☆ 4.7 Review

Perovskite Single-Crystal Solar Cells: Advances and Challenges

SOLAR RRL (2022)

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Engineering the Hole Extraction Interface Enables Single-Crystal MAPbI3 Perovskite Solar Cells with Efficiency Exceeding 22% and Superior Indoor Response

Ning Li et al.

Summary: In this study, hydrophobic P3HT molecules were successfully incorporated into the hole transport layer of perovskite single crystals, resulting in reduced interface and bulk defect density, suppressed nonradiative recombination, accelerated charge transport, and extraction. This led to a significantly enhanced open-circuit voltage and efficiency, making it the highest values achieved for MAPbI(3) single-crystal solar cells. Additionally, the incorporation of P3HT resulted in superior weak light response and an indoor photovoltaic efficiency of 39.2% at 1000 lux irradiation.

ADVANCED ENERGY MATERIALS (2022)

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Managing Growth and Dimensionality of Quasi 2D Perovskite Single-Crystalline Flakes for Tunable Excitons Orientation

Marco Cinquino et al.

Summary: A conceptually innovative approach to easily tune the quantum well width in lead iodide perovskite single-crystalline flakes is presented by controlling the supersaturation levels of the precursor solution. Manipulating the number of inorganic layers allows for the orientation of excitons to be modified, with an increase in the number of inorganic layers enhancing the out-of-plane component of excitons. The combined advances in synthesis and optical characterization provide insights into exciton behavior in low-dimensional perovskite, paving the way for the design of materials with improved optoelectronic characteristics.

ADVANCED MATERIALS (2021)

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Article Chemistry, Multidisciplinary

Triple-Cation and Mixed-Halide Perovskite Single Crystal for High-Performance X-ray Imaging

Yucheng Liu et al.

Summary: This study reports the successful controlled incorporation of methylammonium (MA(+)), cesium (Cs+), and bromine (Br-) ions into the FAPbI3 lattice to grow inch-sized stable perovskite single crystal (FAMACs SC), resulting in X-ray detectors with superior sensitivity and stability.

ADVANCED MATERIALS (2021)

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Review Chemistry, Multidisciplinary

The 2D Halide Perovskite Rulebook: How the Spacer Influences Everything from the Structure to Optoelectronic Device Efficiency

Xiaotong Li et al.

Summary: This review provides guidelines on choosing spacers and incorporating them into crystalline materials and optoelectronic devices for two-dimensional halide perovskites. The comprehensive understanding of the effects of spacers on structure, properties, and device performance can accelerate the discovery and application of novel 2D materials in high-performance devices.

CHEMICAL REVIEWS (2021)

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Review Chemistry, Multidisciplinary

Halide Perovskite Semiconductor Lasers: Materials, Cavity Design, and Low Threshold

Qing Zhang et al.

Summary: Perovskite lasers, combining the advantages of inorganic and organic semiconductors, have emerged as excellent candidates for solution-processable lasers. They offer cost-effectiveness, low threshold, high coherence, and multicolor tunability. Despite rapid development and various types of lasers and devices, critical issues such as mass fabrication and applications still need to be addressed.

NANO LETTERS (2021)

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Mixed halide perovskites for spectrally stable and high-efficiency blue light-emitting diodes

Max Karlsson et al.

Summary: Achieving bright and efficient blue emission in metal halide perovskite light-emitting diodes has been challenging, but the authors demonstrate high EQE and spectrally stable blue light-emitting diodes based on mixed halide perovskites, with emission from 490 to 451nm by using a vapour-assisted crystallization technique.

NATURE COMMUNICATIONS (2021)

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Perovskite Single-Crystal Solar Cells: Going Forward

Bekir Turedi et al.

Summary: Perovskite single crystals have potential for high-efficiency photovoltaics, but higher trap density on surfaces poses a challenge; focusing on surface-trap management is crucial for maximizing the potential of single crystals.

ACS ENERGY LETTERS (2021)

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Tuning of the Berry curvature in 2D perovskite polaritons

Laura Polimeno et al.

Summary: By engineering the energy dispersion of polaritons in a strongly coupled organic-inorganic two-dimensional perovskite single-crystal microcavity, different Berry curvature distributions of polariton bands can be obtained. External magnetic field breaks time-reversal symmetry, leading to exciton Zeeman splitting and lifting the degeneracy of Hamilton diabolical points. This results in bands with non-zero integral Berry curvatures, which can be modified by tuning external parameters like temperature, magnetic field, and sample thickness.

NATURE NANOTECHNOLOGY (2021)

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Efficient perovskite solar cells via improved carrier management

Jason J. Yoo et al.

Summary: Metal halide perovskite solar cells have shown great potential to disrupt the silicon solar cell market with their improved performance, yet still face limitations in light-harvesting due to charge carrier recombination. Efforts to enhance charge carrier management offer a path to increase device performance and approach the theoretical efficiency limit of PSCs.

NATURE (2021)

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Crystallization of CsPbBr3 single crystals in water for X-ray detection

Jiali Peng et al.

Summary: Researchers have developed a low-temperature crystallization strategy to grow CsPbBr3 perovskite single crystals in water, which exhibit superior performance and show great potential for X-ray imaging with enhanced metrics.

NATURE COMMUNICATIONS (2021)

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Article Chemistry, Multidisciplinary

Improved Photostability in Fluorinated 2D Perovskite Single Crystals

Annalisa Coriolano et al.

Summary: The hydrophobic nature of the fluorinated component and the absence of grain boundary defects in two-dimensional perovskite single crystals lead to improved stability by creating a robust barrier that preserves the crystalline structure and hinders photo-degradation processes usually promoted by oxygen and moisture.

NANOMATERIALS (2021)

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Inch-sized high-quality perovskite single crystals by suppressing phase segregation for light-powered integrated circuits

Yucheng Liu et al.

Summary: An effective additive strategy was reported for growing high-quality 2-inch-sized FAMACs SCs, showing superior performance for potential applications in high-performance self-powered integrated circuit photodetectors.

SCIENCE ADVANCES (2021)

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Limits to Electrical Mobility in Lead-Halide Perovskite Semiconductors

Chelsea Q. Xia et al.

Summary: This study shows that polycrystalline films of metal-halide perovskites have electrical performance close to single crystals, with charge-carrier scattering mechanisms dominated by Frohlich scattering and grain-boundary scattering. Considering photon reabsorption can explain the large difference in charge-carrier diffusion lengths between single crystals and films.

JOURNAL OF PHYSICAL CHEMISTRY LETTERS (2021)

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Article Multidisciplinary Sciences

A polymer controlled nucleation route towards the generalized growth of organic-inorganic perovskite single crystals

Lin Ma et al.

Summary: Progress has been made in the growth of organic-inorganic lead halide perovskite single crystals, with a focus on efficient and large-size crystal growth. By utilizing a polymer-controlled nucleation process, the carrier lifetime of FAPbBr(3) single crystals has been significantly improved. This approach shows potential in optimizing solution-based crystal growth and advancing applications of perovskite single crystals.

NATURE COMMUNICATIONS (2021)

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Single crystal of two-dimensional mixed-halide copper-based perovskites with reversible thermochromism

Amr Elattar et al.

Summary: The synthesis of 2D Cu-based mixed-halide perovskite thin films has shown tunable band gap energy and reversible thermochromic behavior, with structural changes in the 2D crystal contributing to the thermochromism.

JOURNAL OF MATERIALS CHEMISTRY C (2021)

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22.8%-Efficient single-crystal mixed-cation inverted perovskite solar cells with a near-optimal bandgap

Abdullah Y. Alsalloum et al.

Summary: By utilizing a mixed-cation single-crystal absorber layer, the external quantum efficiency band edge can be redshifted, leading to increased short-circuit current densities and overall efficiencies.

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U1 snRNP regulates cancer cell migration and invasion in vitro

Jung-Min Oh et al.

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Low-Temperature Crystallization Enables 21.9% Efficient Single-Crystal MAPbI3 Inverted Perovskite Solar Cells

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Polymer-Controlled Growth and Wrapping of Perovskite Single Crystals Leading to Better Device Stability and Performance

Rohit Saraf et al.

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Designing Large-Area Single-Crystal Perovskite Solar Cells

Xiaomei Jiang et al.

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Enhancing Resistive Switching Performance and Ambient Stability of Hybrid Perovskite Single Crystals via Embedding Colloidal Quantum Dots

Adnan Younis et al.

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Jin Young Kim et al.

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A fabrication process for flexible single-crystal perovskite devices

Yusheng Lei et al.

NATURE (2020)

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Strain-activated light-induced halide segregation in mixed-halide perovskite solids

Yicheng Zhao et al.

NATURE COMMUNICATIONS (2020)

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Single Crystals: The Next Big Wave of Perovskite Optoelectronics

Banavoth Murali et al.

ACS MATERIALS LETTERS (2020)

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Tuning the Luminescence of Layered Halide Perovskites

Matthew D. Smith et al.

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Efficient, stable and scalable perovskite solar cells using poly(3-hexylthiophene)

Eui Hyuk Jung et al.

NATURE (2019)

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Prospects for low-toxicity lead-free perovskite solar cells

Weijun Ke et al.

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New tolerance factor to predict the stability of perovskite oxides and halides

Christopher J. Bartel et al.

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Single-Crystal MAPbI3 Perovskite Solar Cells Exceeding 21% Power Conversion Efficiency

Zhaolai Chen et al.

ACS ENERGY LETTERS (2019)

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Kinetically Stable Single Crystals of Perovskite-Phase CsPbI3

Daniel B. Straus et al.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2019)

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Mixed-halide perovskite synthesis by chemical reaction and crystal nucleation under an optical potential

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Two-dimensional hybrid perovskites sustaining strong polariton interactions at room temperature

A. Fieramosca et al.

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Material Design and Optoelectronic Properties of Three-Dimensional Quadruple Perovskite Halides

Yang-Peng Lin et al.

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Thermodynamically stabilized β-CsPbI3-based perovskite solar cells with efficiencies >18%

Yong Wang et al.

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Stable Bandgap-Tunable Hybrid Perovskites with Alloyed Pb-Ba Cations for High-Performance Photovoltaic Applications

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Toward Long-Term Stability: Single-Crystal Alloys of Cesium-Containing Mixed Cation and Mixed Halide Perovskite

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Fast Growth of Thin MAPbI3 Crystal Wafers on Aqueous Solution Surface for Efficient Lateral-Structure Perovskite Solar Cells

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Unravelling Light-Induced Degradation of Layered Perovskite Crystals and Design of Efficient Encapsulation for Improved Photostability

Hong-Hua Fang et al.

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Suppressed Ion Migration along the In-Plane Direction in Layered Perovskites

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ACS ENERGY LETTERS (2018)

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Perovskite light-emitting diodes based on spontaneously formed submicrometre-scale structures

Yu Cao et al.

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Multi-inch single-crystalline perovskite membrane for high-detectivity flexible photosensors

Yucheng Liu et al.

NATURE COMMUNICATIONS (2018)

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Quantitative Phase-Change Thermodynamics and Metastability of Perovskite-Phase Cesium Lead Iodide

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Understanding the Cubic Phase Stabilization and Crystallization Kinetics in Mixed Cations and. Halides Perovskite Single Crystals

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Cation Dynamics in Mixed-Cation (MA)x(FA)1-xPbI3 Hybrid Perovskites from Solid-State NMR

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Intrinsic Instability of Cs2In(I)M(III)X6 (M = Bi, Sb; X = Halogen) Double Perovskites: A Combined Density Functional Theory and Experimental Study

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Dopant compensation in alloyed CH3NH3PbBr3-xClx perovskite single crystals for gamma-ray spectroscopy

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Fast oxygen diffusion and iodide defects mediate oxygen-induced degradation of perovskite solar cells

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Single crystals of caesium formamidinium lead halide perovskites: solution growth and gamma dosimetry

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A formamidinium-methylammonium lead iodide perovskite single crystal exhibiting exceptional optoelectronic properties and long-term stability

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Single crystalline CH3NH3PbI3 self-grown on FTO/TiO2 substrate for high efficiency perovskite solar cells

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Bication lead iodide 2D perovskite component to stabilize inorganic α-CsPbI3 perovskite phase for high-efficiency solar cells

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Stabilizing the α-Phase of CsPbI3 Perovskite by Sulfobetaine Zwitterions in One-Step Spin-Coating Films

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Atomic Structures of CH3NH3PbI3 (001) Surfaces

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Solution-Grown CsPbBr3 Perovskite Single Crystals for Photon Detection

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Ruddlesden-Popper Hybrid Lead Iodide Perovskite 2D Homologous Semiconductors

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Band Gaps of the Lead-Free Halide Double Perovskites Cs2BiAgCl6 and Cs2BiAgBr6 from Theory and Experiment

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General Space-Confined On-Substrate Fabrication of Thickness-Adjustable Hybrid Perovskite Single-Crystalline Thin Films

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A Bismuth-Halide Double Perovskite with Long Carrier Recombination Lifetime for Photovoltaic Applications

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Sensitive X-ray detectors made of methylammonium lead tribromide perovskite single crystals

Haotong Wei et al.

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Screening in crystalline liquids protects energetic carriers in hybrid perovskites

Haiming Zhu et al.

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Incorporation of rubidium cations into perovskite solar cells improves photovoltaic performance

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David P. McMeekin et al.

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20-mm-Large Single-Crystalline Formamidinium-Perovskite Wafer for Mass Production of Integrated Photodetectors

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Entropy-driven structural transition and kinetic trapping in formamidinium lead iodide perovskite

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Investigation of CH3NH3PbI3 Degradation Rates and Mechanisms in Controlled Humidity Environments Using in Situ Techniques

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Giant switchable photovoltaic effect in organometal trihalide perovskite devices (vol 14, pg 193, 2014)

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Formamidinium lead trihalide: a broadly tunable perovskite for efficient planar heterojunction solar cells

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