期刊
SCIENCE OF THE TOTAL ENVIRONMENT
卷 830, 期 -, 页码 -出版社
ELSEVIER
DOI: 10.1016/j.scitotenv.2022.154712
关键词
Magnetization; Activated carbon; Adsorption; Denitrification; Nitrogen migration
资金
- Youth Natural Science Foundation of China [51904347]
- National Natural Science Foundation of China [52174329]
- Innovation-Driven Project of Guangxi Zhuang Autonomous Region [AA18242003]
In this study, a gas pre-magnetization and activated carbon adsorption process was developed to enhance the adsorption of NO onto activated carbon. The results showed that the external magnetic field could increase the removal rate and adsorption capacity of NO, and the gas pre-magnetization mechanism involved increasing the oxidation rate of NO and promoting the chemical reaction between NO and functional groups on the activated carbon.
The NO removal efficiency was relatively low in the traditional activated carbon adsorption process. In this work, a gas pre-magnetization and activated carbon adsorption process was developed to enhance the adsorption of NO onto activated carbon. In this innovative and green process, the mixed gas was magnetized in the external magnetic field and then absorbed by activated carbon. The results indicated that the maximal removal rate of NO could be increased from 75.0% to 89.5%, and the NO adsorption capacity of commercial activated carbon in one hour elevated from 2.28 to 2.60 mg/g when the magnetic induction intensity of external magnetic field increased from 0 T to 2 T. The strengthening mechanism of the gas pre-magnetization was investigated. It was found that magnetic field could elevate the oxidation rate of NO by 11.4% and thus promote the physical adsorption of NO onto activated carbon. External magnetic field could increase the reaction activity of NO and promote the chemical reaction between NO and some functional groups (CO, CO and COOH) on the activated carbon and thus promote the chemisorption process of NO.
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