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Regulation of Quantum Wells Width Distribution in 2D Perovskite Films for Photovoltaic Application

ADVANCED FUNCTIONAL MATERIALS (2022)

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Summary: This article reports the scalable printing of high-quality Dion-Jacobson (DJ) perovskite thin films via tailoring crystallization kinetics. The perovskite films obtained through the optimized crystallization process exhibit enhanced crystallinity, highly vertical orientation, and graded phase distribution, resulting in efficient charge generation and ultrafast interphase charge transfer. The devices processed from the ternary solvent show improved stability under stimuli with light, heat, and humidity, benefiting from their superb phase stability. This work demonstrates an important advancement in scalable deposition of DJ perovskite thin films for efficient and stable photovoltaic devices.

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