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Metal Halide Perovskites toward Electrically Pumped Lasers

LASER & PHOTONICS REVIEWS (2022)

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Summary: Perovskite light-emitting diodes (PeLEDs) have attracted considerable attention due to their unique optoelectronic properties, but their performance is limited by low quantum efficiency and unbalanced charge injection. In this study, a novel co-hole transport layer (HTL) was introduced to improve the performance of CsPbBr3-based PeLEDs through efficient energy transfer and enhanced charge transfer. The proposed dual transfer strategy is expected to revolutionize PeLED research.

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Summary: Quasi-2D perovskites composed of self-organized quantum well structures have shown promise as gain materials for laser applications. This study investigates the impact of domain distribution on the laser emission of CsPbCl1.5Br1.5-based quasi-2D perovskites. Through the use of 2,2-diphenylethylammonium bromide as a ligand, a quasi-2D film with a narrow domain distribution dominated by large-n domains is formed. This reduces the content of small-n domains and improves energy transfer. By controlling the domain distribution, blue amplified spontaneous emission and single-mode vertical-cavity surface-emitting lasing with low thresholds are achieved.

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Amplified Spontaneous Emission from Perovskite Quantum Dots Inside a Transparent Glass

Xiangling Tian et al.

Summary: The study reveals the optical gain characteristics of monodisperse CsPbBr3 quantum dots crystallized in transparent glass. By controlling the temperature, the threshold of amplified spontaneous emission can be changed with a high gain coefficient. The crystallized CsPbBr3 quantum dots in the transparent glass exhibit good stability with small fluctuations in lifetime and long photostability. These findings pave the way for the potential applications of CsPbBr3-based glass-ceramics in light sources and optical amplifiers.

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Summary: This research proposes an anti-solvent treatment strategy to regulate the phase components and surface morphology of quasi-2D perovskite films, and introduces an additional coating to reduce surface defects. Excellent amplified spontaneous emission and two-photon-pumped emission are achieved through these methods.

ADVANCED OPTICAL MATERIALS (2022)

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Enhanced Photoluminescence of Cesium Lead Halide Perovskites by Quasi-3D Photonic Crystals

Jose Mendoza Carreno et al.

Summary: The study introduced a quasi-3D photonic crystal to enhance the photoluminescence of cesium lead halide perovskite nanocrystals, demonstrating a significant improvement in light output by combining 2D gratings and DBRs.

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Ultrahigh Color Rendering in RGB Perovskite Micro-Light-Emitting Diode Arrays with Resonance-Enhanced Photon Recycling for Next Generation Displays

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Toward Continuous-Wave Pumped Metal Halide Perovskite Lasers: Strategies and Challenges

Feiyun Zhao et al.

Summary: This review discusses the challenges and opportunities in improving the performance and stability of continuous-wave (CW) pumped perovskite lasers. Potential strategies from material to device levels are examined, and future prospects are proposed.

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Xun Sun et al.

Summary: In this study, octahedral CsPbBr3 microcrystals were developed via a simple method, exhibiting single or dual-mode lasing under laser pulse excitation. Experimental results showed that the pump threshold varied significantly with microcrystal size, contrary to numerical simulations indicating larger crystals support higher quality factor eigenmodes. The developed CsPbBr3 octahedral microcrystals show potential for high-quality light emitters.

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Deep-Blue Perovskite Single-Mode Lasing through Efficient Vapor-Assisted Chlorination

Joao M. Pina et al.

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ADVANCED MATERIALS (2021)

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Dimensionality Control of Inorganic and Hybrid Perovskite Nanocrystals by Reaction Temperature: From No-Confinement to 3D and 1D Quantum Confinement

Clara Otero-Martinez et al.

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Solution-Processed Efficient Perovskite Nanocrystal Light-Emitting Device Utilizing Doped Hole Transport Layer

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Summary: The all-solution process for inorganic perovskite nanocrystals (PNCs) LEDs shows great potential for new-generation illumination and displays, but the challenge lies in the injection barriers and charge injection imbalance. The introduction of CBP into the hole transport layer (HTL) efficiently modulates the charge carrier mobility and energy level, resulting in barrier-free charge injection and optimal performance for solution-processed PNC LEDs. The luminance of red LEDs reaches 2990 cd m(-2) and the external quantum efficiency achieves 8.1%, with improved turn-on voltage and roll-off due to more balanced charge injection.

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Large-area periodic lead halide perovskite nanostructures for lenticular printing laser displays

Min Wang et al.

Summary: Lenticular printing technique utilizing hybrid perovskite materials can achieve optical modulation in both reflection and light emission, while improving the degree of polarization and directionality in laser actions. This enables the creation of prototype laser displays that vary emission colors at different view angles, potentially useful for high-resolution and high-contrast holographical images.

SCIENCE CHINA-CHEMISTRY (2021)

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Optical Gain of Lead Halide Perovskites Measured via the Variable Stripe Length Method: What We Can Learn and How to Avoid Pitfalls

Ada Lili Alvarado-Leanos et al.

Summary: This study outlines a meticulous analysis to retrieve the optical gain coefficient of MAPbI(3) using the VSL method, discussing experimental implementation and numerical treatment for a robust methodology. The results point to the role of electron-hole bimolecular recombination in dictating stimulated emission properties of MAPbI(3), resembling bulk GaAs behavior.

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Lead-Free Halide Perovskites for Light Emission: Recent Advances and Perspectives

Xin Li et al.

Summary: Lead-based halide perovskites have excellent properties for light-emitting applications but face challenges due to the toxic element lead, highlighting the urgency in developing lead-free alternatives. Recent advances focus on the synthesis, properties, and applications of lead-free halide perovskite materials, particularly in the field of optoelectronics.

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Metal Halide Perovskites for Laser Applications

Lei Lei et al.

Summary: Metal halide perovskites are gaining attention in optoelectronic applications due to their properties such as large absorption coefficient, low defect density, and high charge carrier mobility. While progress has been made in perovskite-based lasers, the development is still in its early stages and electrically pumped lasers have not been realized yet. Understanding the fundamental photophysical characteristics of perovskite gain materials is crucial to accelerating their development in laser applications.

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Ultralow-Threshold Continuous-Wave Room-Temperature Crystal-Fiber/Nanoperovskite Hybrid Lasers for All-Optical Photonic Integration

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Multicolor Random Lasers Based on Perovskite Quantum Dots Embedded in Intrinsic Pb-MOFs

Baoyuan Xu et al.

Summary: A new class of random lasers was proposed in this study by precipitating perovskite quantum dots in metal-organic frameworks. These random lasers leverage the high refractive index of MOFs and the high optical gain of PQDs to achieve high-density PQD gain in MOFs and demonstrate low-threshold multicolor random lasers.

JOURNAL OF PHYSICAL CHEMISTRY C (2021)

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Directional Lasing from Nanopatterned Halide Perovskite Nanowire

Alexey Yu Zhizhchenko et al.

Summary: Directional lasing from a single perovskite CsPbBr3 nanowire is achieved by imprinting a nanograting on its surface, resulting in stimulated emission outcoupling to its vertical direction and a decrease in the number of lasing modes with a 2-fold increase of the quality factor of the remaining modes. The high-throughput laser ablation method used for nanopatterning preserves the luminescent properties of the material, which are typically deteriorated after processing via conventional lithographic approaches.

NANO LETTERS (2021)

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Perovskite solar cells with atomically coherent interlayers on SnO2 electrodes

Hanul Min et al.

Summary: By introducing an interlayer between the electron-transporting and perovskite layers in perovskite solar cells, researchers have successfully enhanced charge extraction and transport from the perovskite, leading to higher power conversion efficiency and fewer interfacial defects. The coherent interlayer allowed the fabrication of devices with a certified efficiency of 25.5%, which maintained about 90% of its initial efficiency even after continuous light exposure for 500 hours. The findings provide guidelines for designing defect-minimizing interfaces in metal halide perovskites and electron-transporting layers.

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Zhizai Li et al.

Summary: X-ray detection has been widely utilized in various fields, and halide perovskites as alternative materials show great potential in high-performance X-ray detectors. Through advanced research and optimization strategies, the performance of X-ray detectors based on halide perovskites has reached a comparative height.

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Summary: By utilizing multidentate ligands to treat mixed-halide perovskite nanocrystals, efficient and color-stable red electroluminescence with a wavelength centered at 620 nanometers and an external quantum efficiency of 20.3% has been achieved. The key function of the ligand treatment is to 'clean' the nanocrystal surface by removing lead atoms, which suppresses the formation of iodine Frenkel defects and halide segregation. This work demonstrates the sensitivity of metal halide perovskites to surface properties and provides a pathway to control surface defect formation and migration, crucial for achieving bandgap stability for light emission and potentially impacting other optoelectronic applications.

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Single-Step Microfluidic Synthesis of Halide Perovskite Nanolasers in Suspension

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Tuning of Amplified Spontaneous Emission Wavelength for Green and Blue Light Emission through the Tunable Composition of CsPb(Br1-xClx)3 Inorganic Perovskite Quantum Dots

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NATURE (2021)

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A general approach to high-efficiency perovskite solar cells by any antisolvent

Alexander D. Taylor et al.

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Continuous-Wave Vertical Cavity Surface-Emitting Lasers based on Single Crystalline Lead Halide Perovskites

Hongbo Zhang et al.

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ADVANCED OPTICAL MATERIALS (2021)

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Review Nanoscience & Nanotechnology

Quasi-2D lead halide perovskite gain materials toward electrical pumping laser

Chenyang Zhao et al.

Summary: Quasi two-dimensional lead halide perovskite materials exhibit excellent performance in photoelectric devices, with high exciton utilization and low threshold characteristics due to their structural flexibility and quantum-well structures. Additionally, the hydrophobic bulky organic cations contribute to improved stability.

NANOPHOTONICS (2021)

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Editorial Material Multidisciplinary Sciences

Continuous-wave lasing from quasi-2D perovskites

Xian Chen et al.

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Haiyun Dong et al.

Summary: The development of a micro-origami technique enables the design of 3D perovskite microarchitectures for a new type of microcavity laser, which exhibits outstanding laser performance and new functionalities such as 3D confined mode lasing and directional emission. This represents a significant advancement towards programmable microarchitectures in perovskite optoelectronics and photonics in the 3D era.

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Perovskite Light-Emitting Diodes with EQE Exceeding 28% through a Synergetic Dual-Additive Strategy for Defect Passivation and Nanostructure Regulation

Zhe Liu et al.

Summary: A synergetic dual-additive strategy was used to prepare perovskite films with low defect density and high environmental stability, leading to the formation of perovskite nanocrystals with a quasi-core/shell structure that exhibited improved stability and efficiency in green PeLEDs.

ADVANCED MATERIALS (2021)

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Nanosecond-Pulsed Perovskite Light-Emitting Diodes at High Current Density

Lianfeng Zhao et al.

Summary: This study presents high-speed PeLEDs, driven by nanosecond electrical pulses, with improved device design and material considerations. The fast operation of PeLEDs allows access to transient charge carrier dynamics and reveals new electroluminescence quenching pathways. Additionally, integrated DFB gratings enhance directional light emission and forward radiation output.

ADVANCED MATERIALS (2021)

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Pulsed-Laser Detectors Based on Metal Halide Perovskites

Yalun Xu et al.

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CO2 doping of organic interlayers for perovskite solar cells

Jaemin Kong et al.

Summary: A fast and reproducible doping method has been reported in this study, involving bubbling a spiro-OMeTAD:LiTFSI solution with CO2 under ultraviolet light. This method quickly promotes p-type doping of spiro-OMeTAD, resulting in significantly higher conductivity without the need for any post-treatments.

NATURE (2021)

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Review Optics

Advances in solution-processed near-infrared light-emitting diodes

Maria Vasilopoulou et al.

Summary: Near-infrared light-emitting diodes fabricated by solution-processed means using organic semiconductors, halide perovskites, and colloidal quantum dots have become a promising technological platform for various applications including biomedical, night vision, surveillance, and optical communications. Despite achieving high external quantum efficiencies exceeding 20%, challenges remain in achieving high radiance, reducing efficiency roll-off, and extending operating lifetime. This review summarizes recent advances in emissive materials synthetic methods and device key attributes contributing to improved performance of the fabricated light-emitting devices.

NATURE PHOTONICS (2021)

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Editorial Material Optics

Characterization of stability and challenges to improve lifetime in perovskite LEDs

Seung-Je Woo et al.

Summary: The low stability of perovskite light-emitting diodes (PeLEDs) poses the biggest challenge to the commercialization of PeLED displays. Analyzing and improving the stability of PeLEDs is crucial, and suggestions provided in this paper may enhance the operational lifetime of PeLEDs.

NATURE PHOTONICS (2021)

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Prospects and challenges of colloidal quantum dot laser diodes

Heeyoung Jung et al.

Summary: Colloidal quantum dots have the potential to provide solution-processable lasers, but face challenges in overcoming optical gain decay and poor stability of QD solids at high current densities. Recent progress has been made in developing electrically pumped optical gain devices operating at ultrahigh current densities.

NATURE PHOTONICS (2021)

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Huachao Zai et al.

Summary: Metal halide perovskites are considered the most promising candidate for the next-generation Photovoltaics due to their superior optoelectronic properties and low cost. However, the poor stability of Perovskite solar cells is largely attributed to ion migration, which remains a crucial challenge for improving their stability.

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Tuning Laser Threshold within the Large Optical Gain Bandwidth of Halide Perovskite Thin Films

Kwangdong Roh et al.

Summary: This study demonstrates continuously tunable single-mode lasing from halide perovskite thin films at room temperature, with a wide spectral range covered. The use of chirped Bragg gratings for optical feedback allows fine-tuning of the lasing output, enabling the lowest possible lasing threshold throughout the gain bandwidth, crucial for designing highly efficient electrically pumped lasers.

ACS PHOTONICS (2021)

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Efficient Amplified Spontaneous Emission from Solution-Processed CsPbBr3 Nanocrystal Microcavities under Continuous Wave Excitation

Modestos Athanasiou et al.

Summary: Solution-processed lasers are cost-effective and compatible with a wide range of photonic resonators, allowing for mass production of flexible, lightweight, and disposable devices. Lead halide perovskite nanocrystals (LHP NCs) show great potential as active mediums for solution-processed lasers due to their optical gain properties and defect-tolerant nature. By optimizing the polymer mirrors, resonators with high Q-factors can be produced, supporting amplified spontaneous emission in the green spectrum under continuous wave excitation with low thresholds. The CsPbBr3 NCs embedded in polymeric Bragg reflectors show promising results in terms of output intensity amplification and radiative rate increase when compared to reference microcavity structures.

ACS PHOTONICS (2021)

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Article Chemistry, Multidisciplinary

Electrical Pumping of Perovskite Diodes: Toward Stimulated Emission

Changsoon Cho et al.

Summary: The perovskite diode structure reported in this study demonstrates stable operation at high current density and optically excited ASE, which is a crucial step towards achieving electrically pumped stimulated emission. The design principles involving the formation of a large angle waveguide mode and reduction of parasitic absorption losses are essential for obtaining a positive gain for stimulated emission in diodes.

ADVANCED SCIENCE (2021)

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Article Nanoscience & Nanotechnology

Room-temperature continuous-wave vertical-cavity surface-emitting lasers based on 2D layered organic-inorganic hybrid perovskites

Hongbo Zhang et al.

Summary: This study demonstrated lasing emission of (PEA)(2)PbI4 in a vertical microcavity under continuous pumping, overcoming the challenge of CW pumped lasing in 2D lead halide perovskites. The high crystallization, excellent thermal stability, and outstanding optical properties of the obtained (PEA)(2)PbI4 single crystal enabled robust VCSEL operation at room temperature with an ultra-low threshold.

APL MATERIALS (2021)

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Surface plasmon coupling regulated CsPbBr3 perovskite lasers in a metal-insulator-semiconductor structure

Maogao Gong et al.

Summary: Researchers have successfully constructed an Ag/SiO2/CsPbBr3 hybrid structure based on surface plasmons, achieving significant enhancement of CsPbBr3 radiative recombination efficiencies and further verifying the effectiveness of optimizing the thickness of the SiO2 layer.

RSC ADVANCES (2021)

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Review Chemistry, Physical

Reality or fantasy-Perovskite semiconductor laser diodes

Wei Gao et al.

Summary: The current research focuses on the lasing performance of optically pumped perovskite lasers and the control of carrier transport and recombination properties. While challenges remain in fabricating electrically pumped perovskite lasers, a new manufacturing strategy based on the successful development of organic semiconductor laser diodes is proposed.

ECOMAT (2021)

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Review Chemistry, Multidisciplinary

Mitigating ion migration in perovskite solar cells

Enbing Bi et al.

Summary: Intrinsic ion migration in metal halide perovskite absorber layers and interfaces severely limits the device stability of perovskite solar cells. Efforts to mitigate this issue have been made, but it remains a formidable challenge in commercializing PSCs. While degradation of PSCs caused by extrinsic factors has been studied and relieved to some extent, intrinsic ion migration remains a major obstacle to commercialization.

TRENDS IN CHEMISTRY (2021)

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Amplified spontaneous emission in thin films of quasi-2D BA3MA3Pb5Br16 lead halide perovskites

Maria Luisa De Giorgi et al.

Summary: The study investigates the ASE properties of multilayered quasi-2D BA(3)MA(3)Pb(5)Br(16) films and sheds light on the emission processes of quasi-2D lead bromide perovskites. The presence of a minor fraction of the high temperature phase above 190 K strongly affects the PL and ASE properties, with ASE only observed between 13 K and 230 K.

NANOSCALE (2021)

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Revealing long-range orbit-orbit interaction between coherent light-emitting excitons occurring in amplified spontaneous emission in CsPbBr3 microstructures

Miaosheng Wang et al.

Summary: This paper discusses the establishment of long-range orbit-orbit interaction between coherent light-emitting excitons in CsPbBr3 microrods during the generation of amplified spontaneous emission (ASE). The study shows that optical generation of orbital polarizations with the same direction can greatly enhance the ASE amplitude, providing evidence for the role of long-range orbit-orbit interaction in developing coherent light-emitting excitons towards ASE in metal halide perovskites.

JOURNAL OF MATERIALS CHEMISTRY C (2021)

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Toward Electrically Pumped Organic Lasers: A Review and Outlook on Material Developments and Resonator Architectures

Qi Zhang et al.

Summary: Organic lasers have seen decades of development with promising applications in various fields. However, the challenge of realizing electrically pumped organic lasers remains due to the inherent drawbacks of organic semiconductors.

ADVANCED PHOTONICS RESEARCH (2021)

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Threshold Size Effects in the Patterned Crystallization of Hybrid Halide Perovskites for Random Lasing

Jingyun Hu et al.

Summary: A threshold effect in periodical patterning of hybrid halide perovskites and a directional output coupling effect in incoherent random lasing from patterned materials have been reported. The confinement of the random crystallization process is strongly dependent on the width of grating grooves, which can be optimized by tuning the patterning periods. The best lasing performance is achieved for a grating period of 10 μm, which corresponds to the highest quality of crystal strips.

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Carrier Dynamics and Evaluation of Lasing Actions in Halide Perovskites

Jiajun Qin et al.

Summary: Metal halide perovskites have shown rapid development in various optoelectronic devices due to their superior optoelectronic properties. The impact of carrier density on the optoelectronic behavior and lasing actions at high carrier densities have been discussed. An outlook on perovskite-based electrically pumped lasers has been provided.

TRENDS IN CHEMISTRY (2021)

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Quasi-2D lead halide perovskite gain materials toward electrical pumping laser

Chenyang Zhao et al.

Summary: Quasi two-dimensional lead halide perovskite materials exhibit excellent performance in photoelectric devices, with flexible structure and quantum-well structures for efficient energy transfer and high exciton utilization, benefiting the performance of perovskite LEDs and lasers. The characteristics of bulky organic cations contribute to improved stability, moisture tolerance, and defects passivation.

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Triplet management for efficient perovskite light-emitting diodes

Chuanjiang Qin et al.

NATURE PHOTONICS (2020)

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Factors that Limit Continuous-Wave Lasing in Hybrid Perovskite Semiconductors

Yufei Jia et al.

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Optically Pumped Lasing from Hybrid Perovskite Light-Emitting Diodes

Hoyeon Kim et al.

ADVANCED OPTICAL MATERIALS (2020)

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Exciton-Polariton Properties in Planar Microcavity of Millimeter-Sized Two-Dimensional Perovskite Sheet

Xiaoli Zhang et al.

ACS APPLIED MATERIALS & INTERFACES (2020)

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Tailoring Dispersion of Room-Temperature Exciton-Polaritons with Perovskite-Based Subwavelength Metasurfaces

Nguyen Ha My Dang et al.

NANO LETTERS (2020)

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