期刊
EPL
卷 139, 期 2, 页码 -出版社
IOP Publishing Ltd
DOI: 10.1209/0295-5075/ac7d0a
关键词
-
资金
- University of Chinese Academy of Sciences
- NSFC [12034019]
This article discusses the importance of aqueous dielectrics in soft- and bio-nano matter systems and reviews the existing continuum phenomenological approaches. It also explores important conceptual issues for the development of a more fundamental continuum theory of liquid dielectrics and proposes a generalized approach to the dielectric behavior of such systems.
Aqueous dielectrics are ubiquitous in soft- and bio-nano matter systems. 'The theoretical description of such systems in terms of continuum (macroscopic) theory remains a serious challenge. In this perspective we first review the existing continuum phenomenological approaches that have been developed in the past decades. In order to describe a path to advance continuum theory beyond these approaches we then take recourse to the Onsager-Dupuis theory of the dielectric behaviour of ice, which, for the case of a solid dielectric, exemplified important conceptual issues we deem relevant for the development of a more fundamental continuum theory of liquid dielectrics. Subsequently, we discuss our recently proposed continuum field theory of structured dielectrics, which provides a generalized approach to the dielectric behavior of such systems. Copyright (C) 2022 EPLA
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