期刊
CHEMOSPHERE
卷 307, 期 -, 页码 -出版社
PERGAMON-ELSEVIER SCIENCE LTD
DOI: 10.1016/j.chemosphere.2022.135873
关键词
Sludge; Biochar; Fenton-like; Degradation; Organic pollutant; Dewatering
资金
- Program for the National Natural Science Foundation of China [51879101, 51579098, 51779090, 51709101, 51809090]
- National Program for Support of Top -Notch Young Professionals of China
- National Innovative Talent Promotion Program of China
- Program for Changjiang Scholars and Innovative Research Team in University [IRT-13R17]
- Hunan Provincial Science and Technology Plan Project [2018SK20410]
- Science and Technology Innovation Program of Hunan Province [2020RC4014]
In today's society, the preparation of wastewater sludge into sludge biochar nanomaterials (SBCs) for resource utilization has become a promising method due to its advantages of complex composition, wide range of raw materials, and the presence of various transition metals with catalytic properties. Heterogeneous Fenton processes using SBCs as catalyst carriers have shown great potential in pollutant removal. This review provides an overview of SBCs synthesis methods, discusses the effects of different synthesis methods on their physicochemical properties, and reviews their successful applications in organic pollutant degradation, sediment remediation, and sludge dewatering. The review explores the mechanisms occurring with different metals as active sites and highlights the satisfactory degradation efficiency and stability of SBCs. An outlook on the future development of SBCs is also provided.
In today's society, wastewater sludge has become solid waste, and the preparation of wastewater sludge into sludge biochar nanomaterials (SBCs) for resource utilization has become a promising method. SBCs have advantages over other biomasses, including their complex composition, wide range of raw materials, and especially the presence of various transition metals with catalytic properties. Heterogeneous Fenton processes using SBCs as catalyst carriers have shown great potential in the removal of pollutants. In this review, the synthesis methods of SBCs are reviewed and the effects of different synthesis methods on their physicochemical properties are discussed. Furthermore, the successful applications of raw SBCs, metal-modified SBCs, and Fenton sludge-SBCs in organic pollutant degradation, sediment remediation, and sludge dewatering are reviewed. The mechanisms occurring with different metals as active sites are explored, and the review shows that the degradation efficiency and stability of SBCs are very satisfactory. We also provide an outlook on the future development of SBCs. We hope that this review will help readers gain a clearer and deeper understanding of SBCs and promote the development of SBCs.
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