期刊
JOURNAL OF CHEMICAL PHYSICS
卷 145, 期 3, 页码 -出版社
AMER INST PHYSICS
DOI: 10.1063/1.4958967
关键词
-
资金
- University of Wisconsin Foundation
Before 2015, heterodyne-detected sum-frequency-generation experiments on the air-water interface showed the presence of a positive feature at low frequency in the imaginary part of the susceptibility. However, three very recent experiments indicate that this positive feature is in fact absent. Armed with a better understanding, developed by others, of how to calculate sum-frequency spectra, we recalculate the spectrum and find good agreement with these new experiments. In addition, we provide a revised interpretation of the spectrum. Published by AIP Publishing.
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