☆ 4.5 Review

The application of nonthermal plasma in methanol synthesis via CO2 hydrogenation

ENERGY SCIENCE & ENGINEERING (2022)

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Selective oxidation of CH4 to CH3OH through plasma catalysis: Insights from catalyst characterization and chemical kinetics modelling

Yanhui Yi et al.

Summary: Using Ni-based catalysts in a plasma environment for the selective oxidation of methane to methanol is an efficient method with high selectivity and good catalytic stability. Chemical kinetics modeling shows that methanol is mainly produced through radical reactions. Improvements in catalyst characterization help promote methanol production and increase yield.

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Methanol synthesis from CO2 using Ni and Cu supported Fe catalytic system: Understanding the role of nonthermal plasma surface discharge

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Summary: This study combines nonthermal plasma (NTP) and thermal catalysis to directly convert CO2 to CH3OH using H-2. By testing a series of catalysts, it was found that 5 wt% CuO/Fe2O3/QW exhibited the best CO2 conversion and CH3OH selectivity. With this catalyst, the study achieved a CH3OH space-time yield of 9.32 mmol h(-1) gcat(-1), which is about two times higher than previous reported values.

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A Review of Non-Thermal Plasma Technology: A novel solution for CO2 conversion and utilization

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Summary: The conversion of CO2 into higher-value products using non-thermal plasma catalysis is a promising approach with great potential for enhancing reaction efficiency. Future research should focus on exploring different NTP sources, reactions, applications, and integrating CO2 conversion with capture technologies, while addressing current challenges and future prospects in this emerging field.

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A promising plasma-catalytic approach towards single-step methane conversion to oxygenates at room temperature

Piu Chawdhury et al.

Summary: Direct conversion of methane into chemicals and fuels under mild conditions is considered a significant achievement. Plasma-catalytic partial oxidation of methane to higher-value liquid fuels and chemicals over supported transition metal catalysts has shown promising results, with Fe/γ-Al2O3 demonstrating the highest methanol selectivity.

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Article Physics, Applied

Influence of ionic conductivity and dielectric constant of the catalyst on DBD plasma-assisted CO2 hydrogenation into methanol

Maxwell Quezada Feliz et al.

Summary: Dielectric barrier discharge (DBD) plasma technology is a promising method for converting CO2 to methanol at atmospheric pressure and temperatures below 100 degrees C. The choice of catalyst is crucial, and the ionic conductivity of the catalyst was identified as a key parameter in plasma-assisted CO2 hydrogenation, with lower conductivity leading to higher CO2 conversion rates.

JOURNAL OF PHYSICS D-APPLIED PHYSICS (2021)

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Review Chemistry, Physical

Methane to Methanol through Heterogeneous Catalysis and Plasma Catalysis

Shangkun Li et al.

Summary: This review summarizes the latest advances in heterogeneous catalysis and plasma catalysis for direct oxidation of methane to methanol (DOMTM), aiming to point out the differences between the two and provide insights into their reaction mechanisms, as well as implications for future development of highly selective catalysts for DOMTM.

CATALYSTS (2021)

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Review Chemistry, Multidisciplinary

CO2 conversion using catalyst-free and catalyst-assisted plasma-processes: Recent progress and understanding

Guoxing Chen et al.

Summary: The paper critically reviews the latest progress, present status, and future directions of CO2 conversion in various gaseous discharges. It emphasizes the advantages of catalytic CO2 decomposition in the plasma phase and systematically analyzes promising candidates among different plasma processes and available catalytic materials. This is important for further progress in the field and potential applications.

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Nitesh Joshi et al.

Summary: The study found that binary mixed metal oxides of NiO-Fe2O3 are more active than pure metal oxides, but increased NiO mixing leads to particle agglomeration. Plasma coupled with the catalyst significantly enhances CO2 conversion and CH3OH yield, showing a 5.8-fold improvement with 10NF at 200 degrees C compared to thermal catalysis.

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Nb2O5 as a radical modulator during oxidative dehydrogenation and as a Lewis acid promoter in CO2 assisted dehydrogenation of octane over confined 2D engineered NiO-Nb2O5-Al2O3

Majid D. Farahani et al.

Summary: Mesoporous 2D NiO-Nb2O5-Al2O3 nanorods were prepared via glycol-thermal synthesis for direct conversion of octane to octenes with high selectivity and conversion rate. The addition of Nb2O5 modified the confinement effect and metal support interaction, leading to optimal performance of the catalyst in the reaction process.

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Article Chemistry, Physical

CO2 conversion by plasma: how to get efficient CO2 conversion and high energy efficiency

Yongxiang Yin et al.

Summary: Converting CO2 into CO with plasma processing is a potential method to convert intermittent sustainable electricity into storable chemical energy. Challenges in developing this technology include achieving efficient CO2 conversion with high energy efficiency and proving its feasibility on an industrial scale.

PHYSICAL CHEMISTRY CHEMICAL PHYSICS (2021)

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Article Chemistry, Physical

Direct conversion of CO2 and CH4 into liquid chemicals by plasma-catalysis

Di Li et al.

APPLIED CATALYSIS B-ENVIRONMENTAL (2020)

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Review Chemistry, Multidisciplinary

Recent Advances in Carbon Dioxide Hydrogenation to Methanol via Heterogeneous Catalysis

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Single-pass transformation of syngas into ethanol with high selectivity by triple tandem catalysis

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Yong Sun et al.

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Highly dispersed Pt-based catalysts for selective CO2 hydrogenation to methanol at atmospheric pressure

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Net reduction of CO2 via its thermocatalytic and electrocatalytic transformation reactions in standard and hybrid processes

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NATURE CATALYSIS (2019)

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ACS CATALYSIS (2019)

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Atmospheric Pressure and Room Temperature Synthesis of Methanol through Plasma-Catalytic Hydrogenation of CO2

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CHEMICAL SOCIETY REVIEWS (2017)

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Challenges in the Greener Production of Formates/Formic Acid, Methanol, and DME by Heterogeneously Catalyzed CO2 Hydrogenation Processes

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A Comparative Study of NiO/Al2O3 Catalysts Prepared by Different Combustion Techniques for Octanal Hydrogenation

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Hydrogenation of CO2 to methanol and CO on Cu/ZnO/Al2O3: Is there a common intermediate or not?

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Understanding plasma catalysis through modelling and simulation-a review

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Mechanistic studies of methanol synthesis over Cu from CO/CO2/H2/H2O mixtures: The source of C in methanol and the role of water

Y. Yang et al.

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Efficiency of CO2 Dissociation in a Radio-Frequency Discharge

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Mechanism of Methanol Synthesis on Cu through CO2 and CO Hydrogenation

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