4.8 Article

Structure of propagating high-stress fronts in a shear-thickening suspension

出版社

NATL ACAD SCIENCES
DOI: 10.1073/pnas.2203795119

关键词

shear thickening; rheology; fluid flow; jamming

资金

  1. NSF [DMR-1809890]
  2. Georgetown Interdisciplinary Chair in Science Fund

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We directly measured the stress at the boundary of a shear-thickening cornstarch suspension and found persistent regions of high local stress propagating in the flow direction. The structure of these propagating fronts was determined, including the profile of boundary stress and the nonaffine velocity of particles. We also measured the relative flow between the particle phase and the suspending fluid and found it to be highly localized to the fronts and changing direction across the front. These fronts are composed of a localized region of high dilatant pressure and low particle concentration.
We report direct measurements of spatially resolved stress at the boundary of a shear-thickening cornstarch suspension revealing persistent regions of high local stress propagating in the flow direction at the speed of the top boundary. The persistence of these propagating fronts enables precise measurements of their structure, including the profile of boundary stress measured by boundary stress microscopy (BSM) and the nonaffine velocity of particles at the bottom boundary of the suspension measured by particle image velocimetry (PIV). In addition, we directly measure the relative flow between the particle phase and the suspending fluid (fluid migration) and find the migration is highly localized to the fronts and changes direction across the front, indicating that the fronts are composed of a localized region of high dilatant pressure and low particle concentration. The magnitude of the flow indicates that the pore pressure difference driving the fluid migration is comparable to the critical shear stress for the onset of shear thickening. The propagating fronts fully account for the increase in viscosity with applied stress reported by the rheometer and are consistent with the existence of a stable jammed region in contact with one boundary of the system that generates a propagating network of percolated frictional contacts spanning the gap between the rheometer plates and producing strong localized dilatant pressure.

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