitor was fabricated without the need for extra stretchable substrates or predefining stretchable structures. It showed high mechanical stretchability, impressive capacitance retention at low temperatures, and an ultralong lifespan, making it an ideal power source for driving multi-functional electronic components.

ENERGY & ENVIRONMENTAL SCIENCE (2021)

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Article Chemistry, Physical

A transparent glycerol-hydrogel with stimuli-responsive actuation induced unexpectedly at subzero temperatures

Meiling Guo et al.

Summary: The study demonstrates a glycerol-hydrogel with outstanding programmable shape memory capabilities, showing excellent transparency and anti-freezing performance at subzero temperatures. This provides a new direction for designing more advanced hydrogel-based devices.

JOURNAL OF MATERIALS CHEMISTRY A (2021)

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Article Materials Science, Multidisciplinary

A Dual-Responsive, Freezing-Tolerant Hydrogel Sensor and Related Thermal- and Strain-Sensitive Mechanisms

Yonggan Yan et al.

Summary: A freezing-tolerant, dual-responsive hydrogel sensor was developed in this study, capable of efficiently detecting different temperature ranges and strains. It was found that the resistance of the hydrogel increased as temperature decreased, and the strain sensitivity increased as temperature decreased.

ACS APPLIED POLYMER MATERIALS (2021)

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Review Chemistry, Multidisciplinary

Light-driven bimorph soft actuators: design, fabrication, and properties

Yuanhao Chen et al.

Summary: Soft robots that mimic living organisms and can adapt to their environment are gaining attention due to advances in material flexibility, human-friendly interaction, and biological adaptation. Light-driven actuators based on responsive soft materials are seen as promising for untethered soft robotics, with researchers focusing on photomechanics, photoswitching, bioinspired design, and actuation realization. This review discusses recent advances in light-driven bimorph soft actuators, highlighting the integration of photoactive and passive layers to endow soft actuators with new features like sensitivity, programmability, compatibility, robustness, and controllability.

MATERIALS HORIZONS (2021)

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Article Materials Science, Multidisciplinary

Molecular mechanisms of cell cryopreservation with polyampholytes studied by solid-state NMR

Kazuaki Matsumura et al.

Summary: Cellular cryopreservation is a crucial technique in modern biology, and the molecular mechanisms of polyampholyte cryoprotectants have been investigated using solid-state NMR. Findings suggest that polyampholytes reduce cell stress by preventing intracellular ice formation and osmotic shock, thus providing cryoprotection.

COMMUNICATIONS MATERIALS (2021)

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Article Chemistry, Physical

Fruit-battery-inspired self-powered stretchable hydrogel-based ionic skin that works effectively in extreme environments

Qinhua Wang et al.

Summary: Self-powered sensors using hydrogels have been developed with high stretchability, skin-like Young's modulus, good electrical conductivity, and other properties. A novel self-powered strain sensing mechanism based on hydrogels was proposed, allowing for responses to pressure and strain signals without external power supply. The self-powered ionic skin assembled from hydrogel sensor units achieved a maximum output voltage of approximately 4.4 V, providing emergency power for small equipment in extreme environments.

JOURNAL OF MATERIALS CHEMISTRY A (2021)

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Article Materials Science, Multidisciplinary

Fully-physically crosslinked silk fibroin/poly(hydroxyethyl acrylamide) hydrogel with high transparency and adhesive properties for wireless sensing and low-temperature strain sensing

Xia Sun et al.

Summary: A hydrogel with excellent mechanical properties, high sensitivity and large sensing range was successfully prepared in this study, making it suitable for strain sensors that can monitor human movements in various situations at both room temperature and low temperature. This indicates its huge potential in flexible electronics, remote health control, and electronic skins.

JOURNAL OF MATERIALS CHEMISTRY C (2021)

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Article Materials Science, Multidisciplinary

Adaptable ionic liquid-containing supramolecular hydrogel with multiple sensations at subzero temperatures

Bo Li et al.

Summary: This study demonstrates a supramolecular ionic liquid hydrogel with excellent mechanical and thermal sensitivity at subzero temperatures, which is utilized for fabricating E-skin for intelligent robots to achieve pressure feedback and thermal recognition. This line of research not only shows the potential of anti-freezing stimuli-responsive hydrogels for E-skin applications in harsh conditions, but also contributes to the design and application of supramolecular polymer-based hydrogel sensors for future artificial intelligence applications.

JOURNAL OF MATERIALS CHEMISTRY C (2021)

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Review Electrochemistry

Zinc Metal Energy Storage Devices under Extreme Conditions of Low Temperatures

Fuyun Li et al.

Summary: Zinc-based energy storage devices face challenges under extreme low temperature conditions, such as electrolyte freezing and sluggish electrode kinetics. In recent years, considerable research efforts have been devoted to addressing these issues.

BATTERIES & SUPERCAPS (2021)

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Article Materials Science, Multidisciplinary

Studies on de-icing and anti-icing of carbon fiber-reinforced composites for aircraft surfaces using commercial multifunctional permanent superhydrophobic coatings

A. Khadak et al.

Summary: The accumulation of ice on structures can pose challenges in various industries, but the use of superhydrophobic coatings on carbon fiber-reinforced composites has been proven to provide a permanent and effective solution for de-icing and anti-icing properties, ensuring longer service life in aerospace, wind turbines, and other applications.

JOURNAL OF MATERIALS SCIENCE (2021)

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Review Chemistry, Multidisciplinary

Biomimetic anti-freezing polymeric hydrogels: keeping soft-wet materials active in cold environments

Yukun Jian et al.

Summary: Hydrogels, as outstanding materials, have been extensively studied for various fields of application, but their properties are compromised at sub-zero temperatures. Lowering the liquid-solid phase transition temperature is crucial for expanding their applications. Research on anti-freezing hydrogels mainly focuses on additives, polymer network modification, and future developments hold promising research directions.

MATERIALS HORIZONS (2021)

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Review Chemistry, Multidisciplinary

Nature-Inspired Emerging Chiral Liquid Crystal Nanostructures: From Molecular Self-Assembly to DNA Mesophase and Nanocolloids

Ling Wang et al.

ADVANCED MATERIALS (2020)

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Review Chemistry, Multidisciplinary

Advanced Soft Materials, Sensor Integrations, and Applications of Wearable Flexible Hybrid Electronics in Healthcare, Energy, and Environment

Hyo-Ryoung Lim et al.

ADVANCED MATERIALS (2020)

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Article Biochemistry & Molecular Biology

Polyampholytes as Emerging Macromolecular Cryoprotectants

Christopher Stubbs et al.

BIOMACROMOLECULES (2020)

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Review Chemistry, Multidisciplinary

Ionic Tactile Sensors for Emerging Human-Interactive Technologies: A Review of Recent Progress

Vipin Amoli et al.

ADVANCED FUNCTIONAL MATERIALS (2020)

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Review Chemistry, Multidisciplinary

Bioinspired Multiscale Wet Adhesive Surfaces: Structures and Controlled Adhesion

Yupeng Chen et al.

ADVANCED FUNCTIONAL MATERIALS (2020)

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Article Chemistry, Multidisciplinary

Antifreezing Hydrogel with High Zinc Reversibility for Flexible and Durable Aqueous Batteries by Cooperative Hydrated Cations

Minshen Zhu et al.

ADVANCED FUNCTIONAL MATERIALS (2020)

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Article Nanoscience & Nanotechnology

Hydrophobic Ionic Liquid Gel-Based Triboelectric Nanogenerator: Next Generation of Ultrastable, Flexible, and Transparent Power Sources for Sustainable Electronics

Pinlei Lv et al.

ACS APPLIED MATERIALS & INTERFACES (2020)

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Article Nanoscience & Nanotechnology

Alkaline Double-Network Hydrogels with High Conductivities, Superior Mechanical Performances, and Antifreezing Properties for Solid-State Zinc-Air Batteries

Na Sun et al.

ACS APPLIED MATERIALS & INTERFACES (2020)

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Article Nanoscience & Nanotechnology

Robust Physically Linked Double-Network Ionogel as a Flexible Bimodal Sensor

Jingxian Sun et al.

ACS APPLIED MATERIALS & INTERFACES (2020)

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Article Chemistry, Multidisciplinary

Zwitterionic Osmolyte-Based Hydrogels with Antifreezing Property, High Conductivity, and Stable Flexibility at Subzero Temperature

Xiaojie Sui et al.

ADVANCED FUNCTIONAL MATERIALS (2020)

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Article Chemistry, Multidisciplinary

Hydrogen-Free and Dendrite-Free All-Solid-State Zn-Ion Batteries

Longtao Ma et al.

ADVANCED MATERIALS (2020)

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Article Chemistry, Multidisciplinary

Near-Infrared Photodriven Self-Sustained Oscillation of Liquid-Crystalline Network Film with Predesignated Polydopamine Coating

Ruochen Lan et al.

ADVANCED MATERIALS (2020)

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Article Biochemistry & Molecular Biology

Trehalose-Based Polyethers for Cryopreservation and Three-Dimensional Cell Scaffolds

Diana Diaz-Dussan et al.

BIOMACROMOLECULES (2020)

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Article Chemistry, Physical

Autonomous Self-Healing, Antifreezing, and Transparent Conductive Elastomers

Ren'ai Li et al.

CHEMISTRY OF MATERIALS (2020)

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Article Biology

Porcine heart valve, aorta and trachea cryopreservation and thawing using polydimethylsiloxane

Stanislav E. Lauk-Dubitskiy et al.

CRYOBIOLOGY (2020)

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Article Polymer Science

Reversibly highly stretchable and self-healable zwitterion-containing polyelectrolyte hydrogel with high ionic conductivity for high-performance flexible and cold-resistant supercapacitor

Wenjing Diao et al.

JOURNAL OF APPLIED POLYMER SCIENCE (2020)

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Review Chemistry, Physical

Recent Advances in Polymer Electrolytes for Zinc Ion Batteries: Mechanisms, Properties, and Perspectives

Kai Wu et al.

ADVANCED ENERGY MATERIALS (2020)

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Article Nanoscience & Nanotechnology

Physically Cross-Linked Silk Fibroin-Based Tough Hydrogel Electrolyte with Exceptional Water Retention and Freezing Tolerance

Wenqi Wang et al.

ACS APPLIED MATERIALS & INTERFACES (2020)

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Article Nanoscience & Nanotechnology

Freezing-Tolerant, Highly Sensitive Strain and Pressure Sensors Assembled from Ionic Conductive Hydrogels with Dynamic Cross-Links

Hongyan Liu et al.

ACS APPLIED MATERIALS & INTERFACES (2020)

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Article Nanoscience & Nanotechnology

Enhancing the Performance of a Stretchable and Transparent Triboelectric Nanogenerator by Optimizing the Hydrogel Ionic Electrode Property

Xin Jing et al.

ACS APPLIED MATERIALS & INTERFACES (2020)

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Article Chemistry, Multidisciplinary

Mussel-Inspired Hydrogels for Self-Adhesive Bioelectronics

Chaoming Xie et al.

ADVANCED FUNCTIONAL MATERIALS (2020)

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Article Materials Science, Biomaterials

Novel Nonreleasing Antibacterial Hydrogel Dressing by a One-Pot Method

Kang Wang et al.

ACS BIOMATERIALS SCIENCE & ENGINEERING (2020)

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Article Multidisciplinary Sciences

Universally autonomous self-healing elastomer with high stretchability

Hongshuang Guo et al.

NATURE COMMUNICATIONS (2020)

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Article Multidisciplinary Sciences

Effects of xylem embolism on the winter survival of Abies veitchii shoots in an upper subalpine region of central Japan

Emiko Maruta et al.

SCIENTIFIC REPORTS (2020)

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Article Chemistry, Multidisciplinary

Physical Organohydrogels With Extreme Strength and Temperature Tolerance

Jing Wen Zhang et al.

FRONTIERS IN CHEMISTRY (2020)

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Article Biochemical Research Methods

Subzero non-frozen preservation of human livers in the supercooled state

Reinier J. de Vries et al.

NATURE PROTOCOLS (2020)

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Article Robotics

Biofuel-powered soft electronic skin with multiplexed and wireless sensing for human-machine interfaces

You Yu et al.

SCIENCE ROBOTICS (2020)

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Article Nanoscience & Nanotechnology

An Antifreezing/Antiheating Hydrogel Containing Catechol Derivative Urushiol for Strong Wet Adhesion to Various Substrates

Xianmou Fan et al.

ACS APPLIED MATERIALS & INTERFACES (2020)

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Article Nanoscience & Nanotechnology

Transparent Stretchable Dual-Network Ionogel with Temperature Tolerance for High-Performance Flexible Strain Sensors

Ji Lan et al.

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Physical hydrogels composed of polyampholytes demonstrate high toughness and viscoelasticity

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Highly sensitive flexible pressure sensors with microstructured rubber dielectric layers

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Effects of trehalose-loaded liposomes on red blood cell response to freezing and post-thaw membrane quality

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Cold tolerance and trehalose accumulation in overwintering larvae of the codling moth, Cydia pomonella (Lepidoptera: Tortricidae)

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Review Plant Sciences

Antifreeze proteins in overwintering plants: a tale of two activities

M Griffith et al.

TRENDS IN PLANT SCIENCE (2004)

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Article Hematology

Seven-day storage of apheresis platelets: report of an in vitro study

LJ Dumont et al.

TRANSFUSION (2003)

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Article Multidisciplinary Sciences

Molecular dynamics simulation of the ice nucleation and growth process leading to water freezing

M Matsumoto et al.

NATURE (2002)

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