期刊
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
卷 61, 期 37, 页码 -出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/anie.202208587
关键词
Desalination; Hydrogels; MoS2; Photo-Vapor Conversion; Solar Steam Generation
资金
- National Natural Science Foundation of China [51978638, 51778598, 51478449]
- Scientific Research Funds of Huaqiao University [20BS109]
In this study, a scalable MoS2-based porous hydrogel with good mechanical stability and salt resistance was successfully prepared. The hydrogel exhibited impressive evaporation rate and photothermal conversion efficiency under sunlight, and maintained high and stable photothermal properties for a prolonged period. Therefore, it holds promise as a feasible device for seawater desalination.
Interfacial photo-vapor conversion has been suggested as a cost-effective and sustainable technology for seawater desalination. However, the conversion performance was still limited by some drawbacks, like salt accumulation and poor mechanical stability. Herein, a scalable MoS2-based porous hydrogel (SMoS2-PH) with good mechanical stability and salt resistance was successfully constructed through a crosslinking foaming polymerization method. With the high porosity (92.63 %), the SMoS2-PH performed an impressive evaporation rate of 3.297 kg m(-2) h(-1) and photothermal conversion efficiency of 93.4 % under 1-sun illumination. Most importantly, the SMoS2-PH could maintain high and stable photothermal properties for 15 days on the surface of seawater. We believe that the excellent salt resistance, the high photothermal conversion efficiency, the ease of scale preparation method and the available commercial MoS2 make the SMoS2-PH a promising device for full-scale seawater desalination.
作者
我是这篇论文的作者
点击您的名字以认领此论文并将其添加到您的个人资料中。
推荐
暂无数据