4.7 Article

Highly thin film with aerosol-deposited perovskite quantum dot/metal oxide composite for perfect color conversion and luminance enhancement

期刊

CHEMICAL ENGINEERING JOURNAL
卷 441, 期 -, 页码 -

出版社

ELSEVIER SCIENCE SA
DOI: 10.1016/j.cej.2022.135991

关键词

Perovskite quantum dots; Aerosol deposition; Color conversion; Scattering effect; OLED backlight

资金

  1. National Research Foundation of Korea (NRF) under the Ministry of Science, ICT & Future Planning (Basic Science Research Program) [2021R1A5A6002853, 2020R1A2C1004943, 2021M3H4A3A01062960, 2020M3A7B4002030, 2020R1A6A1A03048004, 2020R1G1A1102045, 2020R1F1A1073491]
  2. Nano-Material Technology Development Program [2017M3A7B4041696]
  3. Kwangwoon University in 2021, Korea Institute for Advancement of Technology (KIAT) - Korea Government (MOTIE) [P0012451, 2019R1A6C1010052]
  4. National Research Foundation of Korea [2020R1F1A1073491, 2020R1G1A1102045] Funding Source: Korea Institute of Science & Technology Information (KISTI), National Science & Technology Information Service (NTIS)

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This study presents a novel process for producing thin luminescent films that completely convert colors and enhance light intensity. The films are prepared by co-depositing perovskite quantum dots and metal oxide particles as color conversion layers and scattering agents. The films can be directly deposited on blue organic light-emitting diodes using ultrasonic-assisted aerosol deposition (UAD), eliminating the need for color filters.
Erstwhile, displays using down-converting color changing medium utilized color filters as an essential part of clarifying the trade-off between true colors and transmittance. In this study, we report the development of a novel, smart process for producing thin luminescent films that completely convert colors and enhance light intensity. Highly dense films are prepared by the co-deposition of perovskite quantum dots and metal oxide particles as color conversion layers and scattering agents, respectively. These layers can be directly deposited on blue organic light-emitting diodes using ultrasonic-assisted aerosol deposition (UAD). This method can allow displays using a down-conversion system to streamline the process due to absence of color filters. Using this method, films can be a minimum of 3 mu m thick for complete conversion of blue light, a quarter that of inkjetprinted films. We demonstrate 7,353 cd m(-2) in green and 411 cd m(-2) in red converted emissions with no blue light leakage. Furthermore, the developed technique was shown to be compatible with versatile patterning processes. For example, UAD may be combined with a fine-metal shadow mask to produce a pattern of 30-mu m-diameter dots. Even without using a mask, the method still produces a pattern of 13 mu m wide lines. This system provides a new approach that may serve as an alternative to inkjet printing.

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