☆ 4.8 Review

Bimetallic nanoparticles meet polymeric carbon nitride: Fabrications, catalytic applications and perspectives

COORDINATION CHEMISTRY REVIEWS (2022)

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Review Engineering, Environmental

Defective polymeric carbon nitride: Fabrications, photocatalytic applications and perspectives

Jinjuan Yang et al.

Summary: This paper discusses the enhancement of visible light activity in polymeric carbon nitride (CN) through defect control, summarizing methods for preparing defective CN. The paper also delves into the progress of defective CN in various applications such as water oxidation, hydrogen production, CO2 reduction, etc.

CHEMICAL ENGINEERING JOURNAL (2022)

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Review Chemistry, Multidisciplinary

Encapsulated Metal Nanoparticles for Catalysis

Chuanbo Gao et al.

Summary: Encapsulating metal nanoparticles in nanoshells or nanopores is a promising strategy to enhance stability and selectivity, taking advantage of the synergy between the metal nanoparticles and encapsulating materials. This approach also allows for improved catalytic properties and enables tandem catalysis in various applications.

CHEMICAL REVIEWS (2021)

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Article Chemistry, Physical

Defect engineering in polymeric carbon nitride photocatalyst: Synthesis, properties and characterizations

Longbo Jiang et al.

Summary: This review discusses the effects of vacancy defects on CN photocatalysts, highlighting the tuning of photoelectric properties and photocatalytic performance. Various characterization methods are summarized, providing a basis for further research and development in this field.

ADVANCES IN COLLOID AND INTERFACE SCIENCE (2021)

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Review Chemistry, Multidisciplinary

More is Different: Synergistic Effect and Structural Engineering in Double-Atom Catalysts

Yiran Ying et al.

Summary: Double-atom catalysts (DACs) have emerged as a novel frontier in heterogeneous catalysis, showing improved catalytic activity through synergistic effects while maintaining high atomic utilization efficiency, good selectivity, and stability. Current research focuses on the design, experimental and theoretical progress, and practical applications of DACs in various catalytic reactions.

ADVANCED FUNCTIONAL MATERIALS (2021)

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Article Engineering, Environmental

Graphitic carbon nitride (g-C3N4)-based nanostructured materials for photodynamic inactivation: Synthesis, efficacy and mechanism

Yongsheng Ni et al.

Summary: Photodynamic inactivation using graphitic carbon nitride (g-C3N4) has been widely researched for sterilization, with nanostructured materials showing great potential in enhancing its efficacy. This review systematically analyzed studies on g-C3N4-based nanostructured materials, discussing strategies, light sources, targeted organisms, and future perspectives.

CHEMICAL ENGINEERING JOURNAL (2021)

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Article Chemistry, Physical

Facile construction of composition-tuned ruthenium-nickel nanoparticles on g-C3N4 for enhanced hydrolysis of ammonia borane without base additives

Ziqian Wang et al.

Summary: The study successfully achieved the in-situ fabrication of RuNi alloy nanoparticles with tuned compositions using graphitic carbon nitride as a support without additional stabilizing ligands. The optimized catalyst exhibited excellent catalytic activity with high recyclability, showing potential for generating hydrogen through ammonia borane hydrolysis.

INTERNATIONAL JOURNAL OF HYDROGEN ENERGY (2021)

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Review Chemistry, Inorganic & Nuclear

Metal nanoparticles in ionic liquids: Synthesis and catalytic applications

Marina M. Seitkalieva et al.

Summary: The development of metal nanoparticle chemistry in ionic liquids has made a significant impact on fields such as catalysis, energy research, nanotechnology, and materials science. Various methods for producing metal nanoparticles in ILs are highlighted, with a focus on catalytic activity in different reactions.

COORDINATION CHEMISTRY REVIEWS (2021)

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Article Chemistry, Applied

FeCo alloy@N-doped graphitized carbon as an efficient cocatalyst for enhanced photocatalytic H-2 evolution by inducing accelerated charge transfer

Sibo Chen et al.

Summary: A novel noble-metal-free FeCo@NGC cocatalyst was successfully fabricated and showed outstanding performance in photocatalytic H-2 evolution. The optimized FeCo@NGC/g-C3N4 catalyst achieved boosted visible light driven photocatalytic activity, highlighting the potential of noble-metal-free bimetallic nano-alloys as inexpensive and efficient cocatalysts for solar applications.

JOURNAL OF ENERGY CHEMISTRY (2021)

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Article Chemistry, Physical

In-situ synthesis of novel ternary CdS/PdAg/g-C3N4 hybrid photocatalyst with significantly enhanced hydrogen production activity and catalytic mechanism exploration

Jianfeng Gao et al.

Summary: A ternary CdS/PdAg/g-C3N4 hybrid photocatalyst was synthesized using a simple sonochemical method, exhibiting excellent photocatalytic H-2 evolution performance up to 3098.3 mu mol g(-1) h(-1), which is 968.2 times higher than that of g-C3N4. The catalyst also showed an apparent quantum yield of 9.6% at 420 nm, and the enhancement of charge separation efficiency was confirmed through various tests including photoluminescence, surface photovoltage, and electron spin resonance. This work proposes a reasonable catalytic mechanism for the ternary hybrid photocatalyst, showing potential for designing high efficient ternary hybrid photocatalysts.

APPLIED CATALYSIS B-ENVIRONMENTAL (2021)

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Article Engineering, Chemical

Strategic combination of nitrogen-doped carbon quantum dots and g-C3N4: Efficient photocatalytic peroxydisulfate for the degradation of tetracycline hydrochloride and mechanism insight

Haoyun Chen et al.

Summary: Photo-assisted peroxydisulfate (PDS) activation has shown great potential in pollution control, and in this study, a metal-free nitrogen-doped carbon quantum dots (N-CQDs) modified g-C3N4 composite was used to effectively remove tetracycline hydrochloride (HTC) in wastewater under visible light. The combination of PDS and N-CQDs acted as electron acceptors, transferring photogenerated charges and successfully activating PDS for pollutant degradation. The up-conversion effect of N-CQDs contributed to enhanced visible light absorption, providing an innovative approach for synthesizing binary metal-free carbonaceous photocatalysts.

SEPARATION AND PURIFICATION TECHNOLOGY (2021)

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Review Chemistry, Physical

Electrochemical CO2 Reduction to Ethanol with Copper-Based Catalysts

Dilan Karapinar et al.

Summary: This Review highlights the importance and challenges of electrochemical CO2 reduction for ethanol production, categorizing and evaluating the performance of copper-based catalysts to aid in the design of more efficient catalysts for selective ethanol formation.

ACS ENERGY LETTERS (2021)

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Article Engineering, Environmental

Core-shell Ag@nitrogen-doped carbon quantum dots modified BiVO4 nanosheets with enhanced photocatalytic performance under Vis-NIR light: Synergism of molecular oxygen activation and surface plasmon resonance

Jin Zhang et al.

Summary: In this study, a visible-near infrared responsive photocatalyst was developed by integrating BiVO4 nanosheets and core-shell structured Ag@N-CQDs nanoparticles, exhibiting improved photocatalytic performance. The composite material showed surface plasmon resonance and molecular oxygen activation, enhancing charge separation, light absorption, and oxidation ability during photocatalysis. This work provides new insight into designing advanced structure of visible-near infrared responsive photocatalysts.

CHEMICAL ENGINEERING JOURNAL (2021)

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Review Biotechnology & Applied Microbiology

Synthesis and characterization of magnetic nanoparticles, and their applications in wastewater treatment: A review

Saurabh Shukla et al.

Summary: MNPs are efficient tools for wastewater treatment, providing target specificity and cost-effectiveness, and can efficiently remove various pollutants through multiple mechanisms.

ENVIRONMENTAL TECHNOLOGY & INNOVATION (2021)

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Article Chemistry, Analytical

Dynamically Monitoring the Photodeposition of Single Cocatalyst Nanoparticles on Semiconductors via Fluorescence Imaging

Hua Su et al.

Summary: Loading cocatalysts through photodeposition is a promising method for improving semiconductor photocatalytic activities, but the growth kinetics of cocatalysts during the process has remained largely unknown. This study dynamically imaged the photodeposition of single cocatalysts on semiconductors and revealed self-limited growth and significant heterogeneities. Programmable photodeposition and dissolution of CoxP was also achieved using a focused laser beam. This work provides insights into optimizing photodeposition for designing more efficient photocatalysts.

ANALYTICAL CHEMISTRY (2021)

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Article Chemistry, Physical

Bimetallic synergetic regulating effect on electronic structure in cobalt/vanadium co-doped carbon nitride for boosting photocatalytic performance

Hongjun Dong et al.

Summary: The photocatalytic activity of bimetallic co-doped g-C3N4 can be significantly enhanced due to improved charge separation efficiency and visible light harvest ability. Density functional theory investigations show that the incorporation of Co/V into g-C3N4 results in a bimetallic synergetic regulating effect on electronic structure, improving physical, optical, and photoelectrochemical properties.

APPLIED CATALYSIS B-ENVIRONMENTAL (2021)

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Review Chemistry, Inorganic & Nuclear

Strategies to extend near-infrared light harvest of polymer carbon nitride photocatalysts

Longbo Jiang et al.

Summary: In order to enhance the efficiency of g-C3N4 photocatalysts under solar light (UV about 5%, visible light about 43%, NIR light about 52%), recent progress of NIR-driven g-C3N4 based photocatalysts has been reviewed. Various strategies have been summarized to broaden the light absorption of g-C3N4 to NIR light region, and the diverse photocatalytic applications of NIR-driven g-C3N4 photocatalysts have been outlined.

COORDINATION CHEMISTRY REVIEWS (2021)

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Article Engineering, Environmental

Optimizing the metal-support interactions at the Pd-polymer carbon nitride Mott-Schottky heterojunction interface for an enhanced electrocatalytic hydrodechlorination reaction

Kanxin Jiang et al.

Summary: A novel strategy was reported to optimize metal-support interactions at a Mott-Schottky heterojunction interface by band engineering of the semiconductor support, enhancing the metal's electrocatalytic hydrodechlorination (EHDC) performance. Phosphorus (P) doping in PCN significantly boosted EHDC efficiency on Pd, with Pd/P-PCN-0.25 achieving a peak specific activity of 0.172 min^-1 cm^Pd^-2, outperforming most reported catalysts.

JOURNAL OF HAZARDOUS MATERIALS (2021)

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Article Chemistry, Physical

Enhancement of the Oxygen Reduction Reaction Activity of Pt by Tuning Its d-Band Center via Transition Metal Oxide Support Interactions

Fuma Ando et al.

Summary: The study investigated the enhancement of the oxygen reduction reaction (ORR) activity of platinum nanoparticles using transition metal oxide supports, finding that the ORR activity depends significantly on the atomic ratio of metals in the metal oxide composite and the type of metal oxide support. It was observed that a catalyst with a d-band center approximately 0.2 eV lower than that of platinum exhibited maximal ORR activity.

ACS CATALYSIS (2021)

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Article Chemistry, Physical

Confined sub-nanometer PtCo clusters as a highly efficient and robust electrocatalyst for the hydrogen evolution reaction

Fei Guo et al.

Summary: Sub-nanometer PtCo clusters confined into the small pores of ZIF-8 derived N-doped nanomaterials show exceptional hydrogen evolution reaction (HER) catalytic activity and durability, with a mass activity of 13.83 A mg(-1) at an overpotential of 20 mV. The outstanding HER activity is attributed to the charge redistribution and the lower d-band center on Pt due to the enhanced coupling of electrons in the d orbitals between Pt and Co, which increases the HER kinetics and activity.

JOURNAL OF MATERIALS CHEMISTRY A (2021)

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Article Chemistry, Applied

Mesoporous graphitic carbon nitride-supported binary MPt (M: Co, Ni, Cu) nanoalloys as electrocatalysts for borohydride oxidation and hydrogen evolution reaction

Raisa C. P. Oliveira et al.

CATALYSIS TODAY (2020)

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Article Chemistry, Physical

Bimetallic co-effect of Au-Pd alloyed nanoparticles on mesoporous silica modified g-C3N4 for single and simultaneous photocatalytic oxidation of phenol and reduction of hexavalent chromium

Sulagna Patnaik et al.

JOURNAL OF COLLOID AND INTERFACE SCIENCE (2020)

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Article Chemistry, Physical

Carbon nitride embedded with transition metals for selective electrocatalytic CO2 reduction

Chunmei Ding et al.

APPLIED CATALYSIS B-ENVIRONMENTAL (2020)

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Article Chemistry, Physical

AuPd alloy nanoparticles decorated graphitic carbon nitride as an excellent photocatalyst for the visible-light-enhanced Suzuki-Miyaura cross-coupling reaction

Siyavash Kazemi Movahed et al.

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Xiangyu Guo et al.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2020)

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Review Chemistry, Physical

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R. Kavitha et al.

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Facile synthesis of iron and cerium co-doped g-C3N4 with synergistic effect to enhance visible-light photocatalytic performance

Tao Pan et al.

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Ultrathin porous g-C3N4 nanosheets modified with AuCu alloy nanoparticles and C-C coupling photothermal catalytic reduction of CO2 to ethanol

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Zhiliang Jin et al.

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Shi-Long Xu et al.

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Boosting visible-light-driven hydrogen evolution from formic acid over AgPd/2D g-C3N4 nanosheets Mott-Schottky photocatalyst

Chao Wan et al.

CHEMICAL ENGINEERING JOURNAL (2020)

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Visible-Light-Driven Multichannel Regulation of Local Electron Density to Accelerate Activation of O-H and B-H Bonds for Ammonia Borane Hydrolysis

Shengbo Zhang et al.

ACS CATALYSIS (2020)

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IrCo alloy nanoparticles supported on N-doped carbon for hydrogen evolution electrocatalysis in acidic and alkaline electrolytes

Chunxiao Wu et al.

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Graphitic carbon nitride (g-C3N4)-based membranes for advanced separation

Yang Wang et al.

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Monodisperse NiPd alloy nanoparticles decorated on mesoporous graphitic carbon nitride as a catalyst for the highly efficient chemoselective reduction of α,β-unsaturated ketone compounds

Cetin Bayrak et al.

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Yongyong Cao et al.

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Strategic synergy: advances in the shape control of bimetallic nanoparticles with dilute alloyed surfaces

Haeyoon Jung et al.

CURRENT OPINION IN COLLOID & INTERFACE SCIENCE (2019)

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Electrocatalytic methanol oxidation over Cu, Ni and bimetallic Cu-Ni nanoparticles supported on graphitic carbon nitride

Izabela S. Pieta et al.

APPLIED CATALYSIS B-ENVIRONMENTAL (2019)

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Article Chemistry, Physical

Ni-Mo nanoparticles as co-catalyst for drastically enhanced photocatalytic hydrogen production activity over g-C3N4

Xin Han et al.

APPLIED CATALYSIS B-ENVIRONMENTAL (2019)

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JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2019)

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Review Chemistry, Physical

A multifunctional platform by controlling of carbon nitride in the core-shell structure: From design to construction, and catalysis applications

Donghui He et al.

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Electron directed migration cooperated with thermodynamic regulation over bimetallic NiFeP/g-C3N4 for enhanced photocatalytic hydrogen evolution

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Enhanced formic acid dehydrogenation by the synergistic alloying effect of PdCo catalysts supported on graphitic carbon nitride

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Au/Pd/g-C3N4 nanocomposites for photocatalytic degradation of tetracycline hydrochloride

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Size- and density-controlled photodeposition of metallic platinum nanoparticles on titanium dioxide for photocatalytic applications

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Photocatalytic dehydrogenation of formic acid promoted by a superior PdAg@g-C3N4 Mott-Schottky heterojunction

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Novel NiPt alloy nanoparticle decorated 2D layered g-C3N4 nanosheets: a highly efficient catalyst for hydrogen generation from hydrous hydrazine

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NiCu single atom alloys catalyze the C-H bond activation in the selective non- oxidative ethanol dehydrogenation reaction

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A magnetically recoverable bimetallic Au-FeNPs decorated on g-C3N4 for efficient photocatalytic degradation of organic contaminants

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Au-Pd@g-C3N4 as an Efficient Photocatalyst for Visible-Light Oxidation of Benzene to Phenol: Experimental and Mechanistic Study

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