☆ 4.6 Review

Recent Advances in Host-Guest Supramolecular Hydrogels for Biomedical Applications

CHEMISTRY-AN ASIAN JOURNAL (2022)

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Summary: This study reports the engineering of functional hydrogels that respond to physiological and pathological acidic microenvironments using transformable nanoparticles. These nanoparticles can protect mice from gastric injury and be used for triggerable and sustained drug delivery for treating inflammatory diseases. The engineered transformable nanoparticles have great potential for tissue injury protection and site-specific/local delivery of therapeutic agents.

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3D Bioprinting of Heterogeneous Constructs Providing Tissue-Specific Microenvironment Based on Host-Guest Modulated Dynamic Hydrogel Bioink for Osteochondral Regeneration

Wenli Dai et al.

Summary: A novel dynamic hydrogel for 3D bioprinting heterogeneous cell-laden constructs to mimic osteochondral tissue has been developed. This bioink, consisting of dopamine-functionalized GelMA and acrylate beta-cyclodextrin, demonstrates improved cell adaptability, cell adhesion, and mechanical strength with tunable modulus. By utilizing the sustained drug release from beta-cyclodextrin, a heterogeneous construct with different moduli mimicking the osteochondral microenvironment is achieved.

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Review Chemistry, Multidisciplinary

Supramolecular Hydrogels: Design Strategies and Contemporary Biomedical Applications

Jasmin Omar et al.

Summary: This article provides a detailed overview of the dynamic chemistry and design strategies behind supramolecular hydrogel formation, as well as the potential applications in the field of medicine and the considerations for further development.

CHEMISTRY-AN ASIAN JOURNAL (2022)

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Tough, Self-Adhesive, Antibacterial, and Recyclable Supramolecular Double Network Flexible Hydrogel Sensor Based on PVA/Chitosan/Cyclodextrin

Xin Fan et al.

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Advances in the Stimuli-Responsive Injectable Hydrogel for Controlled Release of Drugs

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Antioxidant Thermogelling Formulation for Burn Wound Healing

Minting Liu et al.

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CHEMISTRY-AN ASIAN JOURNAL (2022)

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Flexible polymeric patch based nanotherapeutics against non-cancer therapy

Houjuan Zhu et al.

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Advances in sustainable polymeric materials from lignocellulosic biomass

S. Sugiarto et al.

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PLA-lignin nanofibers as antioxidant biomaterials for cartilage regeneration and osteoarthritis treatment

Ruiming Liang et al.

Summary: In this study, lignin-based nanofibers were developed as antioxidative scaffolds for cartilage tissue engineering. The nanofibers showed the ability to protect cells from oxidative stress and promote cartilage regeneration. These findings suggest that lignin nanofibers could be used for the treatment of osteoarthritis.

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Supramolecular Hydrogels via Light-Responsive Homoternary Cross-Links

Lei Zou et al.

Summary: This study utilized host-guest physical cross-linking to prepare supramolecular hydrogels, with the introduction of asymmetric azobenzene into copolymers enabling temperature and light responsiveness control. UV light was used to disrupt the supramolecular motif leading to a gel-to-sol transition, with rapid hydrogel recovery achieved through thermal relaxation of azobenzene.

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Polysaccharide-Based Supramolecular Hydrogel for Efficiently Treating Bacterial Infection and Enhancing Wound Healing

Jing Wang et al.

Summary: Supramolecular hydrogels are highly biocompatible materials that show outstanding capabilities in drug loading through electrostatic interactions and host-guest inclusion. Biological experiments demonstrate that these hydrogels exhibit strong antibacterial effects and promote wound healing efficiently.

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Novel supramolecular self-healing silk fibroin-based hydrogel via host-guest interaction as wound dressing to enhance wound healing

Rui Yu et al.

Summary: A novel self-healing SF-based hydrogel was developed through dual crosslinking for enhanced wound dressing performance and as a drug carrier with controlled release, showing great potential in wound healing.

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Supramolecular self-healing materials via host-guest strategy between cyclodextrin and specific types of guest molecules

Masoumeh Mohamadhoseini et al.

Summary: The article mainly discusses the different strategies of fabricating HG supramolecular self-healable materials using host-guest interactions between beta-CD and various guest molecules. Comparing different strategies helps to properly address the challenges of this field in the future.

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Rapid self-healing and self-adhesive chitosan-based hydrogels by host-guest interaction and dynamic covalent bond as flexible sensor

Zhijun Ren et al.

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A triple-stimuli responsive supramolecular hydrogel based on methoxy-azobenzene-grafted poly(acrylic acid) and β-cyclodextrin dimer

Hongchao Yan et al.

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Ultrasensitive Exhaled Breath Sensors Based on Anti-Resonant Hollow Core Fiber with In Situ Grown ZnO-Bi2O3 Nanosheets

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Multi-Component Hydrogel Beads Incorporated with Reduced Graphene Oxide for pH-Responsive and Controlled Co-Delivery of Multiple Agents

Sreekanth Reddy Obireddy et al.

Summary: The study reports the generation of multi-component hydrogel beads incorporated with reduced graphene oxide, which are shown to be more effective in inhibiting the growth of MCF-7 cells. The drug release sustainability of the beads is affected by the pH of the release medium, increasing in neutral pH but decreasing in acidic environments.

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Multifunctional Self-Healing Dual Network Hydrogels Constructed via Host-Guest Interaction and Dynamic Covalent Bond as Wearable Strain Sensors for Monitoring Human and Organ Motions

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Prediction of oral hepatotoxic dose of natural products derived from traditional Chinese medicines based on SVM classifier and PBPK modeling

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IEEE SENSORS JOURNAL (2017)

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Shear-Thinning Supramolecular Hydrogels with Secondary Autonomous Covalent Crosslinking to Modulate Viscoelastic Properties In Vivo

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Rational Design of Network Properties in Guest-Host Assembled and Shear-Thinning Hyaluronic Acid Hydrogels

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JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2012)

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PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA (2012)

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SOFT MATTER (2012)

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Review Chemistry, Multidisciplinary

Deep Inside Cucurbiturils: Physical Properties and Volumes of their Inner Cavity Determine the Hydrophobic Driving Force for Host-Guest Complexation

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Supramolecular hydrogels based on cyclodextrin-polymer polypseudorotaxanes: materials design and hydrogel properties

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Self-assembled supramolecular hydrogels formed by biodegradable PEO-PHB-PEO triblock copolymers and α-cyclodextrin for controlled drug delivery

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Injectable drug-delivery systems based on supramolecular hydrogels formed by poly(ethylene oxide) and α-cyclodextrin

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JOURNAL OF BIOMEDICAL MATERIALS RESEARCH PART A (2003)

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