4.7 Article

Communication: The cluster vapor to cluster solid transition

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JOURNAL OF CHEMICAL PHYSICS
卷 144, 期 17, 页码 -

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AMER INST PHYSICS
DOI: 10.1063/1.4948784

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Until now, depletion induced transitions have been the hallmark of multicomponent systems only. Monte Carlo simulations reveal a depletion-induced phase transition from cluster vapor to cluster solid in a one-component fluid with competing short range and long range interactions. This confirms a prediction made by earlier theoretical work. Analysis of renormalized cluster-cluster and cluster-vapor interactions suggests that a cluster liquid is also expected within a very narrow range of model parameters. These insights could help identify the mechanisms of clustering in experiments and assist the design of colloidal structures through engineered self-assembly. Published by AIP Publishing.

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