4.7 Article

Physical properties of crystalline NaNbO3 thin film grown on Sr2Nb3O10 nanosheets at low temperatures for piezoelectric energy harvesters

期刊

APPLIED SURFACE SCIENCE
卷 593, 期 -, 页码 -

出版社

ELSEVIER
DOI: 10.1016/j.apsusc.2022.153464

关键词

SN nanosheet seed layer; Low-temperature deposition process; [001]-oriented crystalline NNO thin film; Piezoelectric energy harvester

资金

  1. National R&D Programs through the National Research Foundation of Korea (NRF) - Ministry of Science and ICT [2020R1A2B5B01002063]
  2. KU-KIST Graduate School Program of Korea University
  3. National Research Foundation of Korea [2020R1A2B5B01002063] Funding Source: Korea Institute of Science & Technology Information (KISTI), National Science & Technology Information Service (NTIS)

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A Sr2Nb3O10 (SN) monolayer was used as a template for the growth of crystalline NaNbO3 (NNO) thin films at low temperatures. The [001]-oriented NNO film displayed good insulating properties and a high piezoelectric coefficient, making it a potential candidate for piezoelectric energy harvesters.
A Sr2Nb3O10 (SN) monolayer deposited on Pt/SiO2/Si (PSS) was employed as the template for the growth of crystalline NaNbO3 (NNO) thin films at low temperatures. The [001]-oriented crystalline NNO film was effectively grown on SN/PSS at 250 degrees C. This NNO film showed a small epsilon(r) of 115, along with good insulating properties with a low leakage-current density (4.5 x 10(-6) A/cm(2) at 0.3 MV/cm). This NNO film displayed a large d(33) of 123 pC/N, which is the largest d(33) value for NNO films to date. Moreover, it shows a very large d(33) x g(33) (14.8 x 10(-12) m(2)/N), which is the figure of merit for the power of piezoelectric energy harvesters (PEHs). The NNO film grown on SN/Ni at 250 degrees C for the fabrication of PEH also demonstrated dielectric and piezoelectric characteristics. The NNO PEH exhibited a high power density (2.1 mu W/mm(3)), indicating that the [001]-oriented NNO film grown on the SN seed layer is a good candidate for PEH. Moreover, this NNO film can be deposited on a polymer substrate and utilized as a future flexible device owing to its very low growth temperature and good physical properties.

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