☆ 4.5 Review

A Review on Lead-Free-Bi0.5Na0.5TiO3 Based Ceramics and Films: Dielectric, Piezoelectric, Ferroelectric and Energy Storage Performance

JOURNAL OF INORGANIC AND ORGANOMETALLIC POLYMERS AND MATERIALS (2022)

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Visible photoresponse of TiO2 nanotubes in comparison to that of nanoparticles and anodic thin film

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Summary: This study synthesized TiO2 with different morphologies using an electrochemical method and investigated the effects of high-temperature annealing on the structures and substrates. Anodic TiO2 nanotubes, annealed under an Ar environment, were found to extend the photoresponse to the visible region, showing potential for enhancing photoelectrochemical performances.

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Piezoelectric enhancement and vacancy defect reduction of lead-free Bi0.5Na0.5TiO3-based thin films

Feier Ni et al.

Summary: Lead-free piezoelectric thin films (BNT-BKT-xBNZ) were prepared by a sol-gel method and the influence of Bi(Ni0.5Zr0.5)O3 content on the properties was investigated. The BNT-BKT-0.02BNZ thin film showed the best electrical and piezoelectric properties with great potential for applications.

CERAMICS INTERNATIONAL (2022)

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Article Materials Science, Ceramics

Crystalline texture analyses of sputtered BiFeO3 thick films on Si with a large polarization

Hanfei Zhu et al.

Summary: By quantitatively analyzing the texture characteristics of the rhombohedral BiFeO3 thick films and adding the contribution from non-textured grains to the preferential growth under compressive strain, the study further explains the ultra-high polarizations of the films.

CERAMICS INTERNATIONAL (2022)

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Article Materials Science, Ceramics

Dielectric and energy storage properties of (La,Li)x[(Bi,Na)BaSrCa]1-xTiO3 high-entropy perovskite ceramics

Chenhe Zhou et al.

Summary: A series of high-entropy perovskite ceramics with excellent dielectric properties and energy storage efficiency were successfully synthesized, suggesting entropy engineering as a viable strategy for tailoring material properties.

CERAMICS INTERNATIONAL (2022)

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Article Materials Science, Ceramics

Realising high comprehensive energy storage performance of BaTiO3-based perovskite ceramics via La(Zn1/2Hf1/2)O3 modification

Dan Meng et al.

Summary: Novel Pb-free BT-xLZH ceramics were designed and synthesized through conventional solid-phase technology, showing excellent electrical performance and thermal stability, with the potential to be a new generation of energy-saving and environmentally friendly dielectric capacitors.

CERAMICS INTERNATIONAL (2022)

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Article Engineering, Multidisciplinary

Simultaneously achieving high energy-storage efficiency and density in Bi-modified SrTiO3-based relaxor ferroelectrics by ion selective engineering

Yuqin Ding et al.

Summary: Through ion selective engineering, Bi-modified SrTiO3 solid-solution ceramics demonstrate excellent performance in energy efficiency, energy density, and thermal stability, offering potential solutions for electrostatic energy storage applications.

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A review of piezoelectric energy harvesting tiles: Available designs and future perspective

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Influence of sodium trimetaphosphate on glycine phosphite single crystals grown by modified thermal gradient method

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Synthesis and properties of lead-free BNT-BT-xCZ ceramics as high-temperature dielectricsY

Thomas Schulz et al.

Summary: Bulk ceramic samples of the perovskite series were prepared using the conventional solid-state route, with careful characterization of Bi2O3 raw materials being essential. X-ray diffraction analysis revealed the formation of perovskite main phase, and samples with higher CaZrO3 fraction showed a flattening of permittivity-temperature curves along with low dielectric losses.Samples with x = 0.2 exhibited a temperature stable permittivity of epsilon(r) approximate to 600 with small dielectric losses, qualifying them as suitable high temperature capacitor dielectric materials.

MATERIALS RESEARCH BULLETIN (2022)

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Article Chemistry, Physical

Enhanced energy-storage performance in BNT-based lead-free dielectric ceramics via introducing SrTi0.875Nb0.1O3

Lukang Wu et al.

Summary: This study reports on an excellent lead-free ferroelectric ceramic with outstanding energy storage capability, relaxor behavior, and breakdown strength, suitable for pulsed power devices in low-consumption systems. The study provides a simple and effective guideline for acquiring high-performance dielectric materials.

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Review Multidisciplinary Sciences

Shedding light on the energy applications of emerging 2D hybrid organic-inorganic halide perovskites

Neng Li et al.

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Interrelation between lattice structures and polarization in high Curie temperature piezoelectric Na0.5Bi4.46Ce0.04Ti4-xCoxOy ceramics

Yuandong Zuo et al.

Summary: The enhanced piezoelectric performance with high piezoelectric coefficient (d(33)) and high Curie temperature (T-c) has been achieved by replacing Ti4+ with Co3+ in lead-free piezoelectrics.

CERAMICS INTERNATIONAL (2022)

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Improving bone regeneration with composites consisting of piezoelectric poly(L-lactide) and piezoelectric calcium/manganese co-doped barium titanate nanofibers

Tianyi Zheng et al.

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Article Chemistry, Physical

Orientation dependent intrinsic and extrinsic contributions to the piezoelectric response in lead-free (Na0.5K0.5)NbO3 based films

Jin Luo et al.

Summary: The intrinsic and extrinsic contributions to the piezoelectric response in (Na0.5K0.5)NbO3 (KNN) based lead-free piezoelectric films are investigated with different crystallographic orientations. The results show that the (100)-oriented film has the highest piezoelectric response, attributed to the extrinsic contribution stimulated by the external electric field, despite the higher dielectric constant and remnant polarization in the (110) and (111)-oriented films.

JOURNAL OF ALLOYS AND COMPOUNDS (2022)

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Synthesis mechanisms and effects of BaTiO3 doping on the optical properties of Bi0.5Na0.5TiO3 lead-free ceramics

Subramani Supriya

JOURNAL OF SOLID STATE CHEMISTRY (2022)

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Study of vacancy ordered double perovskites In2PtX6 (X = Cl, Br, I) for solar cells and renewable energy, alternative of hybrid perovskites

Aiyeshah Alhodaib

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Synthesis of ternary copper antimony sulfide via solventless thermolysis or aerosol assisted chemical vapour deposition using metal dithiocarbamates

Fadiyah Makin et al.

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SCIENTIFIC REPORTS (2022)

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BNNT-ZnO QDs nanocomposites for improving piezoelectric nanogenerator and piezoelectric properties of boron nitride nanotube

Jaeho Shim et al.

Summary: In this study, high-performance piezoelectric devices based on BNNT-ZnO quantum dots nanocomposites were developed to improve piezoelectric properties in the radial direction. Through the combination of zinc oxide quantum dots and boron nitride nanotubes, the piezoelectric coefficient and charge coefficient were significantly increased, showing potential for innovative materials and devices in energy generation.

NANO ENERGY (2022)

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Article Chemistry, Physical

Enhanced strain and electrostrictive properties in lead-free BNT-based ceramics via rare earth doping

Anping Deng et al.

Summary: Rare earth ion doping has a significant effect on the phase structure, microstructure, strain, and electrostrictive properties of lead-free BNT-based ceramics. Moderate La3+ ion doping can drive the ceramics to nonergodic or ergodic relaxor states, resulting in enhanced strain response and high converse piezoelectric coefficient.

JOURNAL OF MATERIOMICS (2022)

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Article Materials Science, Ceramics

Enhancement of energy-storage properties in BiFeO3-based lead-free bulk ferroelectrics

Hui Tang et al.

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CERAMICS INTERNATIONAL (2022)

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Article Materials Science, Ceramics

Highly (00l)-textured BiFeO3 thick films integrated on stainless steel foils with an optimized piezoelectric performance

Jing Yan et al.

Summary: Piezoelectric BiFeO3 films were successfully prepared on stainless steel foils and exhibited enhanced ferroelectric and dielectric properties. The optimized heterostructure achieved large piezoelectric coefficients for applications in actuators and energy harvesters.

JOURNAL OF THE EUROPEAN CERAMIC SOCIETY (2022)

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Article Materials Science, Multidisciplinary

Highly tunable multifunctional rare earth based Bi0.5-xCexNa0.5TiO3 perovskites via site selective doping engineering

Subramani Supriya

Summary: High-quality lead-free relaxor-ferroelectric BCNT electroceramics were fabricated using the modified Pechini method, and the influence of cerium dopant on the material properties was studied. The doping affected the density and sintering temperature, but had a positive effect on crystallinity. BCNT ceramics showed increased grain size and significant changes in shrinkage, making them suitable for commercial applications such as electrode systems and multi-layered structures.

MATERIALS CHEMISTRY AND PHYSICS (2022)

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Dielectric, piezoelectric and magnetic behavior of CoFe2O4/BNT-BT0.08 monolayer thin films composites

Marin Cernea et al.

Summary: This study reports on the monolayer composite thin films with magnetic and piezoelectric properties. CoFe2O4 and BNT-BT0.08 composite thin films were prepared by spin coating method and characterized. The results show that increasing the magnetic phase enhances both magnetization and coercivity while decreasing the dielectric constant. The monolayer structures exhibit superior properties compared to bilayer composites.

MATERIALS SCIENCE AND ENGINEERING B-ADVANCED FUNCTIONAL SOLID-STATE MATERIALS (2022)

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Progress on perovskite materials for energy application

Gobeng R. Monama et al.

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RESULTS IN CHEMISTRY (2022)

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Proceedings Paper Materials Science, Multidisciplinary

Facile wet chemical synthesis and electrochemical performance of double perovskite-La2NiMnO6 for energy storage application

Jashandeep Singh et al.

Summary: We report the synthesis and characterization of the double perovskite electrode material La2NiMnO6 prepared by a facile wet chemical sol-gel method for energy storage application. The La2NiMnO6 electrode exhibits pseudocapacitive behavior and a specific capacitance of 478.2 F/g at a scan rate of 2 mV/s.

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Article Chemistry, Physical

Comparison between layered Pt3Te4 and PtTe2 for electrocatalytic reduction reactions

Subramani Supriya et al.

Summary: In this study, layered Pt3Te4 and PtTe2 were successfully synthesized and characterized, showing promising electrocatalytic properties for hydrogen evolution and oxygen reduction reactions. The direct synthesis of these compounds from respective elements resulted in monoclinic and trigonal crystal structures, indicating potential applications in future catalysis.

FLATCHEM (2021)

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Article Materials Science, Ceramics

Macrodomain structure formed in (Sr0.7Bi0.20.1)TiO3-modified Bi0.5Na0.4 K0.1TiO3 thin film

Liuxue Xu et al.

Summary: Introduction of (Sr0.7Bi0.2 0.1)TiO3 into Bi0.5Na0.4 K0.1TiO3 thin films successfully improved their properties with the principle of optimal tolerance factor. (1-x)BNKT-xSBT lead free piezoelectric thin films were deposited on substrates by the sol-gel method, showing improvements in ferroelectric and piezoelectric properties especially in the BNKT-0.10SBT thin film where macrodomain structure formation was observed.

CERAMICS INTERNATIONAL (2021)

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Large-area and efficient perovskite light-emitting diodes via low-temperature blade-coating

Shenglong Chu et al.

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NATURE COMMUNICATIONS (2021)

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Temperature stable (1-x)(0.9Na0.5Bi0.5TiO3-0.1BiAlO3)-xNaTaO3 ceramics and capacitors with ultra-wide operational range

Han Zhao et al.

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JOURNAL OF ALLOYS AND COMPOUNDS (2021)

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Ultrahigh energy density in short-range tilted NBT-based lead-free multilayer ceramic capacitors by nanodomain percolation

Hongfen Ji et al.

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ENERGY STORAGE MATERIALS (2021)

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An investigation on cubic and monoclinic phase coexistence in sol-gel derived LaFeO3-Na0.5Bi0.5TiO3 ceramics

Surinder Singh et al.

Summary: LaFeO3 modified Sodium Bismuth Titanate (NBT) with varying LaFeO3 content were successfully synthesized via sol-gel method. The XRD and Raman spectra confirmed the phase purity and microstructure of the samples. Ferroelectric behavior decreased with doping, with some samples showing paramagnetic or weak ferromagnetic characteristics. The absence of magnetic ordering was confirmed in certain samples through ZFC and FC magnetization curves.

JOURNAL OF ALLOYS AND COMPOUNDS (2021)

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Review Chemistry, Physical

Perovskite materials as superior and powerful platforms for energy conversion and storage applications

Priyanshu Goel et al.

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NANO ENERGY (2021)

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Enhanced energy storage efficiency by modulating field-induced strain in BaTiO3-Bi(Ni2/3Ta1/3)O3 lead-free ceramics

Huayu Zhao et al.

Summary: By introducing the BNT component to modify BT ceramics, the field-induced strain was reduced and the breakdown strength was enhanced, resulting in higher energy storage efficiency for the BT-BNT ceramics.

CERAMICS INTERNATIONAL (2021)

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Fabrication of poly (vinylidene fluoride) films by ultrasonic spray coating; uniformity and piezoelectric properties

Sepide Taleb et al.

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The energy-storage performance and dielectric properties of (0.94-x) BNT-0.06BT-xST thin films prepared by sol-gel method

Yanjiang Xie et al.

Summary: By controlling the amount of SrTiO3 introduced into the BNT-BT thin films, the maximum polarization and dielectric properties of the films can be enhanced, leading to high energy-storage density and low dielectric loss under certain conditions.

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(Bi0.5Na0.5)TiO3-based relaxor ferroelectrics with simultaneous high energy storage properties and remarkable charge-discharge performances under low working electric fields for dielectric capacitor applications

Xinyu Zhao et al.

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CERAMICS INTERNATIONAL (2021)

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Strengthened magnetoelectric multiferroic response in (K0.5Na0.5[Nb1-xFex/2Mnx/2]O3) ceramics

K. Shalini et al.

MATERIALS LETTERS (2020)

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Large electrostrain in low-temperature sintered NBT-BT-0.025FN incipient piezoceramics

Kai Liu et al.

JOURNAL OF THE AMERICAN CERAMIC SOCIETY (2020)

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Field-induced polarization response and energy storage behavior of lead-free BNT-BKT-SZ films

M. Afifi et al.

CERAMICS INTERNATIONAL (2020)

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Transverse piezoelectric properties of Mn-doped Bi0.5Na0.5TiO3 thin films

Bich Thuy Nguyen et al.

CURRENT APPLIED PHYSICS (2020)

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Significantly improved recoverable energy density and ultrafast discharge rate of Na0.5Bi0.5TiO3-based ceramics

Di Hu et al.

CERAMICS INTERNATIONAL (2020)

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Enhanced mechanical energy harvesting capability in sodium bismuth titanate based lead-free piezoelectric

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Effects of (K0.5Na0.5)(Nb0.96Sb0.04)O3 on microstructure and electrical properties of BNT-based piezoelectric ceramics

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Observation of enhanced electrostrictive strain in (1-2x)Na0.5Bi0.5TiO3-xBaTiO3-xBiAlO3 lead-free ceramics

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Site occupancy and electric-field induced strain response of Er-doped (Bi0.4Na0.4Sr0.2)TiO3 ceramics

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Enhanced energy storage performance in Sn doped Sr0.6(Na0.5Bi0.5)0.4TiO3 lead-free relaxor ferroelectric ceramics

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Enhanced energy density and thermal stability in relaxor ferroelectric Bi0.5Na0.5TiO3-Sr0.7Bi0.2TiO3 ceramics

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Role of tricritical triple point type morphotropic phase boundary (multiple crystalline phases) on energy storage density in Bi0.5Na0.5TiO3 based solid solution

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Huazhang Zhang et al.

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Composite BNT-BT0.08/CoFe2O4 with core-shell nanostructure for piezoelectric and ferromagnetic applications

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Tailoring frequency-insensitive large field-induced strain and energy storage properties in (Ba0.85Ca0.15)(Zr0.1Ti0.9)O3-modified (Bi0.5Na0.5)TiO3 lead-free ceramics

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