4.8 Article

Evidence of a room-temperature quantum spin Hall edge state in a higher-order topological insulator

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NATURE MATERIALS
卷 21, 期 10, 页码 1111-+

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NATURE PORTFOLIO
DOI: 10.1038/s41563-022-01304-3

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资金

  1. US Department of Energy, Office of Science, National Quantum Information Science Research Centers, Quantum Science Center
  2. Princeton University
  3. Gordon and Betty Moore Foundation [GBMF9461, GBMF4547]
  4. US DOE under the Basic Energy Sciences program [DOE/BES DE-FG-02-05ER46200]
  5. Princeton Center for Complex Materials, a National Science Foundation Materials Research Science and Engineering Center [DMR-2011750]
  6. DOE-BES [DE-SC0002613]
  7. National Science Foundation [DMR-1921581, DMR-1945351, DMR-2105139]
  8. Army Research Office [W911NF-18-1-0416]
  9. European Union's Horizon 2020 research and innovation programme [ERC-StG-Neupert-757867-PARATOP]
  10. Young Scholar Fellowship Program under a MOST grant for the Columbus Program [MOST111-2636-M-006-014]
  11. Higher Education Sprout Project, Ministry of Education
  12. National Key Research and Development Program of China [2020YFA0308800]
  13. National Science Foundation of China (NSFC) [92065109, 11734003, 12061131002]
  14. Strategic Priority Research Program of Chinese Academy of Sciences [XDB30000000, XDB28000000]
  15. CAS Interdisciplinary Innovation Team
  16. National Natural Science Foundation of China [12141002]
  17. National Center for Theoretical Sciences (Taiwan)

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This study provides micro-spectroscopic evidence for the presence of a room-temperature quantum spin Hall edge state on the surface of a higher-order topological insulator. The research reveals the microstructural features of the topological phase and suggests further exploration of high-temperature transport quantization.
Room-temperature realization of macroscopic quantum phases is one of the major pursuits in fundamental physics(1,2) . The quantum spin Hall phase(3-6) is a topological quantum phase that features a two-dimensional insulating bulk and a helical edge state. Here we use vector magnetic field and variable temperature based scanning tunnelling microscopy to provide micro-spectroscopic evidence for a room-temperature quantum spin Hall edge state on the surface of the higher-order topological insulator Bi4Br4. We find that the atomically resolved lattice exhibits a large insulating gap of over 200 meV, and an atomically sharp monolayer step edge hosts an in-gap gapless state, suggesting topological bulk-boundary correspondence. An external magnetic field can gap the edge state, consistent with the time-reversal symmetry protection inherent in the underlying band topology. We further identify the geometrical hybridization of such edge states, which not only supports the Z(2) topology of the quantum spin Hall state but also visualizes the building blocks of the higher-order topological insulator phase. Our results further encourage the exploration of high-temperature transport quantization of the putative topological phase reported here.

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