期刊
NANO RESEARCH
卷 15, 期 9, 页码 8524-8535出版社
TSINGHUA UNIV PRESS
DOI: 10.1007/s12274-022-4626-6
关键词
MXene; electromagnetic interference shielding; phase change composites; thermal energy management
类别
资金
- National Natural Science Foundation of China [U20A20299]
- Guangdong Special Support Program [2017TX04N371]
An innovative biomass/MXene-derived conductive hybrid scaffold was prepared in this study, leading to the development of phase change composites with excellent performance and potential for various applications. Among them, CKMPCC-6 showed high solar-thermal and electro-thermal conversion capabilities, making it a multifunctional material.
With the rapid development of new generations of miniaturized, integrated, and high-power electronic devices, it is particularly important to develop advanced composite materials with efficient thermal management capability and excellent electromagnetic interference (EMI) shielding performance. Herein, an innovative biomass/MXene-derived conductive hybrid scaffold, cellulose nanocrystal (CNC)-konjac glucomannan (KGM)/MXene (CKM), was prepared by freeze-drying and thermal annealing, and then paraffin wax (PW) was encapsulated in CKM using vacuum impregnation method to obtain CNC-KGM/MXene@PW phase change composites (CKMPCCs). The results show that the obtained CKMPCCs possess considerable reusable stabilities, excellent EMI shielding properties, and thermal energy management capacities. Among them, the CKMPCC-6 with 2.3 wt.% MXene exhibits excellent solar-thermal and electro-thermal conversion capabilities. In addition, the EMI shielding effectiveness value is as high as 45.0 dB at 8.2-12.4 GHz and the corresponding melting enthalpy value is 215.7 J/g (relative enthalpy efficiency of 99.9%). In conclusion, the synthesized multifunctional phase change composites provide great potential for integrating outstanding EMI shielding and advanced thermal energy management applications.
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