期刊
APPLIED CATALYSIS B-ENVIRONMENTAL
卷 309, 期 -, 页码 -出版社
ELSEVIER
DOI: 10.1016/j.apcatb.2022.121273
关键词
delta-MnO2 ; Catalytic removal; Human-emitted VOCs; Indoor air; Ventilation
资金
- Science and Technology Innovation Program of Shunde of Foshan City [2130218002526]
Efficient removal of human-emitted gaseous pollutants in indoor air can reduce energy consumption. This study reported a catalytic method for the room and low-temperature removal of human-emitted acetic acid. Ultrathin delta-MnO2 nanoribbons were synthesized and could transform acetic acid into CO2 even at room temperature.
Efficient removal of human-emitted gaseous pollutants in indoor air may greatly reduce ventilation-related energy consumption, however few efforts have been made. Here we reported the room and low-temperature catalytic removal of a human-emitted odorant -acetic acid with odor threshold of 5.6 ppb. Ultrathin delta-MnO2 nanoribbons (delta-MnO2 UTNRs) with the thickness of 1-1.5 nm and aspect ratio of 200-600 was synthesized, which produced abundant active oxygen species such as hydroxyl radicals and superoxide at room temperature without light irradiation. Accordingly, as-prepared delta-MnO2 UTNRs could transform acetic acid into CO2 even at room temperature. The 100% one-through removal capacity for ~1 ppm acetic acid was about 20 mg/g, and it could be completely regenerated at 14 & nbsp;C-0. This study opens a new research direction and demonstrates that it is possible to catalytically remove human-emitted gaseous pollutant at low and even at room temperature.
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