期刊
ADVANCED MATERIALS
卷 34, 期 32, 页码 -出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/adma.202204298
关键词
carrier mobility; Corbino disks; domain walls; ferroelectrics; magnetoresistance
类别
资金
- Engineering and Physical Sciences Research Council (EPSRC) [EP/P02453X/1]
- UKRI Future Leaders Fellowship programme [MR/T043172/1]
- US-Ireland R&D Partnership Programme [USI 120]
Recent research has revealed the presence of magnetoresistance in domain walls, providing insight into the conduction properties of homointerfaces.
Recently, electrically conducting heterointerfaces between dissimilar band insulators (such as lanthanum aluminate and strontium titanate) have attracted considerable research interest. Charge transport and fundamental aspects of conduction have been thoroughly explored. Perhaps surprisingly, similar studies on conceptually much simpler conducting homointerfaces, such as domain walls, are not nearly so well developed. Addressing this disparity, magnetoresistance is herein reported in approximately conical 180 degrees charged domain walls, in partially switched ferroelectric thin-film single-crystal lithium niobate. This system is ideal for such measurements: first, the conductivity difference between domains and domain walls is unusually large (a factor of 10(13)) and hence currents driven through the thin film, between planar top and bottom electrodes, are overwhelmingly channeled along the walls; second, when electrical contact is made to the top and bottom of the domain walls and a magnetic field is applied along their cone axes, then the test geometry mirrors that of a Corbino disk: a textbook arrangement for geometric magnetoresistance measurement. Data imply carriers with extremely high room-temperature Hall mobilities of up to approximate to 3700 cm(2) V-1 s(-1). This is an unparalleled value for oxide interfaces (and for bulk oxides) comparable to mobilities in other systems seen at cryogenic, rather than at room, temperature.
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